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In a circuit quantum eletrodynamic system, a chain of N qubits inhomogeneously coupled to a cavity field forms a mesoscopic quasi-lattice, which is characterized by its degree of deformation from a normal lattice. This deformation is a…

量子物理 · 物理学 2014-04-23 Hou Ian , Yu-xi Liu

We analytically tackle opto-vibronic interactions in molecular systems driven by either classical or quantum light fields. In particular, we examine a simple model of molecules with two relevant electronic levels, characterized by potential…

量子物理 · 物理学 2024-02-28 Q. Zhang , M. Asjad , M. Reitz , C. Sommer , B. Gurlek , C. Genes

The paradigm of $N$ quantum emitters coupled to a single cavity mode appears in many situations ranging from quantum technologies to polaritonic chemistry. The ideal case of identical emitters is elegantly modeled in terms of symmetric…

Over the past decade, exciton-polaritons in semiconductor microcavities have attracted a great deal of interest as a driven-dissipative quantum fluid. These systems offer themselves as a versatile platform for performing Hamiltonian…

Using microscopic models in which both photons and excitons are treated as microscopic degrees of freedom, we discuss polaritons of two cases: One is the case when excitonic parameters are time dependent. The time dependence causes creation…

量子物理 · 物理学 2011-04-15 Akira Shimizu , Teruaki Okushima , Kazuki Koshino

We study a system of interacting matter quasiparticles strongly coupled to photons inside an optomechanical cavity. The resulting normal modes of the system are represented by hybrid polaritonic quasiparticles, which acquire effective…

量子气体 · 物理学 2017-02-27 N. Bobrovska , M. Matuszewski , T. C. H. Liew , O. Kyriienko

We develop a microscopic theory for the multimode polariton dispersion in materials coupled to cavity radiation modes. Starting from a microscopic light-matter Hamiltonian, we devise a general strategy for obtaining simple matrix models of…

材料科学 · 物理学 2023-05-09 Arkajit Mandal , Ding Xu , Ankit Mahajan , Joonho Lee , Milan E. Delor , David R. Reichman

We show that an ensemble of organic dye molecules with permanent electric dipole moments embedded in a microcavity can lead to strong optical nonlinearities at the single photon level. The strong long-range electrostatic interaction between…

Polaritonic chemistry offers the possibility of modifying molecular properties and even influencing chemical reactivity through strong coupling between vibrational transitions and confined light modes in optical cavities. Despite…

化学物理 · 物理学 2025-05-16 Thomas Schnappinger , Markus Kowalewski

In the last decade, much theoretical research has focused on studying the strong coupling between organic molecules (or quantum emitters, in general) and light modes. The description and prediction of polaritonic phenomena emerging in this…

Nonlinear optics underpins quantum photonics by enabling the generation and control of quantum states of light. We present new applications of optical resonators as mode selectors in nonlinear processes. First, we show that cavity-enhanced…

量子物理 · 物理学 2025-10-02 Xin Chen

We show that a nonlinear optical response associated with a resonant, atomically thin material can be dramatically enhanced by placing it in front of a partially reflecting mirror, rendering otherwise weakly nonlinear systems suitable for…

介观与纳米尺度物理 · 物理学 2018-09-25 Dominik S. Wild , Ephraim Shahmoon , Susanne F. Yelin , Mikhail D. Lukin

We investigate the impact of the quantized mechanical motion of optically trapped atoms, arranged in proximity to a one-dimensional waveguide, on the propagation of polariton modes. Our study identifies a regime of resonant phonon-assisted…

量子气体 · 物理学 2024-11-28 Denis Ilin , Alexander S. Solntsev , Ivan Iorsh

In a recent preprint (arXiv:1401.1128v1) Cilibrizzi and co-workers report experiments and simulations showing the scattering of polaritons against a localised obstacle in a semiconductor microcavity. The authors observe in the linear…

Systems of coupled cavity modes have the potential to provide bright quantum optical states of light in a highly versatile manner. Microring resonators for instance are highly scalable candidates for photon sources thanks to CMOS…

量子物理 · 物理学 2021-06-04 Will McCutcheon

Driven optical cavities containing a nonlinear medium support stable dissipative solitons, cavity solitons, in the form of bright or dark spots of light on a uniformly-lit background. Broadening effects due to diffraction or group velocity…

光学 · 物理学 2025-09-09 Gian-Luca Oppo , William J. Firth

Newly observed enhanced linear optical features of fullerene solutions (Raman scattering and one-photon luminescence) are due to clusterization of fullerene molecules themselves as well as their composites with solvent molecules. A direct…

Molecular polaritons are the optical excitations which emerge when molecular transitions interact strongly with confined electromagnetic fields. Increasing interest in the hybrid molecular-photonic materials that host these excitations…

介观与纳米尺度物理 · 物理学 2018-02-26 Raphael F. Ribeiro , Luis A. Martínez-Martínez , Matthew Du , Jorge Campos-Gonzalez-Angulo , Joel Yuen-Zhou

Optomechanical systems provide a unique platform for observing quantum behavior of macroscopic objects. However, efforts towards realizing nonlinear behavior at the single photon level have been inhibited by the small size of the radiation…

量子物理 · 物理学 2015-01-14 Xunnong Xu , Michael Gullans , Jacob M. Taylor

The ultrafast non-radiative relaxation of a molecular ensemble coupled to a cavity mode is considered theoretically and by real-time quantum dynamics. For equal coupling strength of single molecules to the cavity mode, the non-radiative…

化学物理 · 物理学 2018-12-26 Oriol Vendrell