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We report time-resolved photoelectron spectroscopy of the $3s3p$ doubly excited states of helium dressed by an intense near-infrared (NIR) laser field. Using synchronized XUV free-electron-laser and 800-nm NIR laser pulses, we observe a…

Measurements of the phase of two-photon matrix elements are presented for resonant and antiresonant two-color ionization of helium. A tunable, narrow-bandwidth, near-infrared (NIR) laser source is used for extreme ultra-violet (XUV)…

原子物理 · 物理学 2022-02-02 Lorenz Drescher , Tobias Witting , Oleg Kornilov , Marc J. J. Vrakking

The photoionization of a helium atom by short intense laser pulses is studied theoretically in the vicinity of the $2s2p\,^1P$ doubly-excited state with the intention to investigate the impact of the intensity and duration of the exciting…

原子物理 · 物理学 2017-09-20 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

We report on the experimental observation of strong-field dressing of an autoionizing two-electron state in helium with intense extreme-ultraviolet laser pulses from a free-electron laser. The asymmetric Fano line shape of this transition…

We investigate the photoionization spectrum of helium by attosecond XUV pulses both in the spectral region of doubly excited resonances as well as above the double ionization threshold. In order to probe for convergence, we compare three…

We integrate numerically the Schr\"odinger equation for the model helium atom irradiated by intense few-cycle laser pulse and find the emitted XUV spectra. They demonstrate resonant peaks at the frequencies of transitions from the…

光学 · 物理学 2025-05-09 S. A. Bondarenko , V. V. Strelkov

We study resonant two-photon ionization of helium atoms via the $1s3p$, $1s4p$ and $1s5p^1$P$_1$ states using the 15$^\mathrm{th}$ harmonic of a titanium-sapphire laser for the excitation and a weak fraction of the laser field for the…

Multiphoton ionization provides a clear window into the nature of electron correlations in the helium atom. In the present study, the final state energy range extends up to the region near the $N=2$ and $N=3$ ionization thresholds, where…

原子物理 · 物理学 2021-03-10 Yimeng Wang , Chris H. Greene

We discuss a method of solving the time dependent Schrodinger equation for atoms with two active electrons in a strong laser field, which we used in a previous paper [A. Scrinzi and B. Piraux, Phys. Rev. A 56, R13 (1997)] to calculate…

原子物理 · 物理学 2014-05-19 Armin Scrinzi , Bernard Piraux

Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…

Few-photon induced breakup of helium is studied using a newly developed ab initio numerical framework for solving the six-dimensional time-dependent Schroedinger equation. We present details of the method and calculate (generalized) cross…

原子物理 · 物理学 2010-06-11 R. Nepstad , T. Birkeland , M. Førre

Above 54.4 eV, two-photon double ionization of helium is dominated by a sequential absorption process, producing characteristic behavior in the single and triple differential cross sections. We show that the signature of this process is…

原子物理 · 物理学 2009-11-13 D. A. Horner , T. N. Rescigno , C. W. McCurdy

In a previous publication, procedures were proposed for unambiguously extracting amplitudes for single and double ionization from a time-dependent wavepacket by effectively propagating for an infinite time following a radiation pulse. Here…

原子物理 · 物理学 2009-11-13 A. Palacios , T. N. Rescigno , C. W. McCurdy

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

The concerted motion of two or more bound electrons governs atomic and molecular non-equilibrium processes and chemical reactions. It is thus a long-standing scientific dream to measure the dynamics of two bound correlated electrons in the…

We study resonant two-color two-photon ionization of Helium via the 1s3p 1P1 state. The first color is the 15th harmonic of a tunable titanium sapphire laser, while the second color is the fundamental laser radiation. Our method uses…

We develop an approximate model for the process of direct (nonsequential) two-photon double ionization of atoms. Employing the model, we calculate (generalized) total cross sections as well as energy-resolved differential cross sections of…

量子物理 · 物理学 2016-08-17 Morten Førre , Sølve Selstø , Raymond Nepstad

The multiconfigurational time-dependent Hartree-Fock method (MCTDHF) is applied for simulations of the two-photon ionization of Helium. We present results for the single- and double ionization from the groundstate for photon energies in the…

原子物理 · 物理学 2011-12-30 D. Hochstuhl , M. Bonitz

Strong-field manipulation of autoionizing states is a crucial aspect of electronic quantum control. Recent measurements of the attosecond transient absorption spectrum of helium dressed by a few-cycle visible pulse [Ott et al.,…

原子物理 · 物理学 2012-11-13 Luca Argenti , Christian Ott , Thomas Pfeifer , Fernando Martín

Two-photon atomic ionization driven by time-locked XUV and IR pulses allows to study dynamics of Fano resonances in time and energy domains. Different time evolution of the two interfering pathways leading to a Fano resonance can be…

原子物理 · 物理学 2026-03-03 Vladislav V. Serov , Anatoli S. Kheifets
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