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相关论文: Magnetic and crystal electric field studies of two…

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We report a comprehensive experimental investigation of the structural, thermodynamic, static, and dynamic properties of a triangular lattice antiferromagnet Rb$_3$Yb(VO$_4$)$_2$. Through the analysis of magnetic susceptibility,…

材料科学 · 物理学 2025-06-10 Sebin J. Sebastian , R. Kolay , Abhidev. B , Q. -P. Ding , Y. Furukawa , R. Nath

Frustration, spin correlations and interplay between competing degrees of freedom are some of the key ingredients that underlie exotic states with fractional excitations in quantum materials. Rare-earth based two dimensional magnetic…

强关联电子 · 物理学 2022-09-13 J. Khatua , M. Pregelj , A. Elghandour , Z. Jaglicic , R. Klingeler , A. Zorko , P. Khuntia

The interplay of magnetic correlations, crystal electric field interactions, and spin-orbit coupling in low-dimensional frustrated magnets fosters novel ground states with unusual excitations. Here, we report the magnetic properties and…

材料科学 · 物理学 2024-09-02 S. Guchhait , A. Painganoor , S. S. Islam , J. Sichelschmidt , M. D. Le , N. B. Christensen , R. Nath

The subtle interplay between competing degrees of freedom, crystal electric fields, and spin correlations can lead to exotic quantum states in 4f ion-based frustrated triangular lattice antiferromagnets. We present the crystal structure,…

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$\frac{1}{2}$ state due to the combined effect of crystal electric field and spin…

强关联电子 · 物理学 2020-04-22 K. M. Ranjith , Ph. Schlender , Th. Doert , M. Baenitz

Frustration-induced strong quantum fluctuations accompanied by spin-orbit coupling and crystal electric field can give rise to rich and diverse magnetic phenomena associated with unconventional low-energy excitations in rare-earth based…

强关联电子 · 物理学 2024-02-13 J. Khatua , S. Bhattacharya , A. M. Strydom , A. Zorko , J. S. Lord , A. Ozarowski , E. Kermarrec , P. Khuntia

The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for the realization of a quantum spin liquid ground state -- an exotic, quantum-disordered magnetic phase featuring…

We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state…

We calculate the crystal-field splitting, ground-state Kramers doublet and intersite exchange interactions within the ground-state doublet manifold using an ab initio Hubbard-I based approach for a representative set of Ce and Yb…

强关联电子 · 物理学 2026-02-06 Leonid V. Pourovskii , Rafael D. Soares , Alexander Wietek

We investigated the spin dynamics by electron spin resonance (ESR) of the Yb-based, effective spin-1/2 delafossites NaYbO$_{2}$, AgYbO$_{2}$, LiYbS$_{2}$, NaYbS$_{2}$, and NaYbSe$_{2}$ which all show an absence of magnetic order down to…

Antiferromagnetically coupled S=1/2 spins on an isotropic triangular lattice is the paradigm of frustrated quantum magnetism, but structurally ideal realizations are rare. Here we investigate NaYbO$_2$, which hosts an ideal triangular…

We investigate the magnetic interactions in triangular rare-earth delafossites materials NaYbO$_2$ and NaYbS$_2$ via first-principles calculations. The calculated Curie-Weiss temperatures are in good agreement with experiments. We perform…

材料科学 · 物理学 2021-04-21 Da-Ye Zheng , Zhen-Xiong Shen , Meng Zhang , Lixin He

Rare-earth chalcogenide compounds $\mathrm{ARECh_2}$ (A = alkali or monovalent metal, RE = rare earth, Ch = O, S, Se, Te) are a large family of quantum spin liquid (QSL) candidate materials. $\mathrm{NaYbS_2}$ is a representative member of…

强关联电子 · 物理学 2024-09-25 Weizhen Zhuo , Zheng Zhang , Mingtai Xie , Anmin Zhang , Jianting Ji , Feng Jin , Qingming Zhang

The interplay between competing degrees of freedom can stabilize non-trivial magnetic states in correlated electron materials. Frustration-induced strong quantum fluctuations can evade long-range magnetic ordering leading to exotic quantum…

强关联电子 · 物理学 2023-10-12 B. Sana , M. Barik , M. Pregelj , U. Jena , M. Baenitz , J. Sichelschmidt , K. Sethupathi , P. Khuntia

We report extensive measurements on a new compound (Yb0.24Sn0.76)Ru that crystallizes in the cubic CsCl structure. Valence band photoemission and L3 x-ray absorption show no divalent component in the 4f configuration of Yb. Inelastic…

Here we present a neutron scattering-based study of magnetic excitations and magnetic order in NaYbO$_2$ under the application of an external magnetic field. The crystal electric field-split $J = 7/2$ multiplet structure is determined,…

$\tilde{S}\!=\!1/2$ triangular-lattice $f$-electron materials define a dynamic research area in condensed matter magnetism. In various Yb 4$f^{13}$ triangular-lattice compounds, for example, spin-liquid ground states seem to be realized.…

强关联电子 · 物理学 2022-06-22 Pritam Bhattacharyya , Liviu Hozoi

We report a comprehensive investigation of the structural and magnetic properties of Na$_5$Yb(MoO$_4$)$_4$, a member of the stretched diamond magnetic lattice family. Neutron powder diffraction at 3.3~K confirms that the compound…

The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect…

强关联电子 · 物理学 2025-09-23 Barkha Khattar , Anzar Ali , Masahiko Isobe , Yogesh Singh

The interplay between spin-orbit coupling, anisotropic magnetic interaction, frustration-induced quantum fluctuations and spin correlations can lead to novel quantum states with exotic excitations in rare-earth-based quantum magnets.…

强关联电子 · 物理学 2023-08-31 J. Khatua , Q. P. Ding , M. S. Ramachandra Rao , K. Y. Choi , A. Zorko , Y. Furukawa , P. Khuntia
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