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Spatio-temporal shaping of electron beams is a bold frontier in electron microscopy, enabling new routes toward spatial-resolution enhancement, selective probing, low-dose imaging and faster data acquisition. Over the last decade, shaping…

The ability to modulate free electrons with light has emerged as a powerful tool to produce attosecond electron wavepackets. However, research has so far aimed at the manipulation of the longitudinal wave function component, while the…

光学 · 物理学 2023-06-14 F. Javier García de Abajo , Claus Ropers

Free electron beams such as those employed in electron microscopes have evolved into powerful tools to investigate photonic nanostructures with an unrivaled combination of spatial and spectral precision through the analysis of electron…

量子物理 · 物理学 2021-04-22 F. Javier García de Abajo , Valerio Di Giulio

Interfacing electrons and light enables ultrafast electron microscopy, quantum control of electrons, as well as new optical elements for high sensitivity imaging. Here we demonstrate for the first time programmable transverse electron beam…

Laser-based preparation, manipulation, and readout of the states of quantum particles has become a powerful research tool that has enabled the most precise measurements of time, fundamental constants, and electromagnetic fields. Laser…

量子物理 · 物理学 2018-12-12 O. Schwartz , J. J. Axelrod , S. L. Campbell , C. Turnbaugh , R. M. Glaeser , H. Müller

Controlled interaction of laser light with electron beams is fundamental for ultrafast electron microscopy and electron-based quantum optics, yet their direct coupling is forbidden in free space. Here we use longitudinally polarized light…

光学 · 物理学 2026-05-22 J. Kuttruff , L. Möhrle , L. Ciorciaro , L. Schmidt-Mende , P. Baum

The ability to tailor laser light on a chip using integrated photonics has allowed for extensive control over fundamental light-matter interactions in manifold quantum systems including atoms, trapped ions, quantum dots, and defect centers.…

Thanks to their exceptional spatial, spectral and temporal resolution, highly-coherent free-electron beams have emerged as powerful probes for material excitations, enabling their characterization even in the quantum regime. Here, we…

量子物理 · 物理学 2023-12-12 J. Abad-Arredondo , A. I. Fernández-Domínguez

We demonstrate the quantized transfer of photon energy and transverse momentum to a high-coherence electron beam. In an ultrafast transmission electron microscope, a three-dimensional phase modulation of the electron wavefunction is induced…

光学 · 物理学 2020-11-18 Armin Feist , Sergey V. Yalunin , Sascha Schäfer , Claus Ropers

Free-electron interactions with light and matter have long served as a cornerstone for exploring the quantum and ultrafast dynamics of material excitation. In recent years, this paradigm has evolved from a classical description of radiation…

光学 · 物理学 2026-02-20 Fatemeh Chahshouri , Sven Ebel , Mitja Funk , Nahid Talebi

Controlling free-electron momentum states is of high interest in electron microscopy to achieve momentum and energy resolved probing and manipulation of physical systems. Free-electron and light interactions have emerged as a powerful…

量子物理 · 物理学 2024-04-08 Sven Ebel , Nahid Talebi

We exploit free-space interactions between electron beams and tailored light fields to imprint on-demand phase profiles on the electron wave functions. Through rigorous semiclassical theory involving a quantum description of the electrons,…

量子物理 · 物理学 2021-03-31 F. Javier García de Abajo , Andrea Konečná

The coherent interaction between free electrons and optical fields can produce free-electron compression and push the temporal resolution of ultrafast electron microscopy to the attosecond regime. However, a large electron-light interaction…

量子物理 · 物理学 2025-03-27 Cruz I. Velasco , F. Javier García de Abajo

In display technologies or data processing, planar and subwavelength free-space components suited for flat photonic devices are needed. Metasurfaces, which shape the optical wavefront within hundreds of nanometers, can provide a solution…

The transmission electron microscope (TEM) has become an essential tool for innovation in nanoscience, material science, and biology. Despite these instruments being widely used across both industry and academia, academics may hesitate to…

仪器与探测器 · 物理学 2022-12-07 Patrick McBean , Zachary Milne , Arjun Kanthawar , Cameron O'Byrne , Khalid Hattar , Lewys Jones

We present a novel method that combines spin resonance spectroscopy with transmission electron microscopy (TEM), enabling localized in-situ detection of microwave (MW)-driven spin excitations. Our approach utilizes continuous wave MW…

We use time-resolved momentum microscopy at a free-electron laser (FEL) and extend orbital tomography into the time domain to image the electronic wave functions of excited molecular orbitals. This technique provides unprecedented insight…

Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…

光学 · 物理学 2026-02-05 Nelin Laštovičková Streshkova , Martin Kozák

In this paper we explore the desirability of a transmission electron microscope in which the phase of the electron wave can be freely controlled. We discuss different existing methods to manipulate the phase of the electron wave and their…

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