相关论文: Electron vortex beams for chirality probing at the…
Optimally-chiral electromagnetic fields with maximized helicity density, recently introduced in [1], enable chirality characterization of optically small nanoparticles. Here, we demonstrate a technique to obtain optimally-chiral nearfields…
Plasmonics, the science and technology of the interaction of light with metallic objects, is fundamentally changing the way we can detect, generate and manipulate light. Although the field is progressing swiftly, thanks to the availability…
Circular dichroism (CD) caused by the response of a chiral object to circularly polarized light has been well established, and the strong CD of plasmonic meta-molecules has also become of interest in recent years; however, their response if…
We present a combined classical and quantum electrodynamics description of the coupling between two circularly-polarized quantum emitters held above a metal surface supporting surface plasmons. Depending on their position and their natural…
The propagation of electron beams carrying angular momentum in crystals is studied using a multislice approach for the model system Fe. It is found that the vortex beam is distorted strongly due to elastic scattering. Consequently, the…
Artificial nanostructures enable fine control of electromagnetic fields at the nanoscale, a possibility that has recently been extended to the interaction between polarised light and chiral matter. The theoretical description of such…
The ability to create surface structures with precisely controlled chirality remains a major challenge in laser-matter interaction experiments. In this work, we theoretically study the interaction of vortex laser beams, characterized by…
We investigate the plasmonic nanohelix as an individual subwavelength element for locally probing light chirality. We show that an hybrid nanoantenna combining a carbon-gold core-shell helix and a plasmonic nanoaperture transmits circularly…
Collective optical excitations, such as localized surface plasmons in metallic nanoparticles and Mie resonances in high-index dielectrics, play a central role in nanoscale light--matter interactions. When such optical modes interact with…
Ultrafast imaging of molecular chirality is a key step towards the dream of imaging and interpreting electronic dynamics in complex and biologically relevant molecules. Here, we propose a new ultrafast chiral phenomenon exploiting recent…
Plasmonic chirality exhibits great potential for novel nanooptical devices due to the generation of a strong chiroptical response. Previous reports on plasmonic chirality explanations are mainly based on phase retardation and coupling. We…
When circularly polarized light interacts with a nanostructure, the optical response depends on the geometry of the structure. If the nanostructure is chiral (i.e., it cannot be superimposed on its mirror image), then its optical response,…
Light is one of the most powerful and precise tools allowing us to control, shape and create new phases of matter. In this task, the magnetic component of a light wave has so far played a unique role in defining the wave's helicity, but its…
Prospects of using metal hole arrays for the enhanced optical detection of molecular chirality in nanosize volumes are investigated. Light transmission through the holes filled with an optically active material is modeled and the activity…
Chirality is a fundamental asymmetry phenomenon, with chiral optical elements exhibiting asymmetric response in reflection or absorption of circularly polarized light. Recent realizations of such elements include nanoplasmonic systems with…
Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…
Single fluorescent molecules, behaving as ideal electric dipole emitters, are powerful nanoscopic probes of complex optical fields. Here, this property is exploited to precisely map the polarization and vectorial structure of tightly…
In light optics, beams with orbital angular momentum (OAM) can be produced by employing a properly-tuned two-cylinder-lens arrangement, also called $\pi$/2 mode converter. It is not possible to convey this concept directly to the beam in an…
The optical Faraday effect describes the rotation of linear polarization upon propagation through a medium in the presence of a longitudinal magnetic field. The effect arises from a different phase delay between the right and left handed…
We demonstrate that nanostructures carefully designed on both sides of a thin suspended metallic membrane couple light into a chiral near field and transmit vortex beams through a central aperture that connects the two sides of the…