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Two-magnon modes are terahertz-frequency magnetic excitations in antiferromagnets, governed by exchange interactions, involving magnons from the entire Brillouin zone and dominated by zone-edge magnons. The ability to couple to light…

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

强关联电子 · 物理学 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

We present a theory for Raman scattering on 2D quantum antiferromagnets. The microscopic Fleury-Loudon Hamiltonian is expressed in terms of an effective $O(3)$ - model. Well within the N\'eel ordered phase, the Raman spectrum contains a…

强关联电子 · 物理学 2015-09-29 S. A. Weidinger , W. Zwerger

Raman selection rules for electronic and magnetic excitations in BaFe2As2 were theoretically investigated and applied them to the separate detection of the nodal and anti-nodal gap excitations at the spin density wave (SDW) transition and…

Resonance Raman scattering, which probes electrons, phonons and their interplay in crystals, is extensively used in two-dimensional materials. Here we investigate Raman modes in MoSe$_2$ at different laser excitation energies from 2.33 eV…

We investigate the experimental signatures of Raman spectroscopy of bi- and tri-magnon excitations in the distorted triangular lattice antiferromagnets alpha-LCr2O4 (L=Sr, Ca). We utilize spin wave theory to analyze the nearly 120 degree…

强关联电子 · 物理学 2023-05-23 Junli Li , Shangjian Jin , Trinanjan Datta , Dao-Xin Yao

The spectral distribution of parametrically excited dipole-exchange magnons in an in-plane magnetized epitaxial film of yttrium-iron garnet was studied by means of frequency- and wavevector-resolved Brillouin light scattering spectroscopy.…

介观与纳米尺度物理 · 物理学 2014-01-14 A. A. Serga , C. W. Sandweg , V. I. Vasyuchka , M. B. Jungfleisch , B. Hillebrands , A. Kreisel , P. Kopietz , M. P. Kostylev

Excitation of four coherent phonon modes of different symmetries has been realized in copper metaborate CuB$_2$O$_4$ via impulsive stimulated Raman scattering (ISRS). Phonons were detected by monitoring changes in the linear optical…

We present a unified theoretical framework for induced (stimulated) scattering-parametric instabilities of electromagnetic waves, including induced Compton, stimulated Brillouin, and stimulated Raman scattering (SRS) in strongly magnetized…

高能天体物理现象 · 物理学 2025-10-16 Rei Nishiura , Shoma F. Kamijima , Kunihito Ioka

We study the second-order Raman process of mono- and few-layer MoTe$_2$, by combining {\em ab initio} density functional perturbation calculations with experimental Raman spectroscopy using 532, 633 and 785 nm excitation lasers. The…

We calculate magnetic Raman spectra of Heisenberg antiferromagnets on the two-dimensional Penrose lattice. We follow the Shastry-Shraiman formulation of Raman scattering in a strongly correlated Hubbard system and obtain the second- and…

强关联电子 · 物理学 2024-08-05 Takashi Inoue , Shoji Yamamoto

Although the parent iron-based pnictides and chalcogenides are itinerant antiferromagnets, the use of local moment picture to understand their magnetic properties is still widespread. We study magnetic Raman scattering from a local moment…

强关联电子 · 物理学 2011-02-14 C. -C. Chen , C. J. Jia , A. F. Kemper , R. R. P. Singh , T. P. Devereaux

We present the results for a model calculation of resonant two-magnon Raman scattering in a spin density wave (SDW) antiferromagnet. The resonant enhancement of the two-magnon intensity is obtained from a microscopic analysis of the…

凝聚态物理 · 物理学 2009-10-28 Friedhelm Schoenfeld , Arno P. Kampf , Erwin Mueller-Hartmann

We utilize conventional wave-vector-resolved Brillouin light scattering technology to investigate the spin wave response in YIG thin films under high-power microwave excitation. By varying the microwave frequency, external bias magnetic…

介观与纳米尺度物理 · 物理学 2025-05-01 Guofu Xu , Kang An , Wenjun Ma , Xiling Li , C. K. Ong , Chi Zhang , Guozhi Chai

We have carried out Raman spectroscopy experiments to investigate two-magnon excitations in epitaxial thin films of the quasi-two-dimensional antiferromagnetic Mott insulator Sr$_2$IrO$_4$ under in-plane misfit strain. With in-plane biaxial…

We report direct spectroscopic evidence of antimagnons, i.e., negative-energy spin waves identified by their signature inverted dispersion with Brillouin light scattering (BLS) spectroscopy. We investigate an ultrathin BiYIG film with a…

Raman spectra obtained by the inelastic scattering of light by crystalline solids contain contributions from first-order vibrational processes (e.g. the emission or absorption of one phonon, a quantum of vibration) as well as higher-order…

材料科学 · 物理学 2017-08-22 Yannick Gillet , Stefan Kontur , Matteo Giantomassi , Claudia Draxl , Xavier Gonze

We study first-order (single-magnon) inelastic light scatterings in spin-$\frac{1}{2}$ two-dimensional quasiperiodic antiferromagnets in comparison with those emergent on periodic lattices. Unlike second-order (two-magnon) Raman scatterings…

强关联电子 · 物理学 2026-04-29 Takashi Inoue , Shoji Yamamoto

The linear spin-wave theory study of PbFeBO4 spin dynamics is presented. It is shown that the modes observed in Raman scattering experiments below Neel temperature are optical magnon and two-magnon excitations. Based on the magnon energy,…

材料科学 · 物理学 2021-04-07 M. A. Prosnikov

We experimentally demonstrate the generation of spin-wave frequency combs based on the nonlinear interaction of propagating spin waves in a microstructured waveguide. By means of time and space-resolved Brillouin light scattering…

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