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In this work, we systematically investigate the spectral and transport properties of exciton-polaritons under the explicit influence of intermolecular vibrational coupling, which introduces dynamic disorder. In the context of a…

化学物理 · 物理学 2025-12-03 Guangming Liu , Hsing-Ta Chen

Strong coupling between excitons and confined modes of light presents a promising pathway to tunable and enhanced energy transport in organic materials. By forming hybrid light-matter quasiparticles, exciton-polaritons, electronic…

化学物理 · 物理学 2024-11-01 Niclas Krupp , Gerrit Groenhof , Oriol Vendrell

While there have been numerous reports of long-range polariton transport at room-temperature in organic cavities, the spatio-temporal evolution of the propagation is scarcely reported, particularly in the initial coherent sub-ps regime,…

The performance of various quantum devices is fundamentally linked to the control of exciton transport. To explore this, we study the exciton transport of the two-dimensional multi-chain systems with different coupling configurations in an…

量子物理 · 物理学 2025-07-02 Jia-Hui Wang , Yu-Ren Shi , Ji-Ming Gao , Zi-Fa Yu , Ju-Kui Xue , Fang-Qi Hu

The interaction between coherent polaritons and incoherent excitons plays an important role in polariton physics. Using resonant pump-probe spectroscopy with selective excitation of single polariton branches, we investigate the different…

介观与纳米尺度物理 · 物理学 2016-11-16 N. Takemura , M. D. Anderson , S. Biswas , M. Navadeh-Toupchi , D. Y. Oberli , M. T. Portella-Oberli , B. Deveaud

Multi-exciton correlations shape the photo-induced response of nanostructured materials, particularly when interactions are enhanced by light confinement. Here multidimensional coherent spectroscopy is used to quantify biexciton and…

介观与纳米尺度物理 · 物理学 2025-07-11 Giuseppe Fumero , Jagannath Paul , Jared K. Wahlstrand , Alan D. Bristow

Exciton transport in 2D semiconductors holds promise for room-temperature, ultra-compact optoelectronic devices, but it is limited by short propagation distances. Hybridization of excitons with cavity photons to form exciton-polaritons can…

介观与纳米尺度物理 · 物理学 2025-07-08 Jamie M. Fitzgerald , Roberto Rosati , Ermin Malic

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

量子物理 · 物理学 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming

Strong light--matter interactions forming hybrid quasiparticles termed polaritons can specifically tailor molecular photophysics. In this spirit, enhancing energy transport has recently been of special interest. Exciton--exciton…

化学物理 · 物理学 2026-01-14 Luca Nils Philipp , Julian Lüttig , Roland Mitric

Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…

介观与纳米尺度物理 · 物理学 2024-08-05 Anna M. Grudinina , Nina S. Voronova

The concept of modifying molecular dynamics in strongly coupled exciton-polariton systems is an emerging topic in photonics due to its potential to produce customized chemical systems with tailored photophysical properties. However, before…

材料科学 · 物理学 2020-10-09 Bin Liu , Vinod M. Menon , Matthew Y. Sfeir

We present a many-body theory for exciton-trion-polaritons in doped two-dimensional materials. Exciton-trion-polaritons are robust coherent hybrid excitations involving excitons, trions, and photons. Signatures of these polaritons have been…

介观与纳米尺度物理 · 物理学 2021-03-31 Farhan Rana , Okan Koksal , Minwoo Jung , Gennady Shvets , A. Nick Vamivakas , Christina Manolatou

We theoretically study the transport of exciton polaritons under different applied photon potentials. The relation between the photon potentials and the thickness of the cavity layer is calculated by the finite element simulation. The…

光学 · 物理学 2015-10-28 Xudong Duan , Bingsuo Zou , Yongyou Zhang

Multi-particle correlations of exciton-polaritons and reservoir-excitons in the strong light-matter coupling regime dictate the quantum dynamics of optical microcavities. In this letter, we examine the many-body exciton-polariton dynamics…

Exciton-polaritons in semiconductor microcavities exhibit large two-body interactions that, thanks to ever refined nanotechnology techniques, are getting closer and closer to the quantum regime where single-photon nonlinearities start being…

Coupling excitons with quantized radiation has been shown to enable coherent ballistic transport at room temperature inside optical cavities. Previous theoretical works employ a simple description of the material, depicting it as a…

量子物理 · 物理学 2026-05-14 Saeed Rahmanian Koshkaki , Arshath Manjalingal , Logan Blackham , Arkajit Mandal

The interplay between exctions and vibrations is considered to be a key factor in determining the exciton transfer properties in light-harvesting exciton transfer complexes. Here we study this interplay theoretically in a model for exciton…

介观与纳米尺度物理 · 物理学 2018-05-25 Omer Goldberg , Yigal Meir , Yonatan Dubi

Excitation energy transport can be significantly enhanced by strong light-matter interactions. In the present work, we explore intriguing features of coherent transient exciton wave packet dynamics on a lossless disordered polaritonic wire.…

量子物理 · 物理学 2024-02-26 Gustavo J. R. Aroeira , Kyle T. Kairys , Raphael F. Ribeiro

The interaction of excitons with lattice vibrations underlies the scattering from bright to dark excitons as well as the coherent modulation of the exciton energy. Unlike the former mechanism, which involves phonons with finite momentum,…

介观与纳米尺度物理 · 物理学 2024-06-24 Enrico Perfetto , Kai Wu , Gianluca Stefanucci

Condensation of bosons causes spectacular phenomena such as superfluidity or superconductivity. Understanding the nature of the condensed particles is crucial for active control of such quantum phases. Fascinating possibilities emerge from…

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