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Experimental observations of the ultrafast (less than 50 fs) demagnetization of Ni have so far defied theoretical explanations particularly since its spin-flipping time is much less than that resulting from spin-orbit and electron-lattice…

强关联电子 · 物理学 2020-07-08 Shree Ram Acharya , Volodymyr Turkowski , Guo-ping Zhang Talat S. Rahman

The ability to controllably manipulate the laser-induced ultrafast magnetic dynamics is a prerequisite for future high speed spintronic devices. The optimization of devices requires the controllability of the ultrafast demagnetization time,…

介观与纳米尺度物理 · 物理学 2018-02-14 Wei Zhang , Wei He , Xiang-Qun Zhang , Zhao-Hua Cheng , Jiao Teng , Manfred Fähnle

Following the demonstration of laser-induced ultrafast demagnetization in ferromagnetic nickel, several theoretical and phenomenological propositions have sought to uncover its underlying physics. In this work we revisit the three…

强关联电子 · 物理学 2023-03-29 Suchetana Mukhopadhyay , Sudip Majumder , Surya Narayan Panda , Anjan Barman

Interest in femtosecond demagnetization experiments was sparked by Bigot's discovery in 1995. These experiments unveil the elementary mechanisms coupling the electrons' temperature to their spin order. Even though first quantitative models…

In spintronics applications, ultrafast spin dynamics have to be controlled at femtosecond (fs) timescales via fs-laser radiation. At such ultrafast timescales, the effect of the Gilbert damping factor {\alpha} on ultrafast demagnetization…

材料科学 · 物理学 2019-10-02 Wei Zhang , Qian Liu , Zhe Yuan , Ke Xia , Wei He , Qing-feng Zhan , Xiang-qun Zhang , Zhao-hua Cheng

The demagnetizing factor N is of both conceptual interest and practical importance. Considering localized magnetic moments on a lattice, we show that for non-ellipsoidal samples, N depends on the spin dimensionality (Ising, XY, or…

We propose a semi-classical model for femtosecond-laser induced demagnetization due to spin-polarized excited electron diffusion in the super-diffusive regime. Our approach treats the finite elapsed time and transport in space between…

材料科学 · 物理学 2011-06-14 Marco Battiato , Karel Carva , Peter M. Oppeneer

Irradiating a ferromagnetic material with an ultrashort laser pulse leads to demagnetization on a femtosecond timescale. We implement Elliott-Yafet type spin-flip scattering, mediated by electron-electron and electron-phonon collisions,…

材料科学 · 物理学 2011-08-29 Benedikt Y. Mueller , T. Roth , M. Cinchetti , M. Aeschlimann , B. Rethfeld

Since the discovery of ultrafast demagnetization in Ni thin films in 1996, laser-induced ultrafast spin dynamics have become a prominent research topic in the field of magnetism and spintronics. This development offers new possibilities for…

Local material inhomogeneities can strongly influence magnetization dynamics and macroscopic magnetic properties, yet detecting such defects from magnetic imaging data remains challenging when thermal fluctuations and experimental noise…

Element specific ultrafast demagnetization was studied in Fe$_{1-x}$Ni$_{x}$ alloys, covering the concentration range between $0.1<x<0.9$. For all compositions, we observe a delay in the onset of Ni demagnetization relative to the Fe…

A hierarchical multiscale approach to model the magnetization dynamics of ferromagnetic ran- dom alloys is presented. First-principles calculations of the Heisenberg exchange integrals are linked to atomistic spin models based upon the…

材料科学 · 物理学 2015-09-02 D. Hinzke , U. Atxitia , K. Carva , P. Nieves , O. Chubykalo-Fesenko , P. M. Oppeneer , U. Nowak

We theoretically investigate laser-induced spin transport in metallic magnetic heterostructures using an effective spin transport description that treats itinerant electrons and thermal magnons on an equal footing. Electron-magnon…

介观与纳米尺度物理 · 物理学 2022-04-27 Maarten Beens , Rembert A. Duine , Bert Koopmans

The integration of machine learning and robotics into thin film deposition is transforming material discovery and optimization. However, challenges remain in achieving a fully autonomous cycle of deposition, characterization, and…

材料科学 · 物理学 2026-02-24 Yuanlong Zheng , Connor Blake , Layla Mravac , Fengxue Zhang , Yuxin Chen , Shuolong Yang

The magneto-optical response of Fe and Ni during ultrafast demagnetization is studied experimentally and theoretically. We have performed pump-probe experiments in the transverse magneto-optical Kerr effect (T-MOKE) geometry using photon…

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

材料科学 · 物理学 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

The Elliott-Yafet mechanism is arguably the most promising candidate to explain the ultrafast demagnetization dynamics in ferromagnetic transition metals on timescales on the order of 100 femtoseconds. So far, only electron-phonon…

By correlating time- and angle-resolved photoemission and time-resolved transverse- magneto- optical Kerr effect measurements, both at extreme ultraviolet wavelengths, we uncover the universal nature of the ultrafast photoinduced magnetic…

The phenomenology of magnetic damping is of critical importance for devices that seek to exploit the electronic spin degree of freedom since damping strongly affects the energy required and speed at which a device can operate. However,…

Engineering of magnetic materials for developing better spintronic applications relies on the control of two key parameters: the spin polarization and the Gilbert damping responsible for the spin angular momentum dissipation. Both of them…

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