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High-harmonic generation (HHG) is widely used for up-conversion of amplified (near) infrared ultrafast laser pulses to short wavelengths. We demonstrate that Ramsey-comb spectroscopy, based on two such pulses derived from a frequency-comb…

原子物理 · 物理学 2019-11-21 L. S. Dreissen , C. Roth , E. L. Gründeman , J. J. Krauth , M. Favier , K. S. E. Eikema

We studied the multi-plateau high-order harmonic generation (HHG) from solids numerically. It is found that the HHG spectrum in the second or higher plateau is redshifted in short laser pulses due to the nonadiabatic effect. The…

光学 · 物理学 2017-09-20 Guang-Rui Jia , Xue-Bin Bian

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

强关联电子 · 物理学 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki

Here we experimentally map the dynamics of electron plasma waves in laser solid interaction. We do time resolved measurements of second harmonic and hard X-ray generation from interaction of intense ($10^{16} W cm^{-2}$, 100 fs, 800nm)…

等离子体物理 · 物理学 2007-05-23 Arvinder S. Sandhu , G. Ravindra Kumar , S. Sengupta , A. Das , P. K. Kaw

We study theoretically the two-center interferences occurring in high harmonic generation from diatomic molecules. By solving the time-dependent Schroedinger equation, either numerically or with the molecular strong-field approximation, we…

光学 · 物理学 2017-07-12 F. Risoud , C. Lévêque , M. Labeye , J. Caillat , A. Maquet , P. Salières , R. Taïeb , T. Shaaran

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

强关联电子 · 物理学 2025-11-03 Takeshi Suzuki , Kozo Okazaki

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

原子物理 · 物理学 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

High-order harmonic generation (HHG) by hydrogenlike atoms/ions in the uniform periodic electric field, formed by the two linearly polarized counterpropagating laser beams of relativistic intensities, is studied. The relativistic quantum…

原子物理 · 物理学 2011-06-14 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

At the fundamental level, full description of light-matter interaction requires quantum treatment of both matter and light. However, for standard light sources generating intense laser pulses carrying quadrillions of photons in a coherent…

In this Letter, it is experimentally and theoretically shown that weak odd harmonics generated during the propagation of an infrared ultrashort ultra-intense pulse unexpectedly modify the nonlinear properties of the medium and lead to a…

光学 · 物理学 2015-06-18 P. Béjot , G. Karras , F. Billard , E. Hertz , B. Lavorel , E. Cormier , O. Faucher

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

光学 · 物理学 2022-03-03 Davis M. Welakuh , Prineha Narang

High-order harmonic generation (HHG) provides a powerful optical tool for probing ultrafast dynamics on the attosecond timescale. While its mechanisms in gases and solids are well-established, understanding nonlinear optical responses in…

Applying the semiclassical model, we identify two connected effects in intraband high-harmonic generation (HHG): (1) propagation time from the point of emission at the source to the point of detection, (2) beyond-electric-dipole corrections…

原子物理 · 物理学 2024-06-12 Simon Vendelbo Bylling Jensen , Lars Bojer Madsen

High harmonic generation due to the interaction of a short ultra relativistic laser pulse with overdense plasma is studied analytically and numerically. On the basis of the ultra relativistic similarity theory we show that the high harmonic…

等离子体物理 · 物理学 2009-11-11 T. Baeva , S. Gordienko , A. Pukhov

We study numerically the Bloch electron wavepacket dynamics in periodic potentials to simulate laser-solid interactions. We introduce a new perspective in the coordinate space combined with the motion of the Bloch electron wavepackets…

光学 · 物理学 2018-01-12 Tao-Yuan Du , Xiao-Huan Huang , Xue-Bin Bian

We study the phase matching of resonant high-harmonic generation (HHG) and high-order frequency mixing (HFM) in plasma. We solve numerically the propagation equations coupled with the time-dependent Schr\"odinger equation for the nonlinear…

光学 · 物理学 2024-04-30 Vasily V. Strelkov , Margarita A. Khokhlova

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

介观与纳米尺度物理 · 物理学 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

High-order harmonic generation (HHG) in isolated atoms and molecules has been widely utilized in extreme ultraviolet (XUV) photonics and attosecond pulse metrology. Recently, HHG has also been observed in solids, which could lead to…