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The $6S_{1/2}-5D_{5/2}$ electric quadrupole transition is investigated in Cesium vapor at room temperature via nonlinear Doppler-free 6P-6S-5D three-level spectroscopy. Frequency-resolved studies of individual E2 hyperfine lines allow one…

Selective Reflection (SR) spectroscopy of the $6s$ $^2S_{1/2} \rightarrow$ $7p$ $^2P_{3/2}$ electric dipole transition of Cesium ($\lambda~=~456$ nm) is performed for the first time using a nanometric-thin cell ($L=50 - 1500$~nm). We…

原子物理 · 物理学 2025-01-22 Armen Sargsyan , Rodolphe Momier , David Sarkisyan

Selective reflection is a high-resolution spectroscopic method that allows the probing of atomic and molecular gases in the near field of dielectric cell windows. It is a sensitive technique for measuring interactions between excited atoms…

量子物理 · 物理学 2025-07-09 B. Dutta , C. Boldt , G. Garcia-Arellano , M. Ducloy , P. Pedri , S. Scheel , A. Laliotis

We report on the coupling of an electric quadrupole transition in atom with plasmonic excitation in a nanostructured metallic metamaterial. The quadrupole transition at 685 nm in the gas of Cesium atoms is optically pumped, while the…

A special vapour cell has been built, that allows the measurement of the atom-surface van der Waals interaction exerted by a CaF2 window at the interface with Cs vapour. Mechanical and thermal fragility of fluoride windows make common…

We report on the analysis of FM selective reflection experiments on the 6S1/2->8P3/2 transition of Cs at 388 nm, and on the measurement of the surface van der Waals interaction exerted by a sapphire interface on Cs(8P3/2). Various…

We demonstrate that a method using the derivative of the selective reflection signal from a nanocell is a convenient and robust tool for atomic laser spectroscopy, achieving a nearly Doppler-free spectral resolution. The recorded linewidth…

Doppler-free two-photon spectroscopy is a standard technique for precision measurement of transition frequencies of dipole-forbidden transitions. The accuracy of such measurements depends critically on fitting of the spectrum to an…

原子物理 · 物理学 2023-08-25 Bubai Rahaman , Sid C. Wright , Sourav Dutta

The features of Doppler-free resonances detected by probing the $^{133}$Cs atom $6S_{1/2}-7P_{3/2}$ transition at 456 nm in a nanometric-thick vapor layer are investigated. The matrix element of this transition is about 11 times smaller…

原子物理 · 物理学 2025-01-31 A. Sargsyan , E. Klinger , R. Boudot , D. Sarkisyan

We present the first evidence of excitation of the $5p_{3/2} \rightarrow 6p_{1/2}$ electric dipole-forbidden transition in atomic rubidium. The experiments were carried out in a rubidium vapor cell using Doppler-free optical-optical…

In this paper, we describe two complementary non-linear spectroscopy methods which both allow to achieve Doppler-free spectra of atomic gases. First, saturated absorption spectroscopy is used to investigate the structure of the $5{\rm…

物理教育 · 物理学 2015-05-13 V. Jacques , B. Hingant , A. Allafort , M. Pigeard , J. -F. Roch

Spectroscopy is a unique experimental tool for measuring the fundamental Casimir-Polder interaction between excited state atoms, or other polarizable quantum objects, and a macroscopic surface. Spectroscopic measurements probe atoms at…

We experimentally demonstrate the cesium electric quadrupole transition from the 6S1/2 ground state to the 7D3/2,5/2 excited state through a virtual level by using a single laser at 767 nm. The excited state energy level population is…

原子物理 · 物理学 2020-08-25 Sandan Wang , Jinpeng Yuan , Lirong Wang , Liantuan Xiao , Suotang Jia

We report the first observation of a non-dipole transition in an ultra-cold atomic vapor. We excite the 3P-4P electric quadrupole (E2) transition in $^{23}$Na confined in a Magneto-Optical Trap(MOT), and demonstrate its application to…

原子物理 · 物理学 2009-11-10 M. Bhattacharya , C. Haimberger , N. P. Bigelow

We present a comprehensive study of the electronic transitions in neutral cadmium (Cd I) with a focus on forbidden transitions, motivated by recent advances in laser technology and the growing relevance of cadmium in quantum gas research,…

原子物理 · 物理学 2025-10-07 P. J. Robert , S. Manzoor , M. Chiarotti , N. Poli

We investigate the temperature dependence of the Casimir-Polder interaction in the electrostatic limit. This unusual phenomenon relies on the coupling between a virtual atomic transition and a thermal excitation of surface polariton modes.…

We report the first experimental study of the influence of a dielectric surface on the transmission spectrum of cesium atoms for the $6S_{1/2} \rightarrow 7P_{3/2}$ ($D_2$) transition in vapor cells with thicknesses in the range…

原子物理 · 物理学 2026-01-09 Armen Sargsyan , Anahit Gogyan , David Sarkisyan

Direct evidence of excitation of the 5p3/2 -> 6p3/2 electric dipole forbidden transition in atomic rubidium is presented. The experiments were performed in a room temperature rubidium cell with continuous wave extended cavity diode lasers.…

Cooperative effects such as super- and subradiance can be observed in the fluorescence emitted by a system of N atoms in vacuum, after interaction with a laser beam. In the vicinity of a dielectric or metallic surface, Casimir-Polder…

We present an experimental scheme that produces Doppler-free spectra of the $5s \to 6p $ second resonance transition in atomic rubidium. The experiment uses the saturation of the cascade fluorescence that occurs when thermal rubidium atoms…

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