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Extracting single photoionization time delays associated with atomic (or molecular) species from attosecond time scale two-photon experiments usually relies on the theoretical description of continuum-continuum transitions. The available…

原子物理 · 物理学 2022-08-29 D. I. R. Boll , L. Martini , O. A. Fojón

Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…

We describe a numerical method that simulates the interaction of the helium atom with sequences of femtosecond and attosecond light pulses. The method, which is based on the close-coupling expansion of the electronic configuration space in…

原子物理 · 物理学 2021-05-25 Luca Argenti , Eva Lindroth

A fully analytical approximation for the observable characteristics of many-electron atoms is developed via a complete and orthonormal hydrogen-like basis with a single-effective charge parameter for all electrons of a given atom. The basis…

量子物理 · 物理学 2017-12-06 O. D. Skoromnik , I. D. Feranchuk , A. U. Leonau , C. H. Keitel

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

We consider the time evolution of the occupation probabilities for the 2s-2p transition in a hydrogen atom interacting with an external field, V(t). A two-state model and a dipole approximation are used. In the case of degenerate energy…

量子物理 · 物理学 2009-11-10 Kh. Kh. Shakov , J. H. McGuire

The self-consistent harmonic approximation is an effective harmonic theory to calculate the free energy of systems with strongly anharmonic atomic vibrations, and its stochastic implementation has proved to be an efficient method to study,…

材料科学 · 物理学 2017-07-26 Raffaello Bianco , Ion Errea , Lorenzo Paulatto , Matteo Calandra , Francesco Mauri

The new approach for calculation of transition form factors of hydrogenlike atoms is proposed. The explicit expressions for form factors of transitions from bound $nS$-states to continuum in terms of the classical polynomials are derived

高能物理 - 唯象学 · 物理学 2007-05-23 O. Voskresenskaya

We present an analytical model capable of describing two-photon ionization of atoms with attosecond pulses in the presence of intermediate and final isolated autoionizing states. The model is based on the finite-pulse formulation of…

原子物理 · 物理学 2016-03-02 Álvaro Jiménez Galán , Fernando Martín , Luca Argenti

In the present paper, we consider nonresonant corrections to $ 2s-ns/nd $ transition frequencies in hydrogen for the experiments based on two-photon spectroscopy. A detailed study of angular correlations of quantum interference effects…

原子物理 · 物理学 2021-03-03 A. Anikin , T. Zalialiutdinov , D. Solovyev

We consider the two-photon ionization of Hydrogen-like atoms. We find an approximate expression of the long-range phase based on an asymptotic expansion of the continuum eigenfunctions within the Wentzel-Kramers-Brillouin approximation.…

A simple procedure is presented to study the conservation of energy equation with dissipation in continuum mechanics in 1D. This procedure is used to transform this nonlinear evolution-diffusion equation into a hyperbolic PDE; specifically,…

经典物理 · 物理学 2020-08-13 Hamid A Said

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

In 2003 we have measured the absolute frequency of the $(1S, F=1, m_F=\pm 1) \leftrightarrow (2S, F'=1, m_F'=\pm 1)$ two-photon transition in atomic hydrogen. We observed a variation of $(-29\pm 57)$ Hz over a 44 months interval separating…

Attosecond transient-absorption spectroscopy (ATAS) is an established method for exploring electron dynamics on the subfemtosecond time-scale. ATAS spectra contain certain ubiquitous features, such as oscillating fringes, light-induced…

原子物理 · 物理学 2017-08-02 Jørgen Johansen Rørstad , Jens E. Bækhøj , Lars Bojer Madsen

We provide approximate analytic expressions for above-threshold ionization (ATI) transition probabilities and photoelectron angular distributions (PADs). These analytic expressions are more general than those existing in the literature and…

原子物理 · 物理学 2018-02-14 A. S. Maxwell , A. Al-Jawahiry , X. Y. Lai , C. Figueira de Morisson Faria

New method for ab initio calculations of the properties of large size system based on phase-amplitude functional is presented. It is shown that Schrodinger equation for many electrons complex system including large size molecules, or…

计算物理 · 物理学 2019-10-10 Pawel Strak , Konrad Sakowski , Pawel Kempisty , Stanislaw Krukowski

The femtosecond optical pump-probe technique was used to study dynamics of photoexcited electrons and coherent optical phonons in transition metals Zn and Cd as a function of temperature and excitation level. The optical response in time…

强关联电子 · 物理学 2009-11-11 Muneaki Hase , Kunie Ishioka , Jure Demsar , Kiminori Ushida , Masahiro Kitajima

We have used ab-initio density functional theory technique to understand the phase transitions and structural changes in various high temperature/pressure phases of LiAlO2. The electronic band structure as well as phonon spectra are…

材料科学 · 物理学 2018-06-05 Baltej Singh , M. K. Gupta , R. Mittal , S. L. Chaplot

We theoretically investigate a relation between the crystalline symmetry and the transient modulation of optical properties of crystalline dielectrics in pump-probe measurements using intense pump and attosecond probe fields. When the…

材料科学 · 物理学 2020-04-29 Shunsuke Yamada , Kazuhiro Yabana
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