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We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal…

量子物理 · 物理学 2021-06-23 Zhedong Zhang , Tao Peng , Xiaoyu Nie , Girish S. Agarwal , Marlan O. Scully

THz quantum cascade lasers based on a novel buried cavity geometry are demonstrated by combining double-metal waveguides with proton implantation. Devices are realised with emission at 2.8 THz, displaying ultra low threshold currents of 19…

材料科学 · 物理学 2009-11-11 S. Dhillon , J. Alton , S. Barbieri , C. Sirtori , A. de Rossi , M. Calligaro , H. E. Beere , D. Ritchie

In this article we propose a system capable of THz radiation with quantum yield above unity. The system consists of nanoparticles where the material composition varies along the radial direction of each nanoparticle in such a way that a…

介观与纳米尺度物理 · 物理学 2018-06-06 K. B. Arnardottir , T. C. H. Liew

Contribution of plasma oscillation to the broadband terahertz emission is revealed by interacting two-color laser pulses with a supersonic jet of nitrogen molecules. Temporal and spectral shifts of THz waves are observed as the plasma…

光学 · 物理学 2016-11-03 Na Li , Ya Bai , Tianshi Miao , Peng Liu , Ruxin Li , Zhizhan Xu

Simultaneous measurements of THz wave and hard X-ray emission from thin and flat water flow when irradiated by double femtosecond laser pulses (800 nm, 35 fs, transform-limited, 0.5 kHz, delay times up to 15 ns) were carried out at the…

Ultrafast spectroscopy paved the way for probing transient states of matter produced through photoexcitation. Despite significant advances, the microscopic processes governing the formation of these states remain largely unknown. This study…

材料科学 · 物理学 2024-08-23 Francesco Libbi , Anders Johansson , Boris Kozinsky , Lorenzo Monacelli

We report the observation of a clear single-mode instability threshold in continuous-wave Fabry-Perot quantum cascade lasers (QCLs). The instability is characterized by the appearance of sidebands separated by tens of free spectral ranges…

Due to their conceptual appeal and computational convenience, two-level systems (TLS) and their generalisations are often used to investigate nonlinear behavior in quantum optics, and to assess the applicability of theoretical methods. Here…

量子物理 · 物理学 2023-12-22 Megha Gopalakrishna , Yaroslav Pavlyukh , Claudio Verdozzi

We show theoretically and experimentally that a quantum cascade laser (QCL) in an external Fabry-Perot cavity (EC) can produce regular self-pulsations (SP) of the output intensity at frequencies ~75 GHz. We recognize that the propagation…

Terahertz (THz) generation by optical rectification (OR) using tilted-pulse-fronts is studied. One-dimensional (1-D) and 2-D spatial models, which simultaneously account for (i) the nonlinear coupled interaction of the THz and optical…

We review our recent work leading to steady-state solutions of the semiclassical (Maxwell-Bloch) equations of a laser. These are coupled non-linear partial differential equations in space and time which have previously been solved either by…

光学 · 物理学 2009-01-08 Hakan E. Türeci , A. Douglas Stone , Li Ge , Stefan Rotter , Robert J. Tandy

We report a two-photon interference effect, in which the entangled photon pairs are generated from two laser pulses well-separated in time. In a single pump pulse case, interference effects did not occur in our experimental scheme. However,…

Mollow physics in the two-photon regime shows interesting features such as path-controlled time-reordering of photon pairs without the need to delay them. Here, we calculate analytically the two-photon correlations $ g^{(2)}(\tau)$,…

量子物理 · 物理学 2019-02-13 Alexander Carmele , Samir Bounouar , Max Strauß , Stephan Reitzenstein , Andreas Knorr

Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…

光学 · 物理学 2021-07-07 Szilard Szoke , Manni He , Bryce P. Hickam , Scott K. Cushing

We demonstrate that by coherent driving two uncoupled rings in same direction, the effective photon circulating time in the dual ring modulator is reduced, with increased modulation quality. The inter-ring detuning dependent photon…

光学 · 物理学 2015-06-22 Tingyi Gu , Young-kai Chen , Chee Wei Wong , Po Dong

The feasibility to generate correlated photon pairs at variable frequencies is investigated. For this purpose, we consider the interaction of an off-resonant laser field with a two-level system possessing broken inversion symmetry. We show…

量子物理 · 物理学 2015-06-05 Fernando Oster , Christoph H Keitel , Mihai Macovei

Photonic molecules - particular systems composed of coupled optical resonators - emulate the behavior of complex physical systems exhibiting discrete energy levels. In this work, we present a novel photonic molecule composed of two strongly…

光学 · 物理学 2023-12-06 Sara Kacmoli , Deborah L. Sivco , Claire F. Gmachl

We study the real-time nonequilibrium dynamics in hot QED plasmas implementing a dynamical renormalization group and using the hard thermal loop (HTL) approximation. The focus is on the study of the relaxation of gauge and fermionic mean…

高能物理 - 唯象学 · 物理学 2007-05-23 S. -Y. Wang , D. Boyanovsky , H. J. de Vega , D. -S. Lee

Energy level statistics of a bounded quantum system, whose classical dynamical system exhibits bifurcations, is investigated using the two-point correlation function (TPCL), which at the bifurcation points exhibits periodic spike…

混沌动力学 · 物理学 2022-08-30 Hironori Makino

The amplified spontaneous emission from a superluminescent diode was frequency doubled in a periodically poled lithium niobate waveguide crystal. The temporally incoherent radiation of such a superluminescent diode is characterized by a…

光学 · 物理学 2017-04-05 Henning Kurzke , Jan Kiethe , Axel Heuer , Andreas Jechow