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A quantum spin liquid (QSL) is an exotic state of matter in which electrons' spins are quantum entangled over long distances, but do not show symmetry-breaking magnetic order in the zero-temperature limit. The observation of QSL states is a…

强关联电子 · 物理学 2017-03-08 J. A. M. Paddison , M. Daum , Z. L. Dun , G. Ehlers , Y. Liu , M. B. Stone , H. D. Zhou , M. Mourigal

The delafossite-like compound NaYbO$_2$ hosts a triangular lattice of Yb$^{3+}$ moments and is a promising candidate for the realization of a quantum spin liquid ground state -- an exotic, quantum-disordered magnetic phase featuring…

High-quality single crystals of NaYbSe$_2$, which resembles a perfect triangular-lattice antiferromagnet without the intrinsic disorder, are investigated by magnetization and specific heat, as well as the local probe techniques nuclear…

The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…

强关联电子 · 物理学 2007-05-23 Yasuhiro Shimizu , Kazuya Miyagawa , Kazushi Kanoda , Maesato Mitsuhiko , Gunzi Saito

Here, we report the synthesis and magnetic properties of a Yb-based triangular-lattice compound LiYbS$_2$. At low temperatures, it features an effective spin-$\frac{1}{2}$ state due to the combined effect of crystal electric field and spin…

强关联电子 · 物理学 2020-04-22 K. M. Ranjith , Ph. Schlender , Th. Doert , M. Baenitz

Na$_4$Ir$_3$O$_8$ is a candidate material for a 3-dimensional quantum spin-liquid on the hyperkagome lattice. We present thermodynamic measurements of heat capacity $C$ and thermal conductivity $\kappa$ on high quality polycrystalline…

强关联电子 · 物理学 2015-06-18 Yogesh Singh , Y. Tokiwa , J. Dong , P. Gegenwart

$\tilde{S}\!=\!1/2$ triangular-lattice $f$-electron materials define a dynamic research area in condensed matter magnetism. In various Yb 4$f^{13}$ triangular-lattice compounds, for example, spin-liquid ground states seem to be realized.…

强关联电子 · 物理学 2022-06-22 Pritam Bhattacharyya , Liviu Hozoi

Conventional crystalline magnets are characterized by symmetry breaking and normal modes of excitation called magnons with quantized angular momentum $\hbar$. Neutron scattering correspondingly features extra magnetic Bragg diffraction at…

We introduce the rare-earth delafossite compound TlYbSe$_2$ -- extending the search for quantum spin liquids in frustrated triangular lattice magnets. While the DC magnetisation suggests magnetic exchange interactions in the order of…

强关联电子 · 物理学 2025-09-16 Bishnu P. Belbase , Arjun Unnikrishnan , Shi Feng , Eun Sang Choi , Johannes Knolle , Arnab Banerjee

The delafossite structure of NaYbS2 contains a planar spin-1/2 triangular lattice of Yb3+ ions and features a possible realisation of a quantum spin-liquid state. We investigated the Yb3+ spin dynamics by Electron Spin Resonance (ESR) in…

强关联电子 · 物理学 2019-03-11 Jörg Sichelschmidt , Philipp Schlender , Burkhard Schmidt , Michael Baenitz , Thomas Doert

Although magnetically ordered at low temperatures, the spin-1/2 triangular antiferromagnet Cs_2CuCl_4 exhibits remarkable spin dynamics that strongly suggest proximity to a spin liquid phase. Here we address the question of whether a…

强关联电子 · 物理学 2013-05-29 Jason Alicea , Matthew P. A. Fisher

We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…

强关联电子 · 物理学 2017-12-06 P. Khuntia , R. Kumar , A. V. Mahajan , M. Baenitz , Y. Furukawa

The search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature, is a main theme in current condensed matter physics. However, there is no smoking-gun evidence…

In this paper, we study the spin excitation properties of the frustrated triangular-lattice antiferromagnet Yb(BaBO$_3$)$_3$ with nuclear magnetic resonance. From the spectral analysis, neither magnetic ordering nor spin freezing is…

强关联电子 · 物理学 2020-08-03 K. Y. Zeng , Long Ma , Y. X. Gao , Z. M. Tian , L. S. Ling , Li Pi

We report a direct observation of the magnetic vortex lattice in the model high-temperature superconductor HgBa2CuO4+x. Using small-angle neutron scattering on high-quality crystals, we observe two equal domains of undistorted triangular…

超导电性 · 物理学 2015-05-20 Yuan Li , N. Egetenmeyer , J. L. Gavilano , N. Barisic , M. Greven

We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated…

Quantum spin liquid (QSL) state in rare-earth triangular lattice has attracted much attention recently due to its potential application in quantum computing and communication. Here we report the single-crystal growth synthesis, crystal…

强关联电子 · 物理学 2021-11-16 Jie Xing , Liurukara D. Sanjeewa , Andrew F. May , Athena S. Sefat

DC-magnetization data measured down to 40 mK speak against conventional freezing and reinstate YbMgGaO$_4$ as a triangular spin-liquid candidate. Magnetic susceptibility measured parallel and perpendicular to the $c$-axis reaches constant…

Spin fluctuations in the triangular-lattice Heisenberg antiferromagnet NaCrO$_2$ are investigated by means of quasi-elastic neutron scattering with high energy resolution and wide energy band. Two components with the following features are…

强关联电子 · 物理学 2022-08-17 K. Tomiyasu , Y. P. Mizuta , M. Matsuura , K. Aoyama , H. Kawamura

Quantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T = 0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin…

强关联电子 · 物理学 2020-11-20 C. Wessler , B. Roessli , K. W. Krämer , B. Delley , O. Waldmann , L. Keller , D. Cheptiakov , H. B. Braun , M. Kenzelmann