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Point source atom interferometry (PSI) uses the velocity distribution in a cold atom cloud to simultaneously measure one axis of acceleration and two axes of rotation from the phase, orientation, and period of atomic interference fringe…

We demonstrate experimentally a scheme to measure small temporal delays, much smaller than the pulse width, between optical pulses. Specifically, we observe an interference effect, based on the concepts of quantum weak measurements and weak…

Here, we report on the nonlinear ionization of argon atoms in the short wavelength regime using ultraintense x rays from the European XFEL. After sequential multiphoton ionization, high charge states are obtained. For photon energies that…

Photoionization as a half-scattering process is not instantaneous. Usually, time delays in photoionization are of the order of few tens of attoseconds (1 as = 10$^{-18}$ s). While going from a single atom to a nano-object, one can expect…

Resonance-enhanced multiphoton ionization (REMPI) is a widely used technique for studying molecular photoionization and producing molecular cations for spectroscopy and dynamics studies. Here, we present a model for describing…

化学物理 · 物理学 2016-08-24 Matthias Germann , Stefan Willitsch

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

Ionization of atoms and molecules by absorption of a light pulse results in electron wavepackets carrying information on the atomic or molecular structure as well as on the dynamics of the ionization process. These wavepackets can be…

We report on the response of microchannel plates (MCPs) to single relativistic particles and to electromagnetic showers. Particle detection by means of secondary emission of electrons at the MCP surface has long been proposed and is used…

The R-Matrix incorporating Time (RMT) method is a new method for solving the time-dependent Schroedinger equation for multi-electron atomic systems exposed to intense short-pulse laser light. We have employed the RMT method to investigate…

原子物理 · 物理学 2012-04-27 L. R. Moore , M. A. Lysaght , J. S. Parker , H. W. van der Hart , K. T. Taylor

Photoelectrochemical impedance spectroscopy (PEIS) is a useful tool for the characterization of photoelectrodes for solar water splitting. However, the analysis of PEIS spectra often involves a priori assumptions that might bias the…

化学物理 · 物理学 2020-12-10 Dino Klotz , Daniel A. Grave , Hen Dotan , Avner Rothschild

We develop a formalism for photoionization (PI) and potential energy curves (PECs) of Rydberg atoms in ponderomotive optical lattices and apply it to examples covering several regimes of the optical-lattice depth. The effect of…

原子物理 · 物理学 2021-08-11 Ryan Cardman , Jamie MacLennan , Sarah E. Anderson , Yun-Jhih Chen , Georg Raithel

We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…

原子物理 · 物理学 2015-06-12 J. M. Dahlström , T. Carette , E. Lindroth

We show how two circular polarization components of a linearly polarized pulse, propagating through a coherently driven dilute atomic vapor, can be well resolved in time domain by weak measurement. Slower group velocity of one of the…

量子物理 · 物理学 2016-07-28 Pardeep Kumar , Shubhrangshu Dasgupta

We describe an ab initio and non-perturbative $R$-matrix with time-dependence theory for ultrafast atomic processes in light fields of arbitrary polarization. The theory is applicable to complex, multielectron atoms and atomic ions subject…

原子物理 · 物理学 2018-12-04 D. D. A. Clarke , G. S. J. Armstrong , A. C. Brown , H. W. van der Hart

Present photoionization experiments cannot measure molecular frame photoelectron angular distributions (MFPAD) from the outermost valence electrons of molecules. We show that details of the MFPAD can be retrieved with high-order harmonics…

原子物理 · 物理学 2009-05-24 Anh-Thu Le , R. R. Lucchese , M. T. Lee , C. D. Lin

Attosecond dynamics in strong-field tunnel ionization are encoded in intricate holographic patterns in the photoelectron momentum distributions (PMDs). These patterns show the interference between two or more superposed quantum electron…

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

We present a joint experimental and theoretical study of non-sequential double ionization (NSDI) in argon driven by a 3100-nm laser source. The correlated photoelectron momentum distribution (PMD) shows a strong dependence on the pulse…

Formation of electron vortices and momentum spirals in photodetachment of the H$^-$ anion driven by isolated ultrashort laser pulses of circular polarization or by pairs of such pulses (of either corotating or counterrotating polarizations)…

原子物理 · 物理学 2022-11-23 M. M. Majczak , F. Cajiao Vélez , J. Z. Kamiński , K. Krajewska

In this work, we present the implementation of all-optical method for directly measuring electron pulse duration in an ultrafast scanning electron microscope. Our approach is based on the interaction of electrons with the ponderomotive…