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This work describes through semiclassical Boltzmann transport theory and simulation a novel nanostructured material design that can lead to unprecedentedly high thermoelectric power factors, with improvements of more than an order of…

Energy filtering has been suggested by many authors as a means to improve thermoelectric properties. The idea is to filter away low-energy charge carriers in order to increase Seebeck coefficient without compromising electronic…

The addition of porosity to thermoelectric materials can significantly increase the figure of merit, ZT, by reducing the thermal conductivity. Unfortunately, porosity is also detrimental to the thermoelectric power factor in the numerator…

介观与纳米尺度物理 · 物理学 2021-03-29 S. Aria Hosseini , Giuseppe Romano , P. Alex Greaney

Cross-plane superlattices composed of nanoscale layers of alternating potential wells and barriers have attracted great attention for their potential to provide thermoelectric power factor improvements and higher ZT figure of merit.…

材料科学 · 物理学 2015-12-16 Mischa Thesberg , Mahdi Pourfath , Hans Kosina , Neophytos Neophytou

Nano-structuring is an extremely promising path to high performance thermoelectrics. Favorable improvements in thermal conductivity are attainable in many material systems, and theoretical work points to large improvements in electronic…

Large efforts in improving thermoelectric energy conversion are devoted to energy filtering by nanometer size potential barriers. In this work we perform an analysis and optimization of such barriers for improved energy filtering. We merge…

材料科学 · 物理学 2013-08-01 Neophytos Neophytou , Hans Kosina

Nanocomposites are promising candidates for the next generation of thermoelectric materials since they exhibit extremely low thermal conductivities as a result of phonon scattering on the boundaries of the various material phases. The…

介观与纳米尺度物理 · 物理学 2017-12-06 Samuel Foster , Mischa Thesberg , Neophytos Neophytou

The thermoelectric power factor of hierarchically nanostructured materials is investigated using the nonequilibrium Greens function method for quantum transport, including interactions of electrons with acoustic and optical phonons. We…

介观与纳米尺度物理 · 物理学 2019-01-30 Vassilios Vargiamidis , Neophytos Neophytou

Some of the most promising candidates for next generation thermoelectrics are nanocomposites due to their low thermal conductivities that result from phonon scattering on the boundaries of the various material phases. However, in order to…

材料科学 · 物理学 2019-03-04 Samuel Foster , Mischa Thesberg , Neophytos Neophytou

The physics of energy filtering in electronic transport through nanoscale barriers is a fundamental aspect in the context of electronic engineering of nanostructured thermoelectrics. In the context of thermoelectric generators, it aims to…

介观与纳米尺度物理 · 物理学 2016-09-27 Aniket Singha , Bhaskaran Muralidharan

Nanostructured materials and nanocomposites have shown great promise for improving the efficiency of thermoelectric materials. Herein, Fe nanoparticles were imbedded into a CrN matrix by combining two physical vapor deposition approaches,…

Electron energy filtering has been suggested as a promising way to improve the power factor and enhance the ZT figure of merit of thermoelectric materials. In this work we explore the effect that reduced dimensionality has on the success of…

介观与纳米尺度物理 · 物理学 2017-01-11 Mischa Thesberg , Hans Kosina , Neophytos Neophytou

In this letter, we explore electron filtering as a technique to increase Seebeck coefficient and the thermoelectric power factor of heterostructured materials over that of the bulk. We present a theoretical model in which Seebeck…

材料科学 · 物理学 2007-05-23 J. M. O. Zide , D. Vashaee , G. Zeng , J. E. Bowers , A. Shakouri , A. C. Gossard

There is a growing momentum in recent thermoelectric materials research for flexible materials which enhance power output and efficiency at human wearable temperatures. In our previous work, we established the method to improve…

A numerical study of thermoelectric nanocomposites is presented. Thermoelectric properties as a function of average grain size or nanoparticle density are examined by simulating the measurements as they would be done experimentally. In…

材料科学 · 物理学 2020-01-08 Xufeng Wang , Mark Lundstrom

We investigate the electric and thermoelectric transport coefficients of nanocomposites using the Non-Equilibrium Greens Function (NEGF) method, which can accurately capture the details of geometry and disorder in these structures. We…

介观与纳米尺度物理 · 物理学 2018-10-17 Vassilios Vargiamidis , Samuel Foster , Neophytos Neophytou

The field of thermoelectric materials has undergone a revolutionary transformation over the last couple of decades as a result of the ability to nanostructure and synthesize myriads of materials and their alloys. The ZT figure of merit,…

Research on conjugated polymers for thermoelectric applications has made tremendous progress in recent years, which is accompanied by surging interest in molecular doping as a means to achieve the high electrical conductivities that are…

Monte Carlo statistical ray-tracing methods are commonly employed to simulate carrier transport in nanostructured materials. In the case of a large degree of nanostructuring and under linear response (small driving fields), these…

介观与纳米尺度物理 · 物理学 2023-02-09 Pankaj Priyadarshi , Neophytos Neophytou

Silicon carbide nanoparticles with diameters around 8 nm and with narrow size distribution have been finely mixed with doped silicon nanopowders and sintered into bulk samples to investigate the influence of nanoinclusions on electrical and…

材料科学 · 物理学 2021-10-27 S. Aria Hosseini , Devin Coleman , Sabah Bux , P. Alex Greaney , Lorenzo Mangolini
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