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Thermodynamic properties of fluids confined in nanopores differ from those observed in the bulk. To investigate the effect of nanoconfinement on water compressibility, we performed water sorption experiments on two nanoporous glass samples…

Nanoporous materials provide high surface area per unit mass and are capable of fluids adsorption. While the measurements of overall amount of fluid adsorbed by a nanopororus sample are straightforward, probing the fluid spacial…

地球物理 · 物理学 2018-02-20 Boris Gurevich , Michel M. Nzikou , Gennady Y. Gor

Fluids confined in nanopores are ubiquitous in nature and technology. In recent years, the interest in confined fluids has grown, driven by research on unconventional hydrocarbon resources -- shale gas and shale oil, much of which are…

软凝聚态物质 · 物理学 2021-11-16 C. D. Dobrzanski , B. Gurevich , G. Y. Gor

Liquids under confinement differ in behavior from their bulk counterparts and can acquire properties that are specific to the confined phase and linked to the nature and structure of the host matrix. While confined liquid water is not a new…

材料科学 · 物理学 2020-07-22 François-Xavier Coudert

Water plays a key role in biological membrane transport. In ion channels and water-conducting pores (aquaporins), one dimensional confinement in conjunction with strong surface effects changes the physical behavior of water. In molecular…

生物物理 · 物理学 2019-07-02 Oliver Beckstein , Mark S. P. Sansom

Moisture-capturing hydrogels have emerged as attractive sorbent materials capable of converting ambient humidity into liquid water. Recent works have demonstrated exceptional water capture capabilities of hydrogels, while simultaneously,…

软凝聚态物质 · 物理学 2023-11-03 Gustav Graeber , Carlos D. Díaz-Marín , Leon C. Gaugler

The diffusion of water molecules through mesoporous dust of amorphous carbon (a-C) is a key process in the evolution of prestellar, protostellar, and protoplanetary dust, as well as in that of comets. It also plays a role in the formation…

天体物理仪器与方法 · 物理学 2024-03-05 Romain Basalgète , Gaël Rouillé , Cornelia Jäger

Recent progress in extraction of unconventional hydrocarbon resources has ignited the interest in the studies of nanoporous media. Since many thermodynamic and mechanical properties of nanoscale solids and fluids differ from the analogous…

地球物理 · 物理学 2018-01-08 Gennady Y. Gor , Boris Gurevich

Porous carbonaceous materials have many important industrial applications including energy storage, water purification, and adsorption of volatile organic compounds. Most of their applications rely upon the adsorption of molecules or ions…

材料科学 · 物理学 2020-12-15 Alexander C. Forse , Céline Merlet , Clare P. Grey , John M. Griffin

Fluids confined in nanopores exhibit properties different from the properties of the same fluids in bulk, among these properties are the isothermal compressibility or elastic modulus. The modulus of a fluid in nanopores can be extracted…

化学物理 · 物理学 2018-03-14 Christopher D. Dobrzanski , Max A. Maximov , Gennady Y. Gor

We use molecular simulations of an ionic liquid in contact with a range of nanoporous carbons to investigate correlations between ion size, pore size, pore topology and properties of the adsorbed ions. We show that diffusion coefficients…

材料科学 · 物理学 2020-02-21 El Hassane Lahrar , Anouar Belhboub , Patrice Simon , Céline Merlet

In this paper, we introduce a novel, adapted approach for computing gas adsorption properties in porous materials. We analyze the Dubinin-Polanyi's adsorption model and investigate various frameworks to estimate its required essential…

材料科学 · 物理学 2023-10-25 F. Stavarache , A. Luna-Triguero , S. Calero , J. M. Vicent-Luna

When water molecules are confined to nanoscale spacings, such as in the nanometer size pores of activated carbon fiber (ACF), their freezing point gets suppressed down to very low temperatures ($\sim$ 150 K), leading to a metastable liquid…

软凝聚态物质 · 物理学 2015-06-23 S. O. Diallo , L. Vlcek , E. Mamontov , J. K. Keum , Jihua Chen , J. S. Hayes , A. A. Chialvo

When a fluid is confined to a nanopore, its thermodynamic properties differ from the properties of a bulk fluid, so measuring such properties of the confined fluid can provide information about the pore sizes. Here we report a simple…

The energy absorption on nanometer scale is vital for many bio and chemical systems. We report here that a two times amplification in absorption efficiency can be achieved by water molecules confined in carbon nanotubes with small radius,…

介观与纳米尺度物理 · 物理学 2022-07-19 Rong-Yao Yang , Wei-Zhou Jiang , Pei-Ying Huo , Qi-Lin Zhang

Liquid adsorption in nanoporous materials induces their deformation due to strong capillary forces. The linear relationship between the liquid pressure and the solid strain (pore-load modulus) provides an experimental technique to determine…

软凝聚态物质 · 物理学 2017-10-31 J. Puibasset

Adsorption in nanoporous materials is one strategy that can be used to store hydrogen at conditions of temperature and pressure that are economically viable. Adsorption capacity of nanoporous materials depends on surface area which can be…

材料科学 · 物理学 2024-05-28 Siddharth Gautam , David R. Cole , Zoltán Imre Dudás , Indu Dhiman

Understanding the adsorption of water and characterizing the water film formed within nanostructures are essential for advancements in fields such as nanofluidics, water purification, and biosensing devices. In our research, we focus on…

We use molecular dynamics simulations to study the diffusion of water inside deformed carbon nanotubes with different degrees of deformation at 300 K. We found that the number of hydrogen bonds that water forms depends on nanotube topology,…

软凝聚态物质 · 物理学 2020-01-16 Bruno H. S. Mendonça , Patricia Ternes , Evy Salcedo , Alan B. de Oliveira , Marcia C. Barbosa

We consider the theoretical description of a fluid adsorbed in a nanopore. Hysteresis and discontinuities in the isotherms in general hampers the determination of equilibrium thermodynamic properties, even in computer simulations. A…

软凝聚态物质 · 物理学 2015-06-18 Joël Puibasset , Edouard Kierlik , Gilles Tarjus
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