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This letter addresses basic questions concerning ferroelectric order in positionally disordered dipolar materials. Three models distinguished by dipole vectors which have one, two or three components are studied by computer simulation.…

凝聚态物理 · 物理学 2009-10-28 G. Ayton , M. J. P. Gingras , G. N. Patey

In a recent letter [Phys. Rev. Lett. {\bf 75}, 2360 (1996)] we briefly discussed the existence and nature of ferroelectric order in positionally disordered dipolar materials. Here we report further results and give a complete description of…

无序系统与神经网络 · 物理学 2009-10-30 G. Ayton , M. J. P. Gingras , G. N. Patey

We investigate the effect of polar Sr-O vacancy pairs on the electric polarization of SrMnO$_3$ (SMO) thin films using density functional theory (DFT) calculations. This is motivated by indications that ferroelectricity in complex oxides…

材料科学 · 物理学 2021-05-21 Chiara Ricca , Danielle Berkowitz , Ulrich Aschauer

Electric polarization in conventional ferroelectric oxides usually involves nonmagnetic transition-metal ions with an empty d shell (the d$^0$ rule). Here we unravel a new mechanism for local electric dipoles based on magnetic Fe$^{3+}$…

强关联电子 · 物理学 2015-07-07 Shi-Peng Shen , Yi-Sheng Chai , Jun-Zhuang Cong , Pei-Jie Sun , Jun Lu , Li-Qin Yan , Shou-Guo Wang , Young Sun

We report the experimental determination of the structure and response to applied electric field of the lower-temperature nematic phase of the previously reported calamitic compound 4-[(4-nitrophenoxy)carbonyl]phenyl2,4-dimethoxybenzoate…

By means of first-principles simulations, we unambiguously show that improper ferroelectricity in magnetite in the low-temperature insulating phase is driven by charge-ordering. An accurate comparison between monoclinic ferroelectric Cc and…

材料科学 · 物理学 2015-05-13 Kunihiko Yamauchi , Tetsuya Fukushima , Silvia Picozzi

We show that surface interactions can vectorially structure the three-dimensional polariza-tion field of a ferroelectric fluid. The contact between a ferroelectric nematic liquid crystal and a surface with in-plane polarity generates a…

软凝聚态物质 · 物理学 2024-01-19 Xi Chen , Eva Korblova , Matthew A. Glaser , Joseph E. Maclennan , David M. Walba , Noel A. Clark

Ferroelectricity has been found to occur in several insulating systems, such as TbMnO$_3$ (TMO) and Ni$_3$V$_2$O$_8$ (NVO) which have more than one phase with incommensurately modulated long-range magnetic order. Here we give a…

材料科学 · 物理学 2009-11-11 A. Brooks Harris

Magnetoelectric coupling in the polycrystalline antiferromagnets CuFe0.95Rh0.05O2 and CuFeO2 has been investigated. For both samples, electric polarization was observed in the absence of an applied external magnetic field demonstrating that…

材料科学 · 物理学 2009-05-27 B. Kundys , A. Maignan , D. Pelloquin , Ch. Simon

Liquid crystal materials exhibiting up to three nematic phases are reported. Dielectric response measurements show that while the lower temperature nematic phase has ferroelectric order and the highest temperature nematic phase is apolar,…

软凝聚态物质 · 物理学 2021-09-07 S. Brown , E. Cruickshank , J. M. D. Storey , C. T. Imrie , D. Pociecha , M. Majewska , A. Makal , E. Gorecka

Magnetoelectric phenomena are intimately linked to relativistic effects and also require the material to break spatial inversion symmetry and time reversal invariance. Magnetoelectric coupling can substantially affect light-matter…

We have investigated the magnetic and dielectric properties of orthorhombic Eu$_{1-y}$Y$_y$MnO$_3$ ($0\leq y\leq 0.6$) single crystals without the presence of the 4$f$ magnetic moments of the rare-earth ions. In $y\geq 0.2$, the…

强关联电子 · 物理学 2015-05-28 Mitsuru Akaki , Masaaki Hitomi , Mizuaki Ehara , Daisuke Akahoshi , Hideki Kuwahara

Using molecular dynamics simulation, we study dipolar glass in crystals composed of slightly spheroidal, polar particles and spherical, apolar impurities between metal walls. We present physical pictures of ferroelectric glass, which have…

软凝聚态物质 · 物理学 2017-03-27 Kyohei Takae , Akira Onuki

Ferroelectric nematic liquid crystals are formed by achiral molecules with large dipole moments. Its three-dimensional orientational order is universally described as unidirectionally polar. We demonstrate that the ground state of…

软凝聚态物质 · 物理学 2024-04-01 Priyanka Kumari , Bijaya Basnet , Maxim O. Lavrentovich , Oleg D. Lavrentovich

AgNbO$_3$ is a lead-free perovskite with considerable potential for energy storage and optoelectronic applications, yet its low-temperature crystal structure has remained controversial. In this Letter, we revisit its low-energy structural…

材料科学 · 物理学 2026-02-24 Ying Song , Lingzhi Cao , Jinming Zhai , Zhilong Yang , Yali Yang , Laurent Bellaiche , Jiangang He

Based on Monte-Carlo simulations, the stable magnetization configurations of an antiferromagnet on a quasiperiodic tiling are derived theoretically. The exchange coupling is assumed to decrease exponentially with the distance between…

无序系统与神经网络 · 物理学 2007-05-23 E. Y. Vedmedenko , U. Grimm , R. Wiesendanger

We present a study based on several advanced First-Principles methods, of the recently synthesized PbNiO3 [J. Am. Chem. Soc 133, 16920 (2011)], a rhombohedral antiferromagnetic insulator which crystallizes in the highly distorted R3c…

强关联电子 · 物理学 2015-06-05 X. F. Hao , A. Stroppa , S. Picozzi , A. Filippetti , C. Franchini

We study the electrical behavior of multiferroic BiFeO$_3$ by means of first-principles calculations. We do so by constraining a specific component of the electric displacement field along a variety of structural paths, and by monitoring…

材料科学 · 物理学 2016-01-20 Massimiliano Stengel , Jorge Íñiguez

Electronic electro-optic (EEO) phase modulation is a key emerging technology for the chip-scale inter-conversion of signals between the electronic and photonic domains. The recent discovery of the ferroelectric nematic ($N_F$) liquid…

Recent interests towards novel functionalities arising at domain walls of ferroic materials naturally call for a microscopic understanding. To this end, first-principles calculations have been performed in order to provide solid evidence of…

材料科学 · 物理学 2014-04-09 Paolo Barone , Domenico Di Sante , Silvia Picozzi