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Despite the widespread use of solution-processable hybrid organic-inorganic perovskites in photovoltaic and light-emitting applications, determination of their intrinsic charge transport parameters has been elusive due to the variability of…

材料科学 · 物理学 2019-06-26 Xin Yu Chin , Daniele Cortecchia , Jun Yin , Annalisa Bruno , Cesare Soci

Molecular triplet states can produce significant phosphorescence and act as a relay state for luminescence, such as in up-conversion processes. While this property makes triplet emitters interesting for organic light-emitting diodes…

介观与纳米尺度物理 · 物理学 2026-05-14 Li-Qing Zheng , Fábio J. R. Costa , Abhishek Grewal , Ruonan Wang , Fengmin Wang , Wei Li , Anna Rosławska , Klaus Kuhnke , Klaus Kern

In the previous decade, there has been a significant advancement in the performance of perovskite solar cells (PSCs), characterized by a notable increase in efficiency from 3.8% to 25%. Nonetheless, PSCs face many problems when we…

Despite the youthfulness of hybrid halide perovskite solar cells, their efficiencies are currently comparable to commercial silicon and have surpassed quantum-dots solar cells. Yet, the scalability of these devices is a challenge due to…

The incorporation of even small amounts of strontium (Sr) into lead-based quadruple cation hybrid perovskite solar cells results in a systematic increase of the open circuit voltage (Voc) in pin-type perovskite solar cells. We demonstrate…

Perovskite solar cells have potential to deliver terawatt-scale power via low-cost manufacturing. However, scaling is limited by slow, high-temperature annealing of the inorganic transport layers and the lack of reliable, large-area methods…

材料科学 · 物理学 2022-01-25 Julia E. Huddy , Youxiong Ye , William J. Scheideler

Metal halide perovskites (MHPs) are low-temperature processable hybrid semiconductor materials with exceptional performances that are revolutionizing the field of optoelectronic devices. Despite their great potential, commercial deployment…

Current technologies for X-ray detection rely on scintillation from expensive inorganic crystals grown at high-temperature, which so far has hindered the development of large-area scintillator arrays. Thanks to the presence of heavy atoms,…

仪器与探测器 · 物理学 2016-11-21 M. D. Birowosuto , D. Cortecchia , W. Drozdowski , K. Brylew , W. Lachmanski , A. Bruno , C. Soci

Two-dimensional halide perovskite nanoplatelets (NPLs) have exceptional light-emitting properties, including wide spectral tunability, ultrafast radiative decays, high quantum yields (QY), and oriented emission. To realize efficient…

Manipulating strong light-matter interaction in semiconductor microcavities is crucial for developing high-performance exciton polariton devices with great potentials in next-generation all-solid state quantum technologies. In this work, we…

介观与纳米尺度物理 · 物理学 2018-08-01 Qiuyu Shang , Shuai Zhang , Jie Chen , Pengfei Yang , Wei Li , Yanfeng Zhang , Qihua Xiong , Xinfeng Liu , Qing Zhang

Perovskite nanocrystals (PNCs) are promising building blocks for quantum photonic devices. Optical properties of PNCs can be enhanced by integration with optical cavities or nanoantennas. Designing such structures requires accurate size…

Singlet fission is a spin-allowed exciton multiplication process in organic semiconductors that converts one spin-singlet exciton to two triplet excitons. It offers the potential to enhance solar energy conversion by circumventing the…

Halide perovskite materials raised tremendous interest in recent years since their cheap fabrication, superior performance in both solar cell and light emitting diode (LED). Due to the existence of layered quantum well structure, quasi…

材料科学 · 物理学 2021-11-23 Wei Tang , Liting Tao , Tian Zhang , Yanjun Fang , Deren Yang , Linjun Li

Understanding the nature of the photoexcitation and ultrafast charge dynamics pathways in organic halide perovskite nanocubes and their aggregation into superlattices is key for the potential applications as tunable light emitters, photon…

Lead-halide perovskites have demonstrated astonishing increases in power conversion efficiency in photovoltaics over the last decade. The most efficient perovskite devices now outperform industry-standard multi-crystalline silicon solar…

应用物理 · 物理学 2023-02-20 Yi-Teng Huang , Sean R. Kavanagh , David O. Scanlon , Aron Walsh , Robert L. Z. Hoye

Electric force microscopy was used to record the light-dependent impedance spectrum and the probe transient photoconductivity of a film of butylammonium lead iodide, BA$_{2}$PbI$_{4}$, a 2D Ruddlesden--Popper perovskite semiconductor. The…

介观与纳米尺度物理 · 物理学 2020-06-02 Ali Moeed Tirmzi , Ryan P. Dwyer , Fangyuan Jiang , John A. Marohn

Lead halide perovskites (MAPbX3) have emerged as promising materials for photovoltaic and optoelectronic devices. However, their exceptional nonlinear properties have not been fully exploited in nanophotonics yet. Herein we fabricate MAPbX3…

应用物理 · 物理学 2019-04-03 Yubin Fan , Yuhan Wang , Nan Zhang , Wenzhao Sun , Yisheng Gao , Cheng-wei Qiu , Qinghai Song , Shumin Xiao

Exciton-phonon interactions govern the optical response of semiconductors, yet disentangling multiple coupling channels in lead halide perovskites remains challenging. We investigate CsPbBr3 microcrystals using photoluminescence, Raman and…

Metal-halide perovskites are a class of solution processed materials with remarkable optoelectronic properties such as high photoluminescence quantum yields and long carrier lifetimes, which makes them promising for a wide range of…

Layered halide perovskites are solution-processed natural heterostructures where quantum and dielectric confinement effects down to the nanoscale strongly influence the optical properties, leading to stabilization of bound excitons.…

材料科学 · 物理学 2022-12-09 Claudio Quarti , Giacomo Giorgi , Claudine Katan , Jacky Even , Maurizia Palummo