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Identifying weakly coupled nuclear spins around single electron spins is a key step of implementing quantum information processing using coupled electron-nuclei spin systems or sensing like single spin nuclear magnetic resonance detection…

介观与纳米尺度物理 · 物理学 2015-01-08 Nan Zhao , Jörg Wrachtrup , Ren-Bao Liu

Quantum Information processing by NMR with small number of qubits is well established. Scaling to higher number of qubits is hindered by two major requirements (i) mutual coupling among qubits and (ii) qubit addressability. It has been…

量子物理 · 物理学 2009-11-10 Ranabir Das , Rangeet Bhattacharyya , Anil Kumar

Photons and nuclear spins are two well-known building blocks in quantum information science and technology. Establishing an efficient interface between optical photons and nuclear spins, while highly desirable for hybridizing these two…

量子物理 · 物理学 2023-03-02 Haowei Xu , Changhao Li , Guoqing Wang , Hua Wang , Hao Tang , Ariel Rebekah Barr , Paola Cappellaro , Ju Li

The electric quadrupole response is investigated theoretically by HFB and QPM calculations along the Sn isotopic chain with special emphasis on excitations above the first collective state and below the particle threshold. Depending on the…

核理论 · 物理学 2011-06-27 N. Tsoneva , H. Lenske

Entangled quantum states are an important element of quantum information techniques. We determine the requirements for states of quadrupolar nuclei with spins >1/2 to be entangled. It was shown that entanglement is achieved at low…

量子物理 · 物理学 2015-05-19 Gregory Furman , Victor Meerovich , Vladimir Sokolovsky

Quantum decoherence has been studied using nuclear magnetic resonance(NMR). By choosing one qubit to simulate environment, we examine the decoherence behavior of two quantum systems: a one qubit system and a two qubit system. The…

量子物理 · 物理学 2007-05-23 Jingfu Zhang , Zhiheng Lu , Lu Shan , Zhiwei Deng

A general algorithm for computing the quadrupole-hyperfine effects in the rovibrational spectra of polyatomic molecules is presented for the case of ammonia (NH$_3$). The method extends the general variational approach TROVE by adding the…

化学物理 · 物理学 2017-10-25 Andrey Yachmenev , Jochen Küpper

Nuclear magnetic resonance (NMR) is a powerful quantum probe, but the early conclusions on the physics of the cuprates, based on a limited set of data, have to be revised in view of recent findings and results from extensive literature…

超导电性 · 物理学 2022-06-29 Jürgen Haase

Our recent developments in in-situ nuclear magnetic resonance (NMR) spectroscopy under extreme conditions led to the observation of a wide variety of physical phenomena not accessible with standard high pressure experimental probes.…

Electric-dipole forbidden spectroscopic transitions in atoms form the basis of many advanced implementations of quantum computers, atomic clocks and quantum sensors. Coherently addressing such transitions in molecules which are among the…

We have performed nuclear quadrupole resonance (NQR) experiments on $^{47}$Ti nuclei in Dy$_2$Ti$_2$O$_7$ in the temperature range 70 -- 300 K in order to investigate the dynamics of $4f$ electrons with strong Ising anisotropy. A…

强关联电子 · 物理学 2008-06-04 K. Kitagawa , R. Higashinaka , K. Ishida , Y. Maeno , M. Takigawa

Nuclear spin optical rotation (NSOR) is a recently developed technique for detection of nuclear magnetic resonance via rotation of light polarization, instead of the usual long-range magnetic fields. NSOR signals depend on hyperfine…

化学物理 · 物理学 2012-02-21 Junhui Shi , Suvi Ikäläinen , Juha Vaara , Michael V. Romalis

We investigate analytically and numerically the Multiple Quantum (MQ) NMR dynamics in dipolar ordered spin systems of nuclear spins 1/2 at a low temperatures. We suggest two different methods of MQ NMR. One of them is based on the…

介观与纳米尺度物理 · 物理学 2013-09-24 G. B. Furman , V. M. Meerovich , V. L. Sokolovsky

We demonstrate a novel method for coherent optical manipulation of individual nuclear spins in the solid state, mediated by the electronic states of a proximal quantum emitter. Specifically, using the nitrogen-vacancy (NV) color center in…

量子物理 · 物理学 2020-04-22 M. L. Goldman , T. L. Patti , D. Levonian , S. F. Yelin , M. D. Lukin

Quantum spectroscopy with single two level systems has considerably improved our ability to detect weak signals. Recently it was realized that for classical signals, precision and resolution of quantum spectroscopy is limited mainly by…

量子物理 · 物理学 2018-08-01 Tuvia Gefen , Maxim Khodas , Liam P. McGuinness , Fedor Jelezko , Alex Retzker

The algebraic reformulation of molecular Quantum Electrodynamics (mQED) at finite temperatures is applied to Nuclear Magnetic Resonance (NMR) in order to provide a foundation for the reconstruction of much more detailed molecular…

量子物理 · 物理学 2020-09-25 Kolja Them

We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…

介观与纳米尺度物理 · 物理学 2015-06-04 A. Dréau , J. -R. Maze , M. Lesik , J. -F. Roch , V. Jacques

Sensing the internal dynamics of individual nuclear spins or clusters of nuclear spins has recently become possible by observing the coherence decay of a nearby electronic spin: the weak magnetic noise is amplified by a periodic,…

量子物理 · 物理学 2016-01-05 J. E. Lang , Ren-Bao Liu , T. S. Monteiro

By choosing H nucleus in Carbon-13 labelled trichloroethylene as one qubit environment, and two C nuclei as a two-qubit system, we have simulated quantum decoherence when the system lies in an entangled state using nuclear magnetic…

量子物理 · 物理学 2009-09-29 Jingfu Zhang , Zhiheng Lu , Lu Shan , Zhiwei Deng

The ongoing miniaturization in nanoscience and -technology challenges the sensitivity and selectivity of experimental analysis methods to the ultimate level of single atoms and molecules. A promising new approach, addressed here, focuses on…

介观与纳米尺度物理 · 物理学 2014-03-28 Stefan Müllegger , Stefano Tebi , Amal K. Das , Wolfgang Schöfberger , Felix Faschinger , Reinhold Koch