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In this work we identify coherent electron-vibron interactions between near-resonant and non-resonant electronic levels that contribute beyond standard optomechanical models for off-resonant or resonance SERS. By developing an open-system…

量子物理 · 物理学 2024-01-19 Miguel A. Martínez-García , Diego Martín-Cano

Nanoscale gaps between adjacent metallic nanostructures give rise to extraordinarily large field enhancements, known as "hot spots", upon illumination. Incident light with the electric field polarized across the gap (along the interparticle…

介观与纳米尺度物理 · 物理学 2013-03-27 Joseph B. Herzog , Mark W. Knight , Yajing Li , Kenneth M. Evans , Naomi J. Halas , Douglas Natelson

Optical nonlinearities are crucial for advanced photonic technologies since they allow photons to be managed by photons. Exciton-polaritons resulting from strong light-matter coupling are hybrid in nature: they combine small mass and high…

All-inorganic halide perovskites have received a lot of attention as attractive alternatives to overcome the stability issues of hybrid halide perovskites that are commonly associated with organic cations. To find a compromise between the…

材料科学 · 物理学 2026-04-28 Mike Pols , Adri C. T. van Duin , Sofía Calero , Shuxia Tao

Mixed-halide perovskites offer a route to enhance phase stability and modify optoelectronic properties. Here, we use large-scale molecular dynamics simulations with a reactive force field to investigate defects in…

材料科学 · 物理学 2026-05-12 Konrad Wilke , Mike Pols , Titus S. van Erp , Geert Brocks , Shuxia Tao

We report a comparative study of temperature-dependent photoluminescence and structural dynamics of two perovskite semiconductors, the chalcogenide BaZrS$_3$ (BZS) and the halide CsPbBr$_3$ (CPB). These materials have similar crystal…

材料科学 · 物理学 2024-04-16 K. Ye , M. Menahem , T. Salzillo , F. Knoop , B. Zhao , S. Niu , O. Hellman , J. Ravichandran , R. Jaramillo , O. Yaffe

Exciton-phonon interactions govern the optical response of semiconductors, yet disentangling multiple coupling channels in lead halide perovskites remains challenging. We investigate CsPbBr3 microcrystals using photoluminescence, Raman and…

The creation of light-matter hybrid states, polaritons, in a cavity offers new intriguing opportunities to manipulate the electronic structure and electron dynamics of atoms and molecules. Here, we investigate the effect of electronic…

量子物理 · 物理学 2025-07-30 Paul A. Albrecht , Eric W. Fischer , Tillmann Klamroth , Peter Saalfrank

Light-matter interactions in crystals are powerful tools that seamlessly allow both functionalities of sizeable bandgap modulation and non-invasive spectroscopy. While we often assume that the border between the two regimes of modulation…

Sign-changing interactions constitute a crucial ingredient in the creation of frustrated many-body systems such as spin glasses. We present here the demonstration of a photon-mediated sign-changing interaction between Bose-Einstein…

量子气体 · 物理学 2019-05-23 Yudan Guo , Ronen M. Kroeze , Varun V. Vaidya , Jonathan Keeling , Benjamin L. Lev

We investigate a semiconductor $p$-$n$ junction in contact with superconducting leads that is operated under forward bias as a light-emitting diode. The presence of superconductivity results in a significant increase of the…

介观与纳米尺度物理 · 物理学 2015-05-12 Patrik Hlobil , Peter P. Orth

Halide perovskites have emerged as promising materials for next-generation photovoltaics, laser sources and X-ray detectors. There is intense debate as to whether some photoactive halide perovskites exhibit ferroelectric behaviour and…

材料科学 · 物理学 2026-01-21 Weilun Li , Qimu Yuan , Michael B. Johnston , Joanne Etheridge

The influence of the Hall voltage on the photoluminescence of a dense hydrodynamic electron-hole plasma laser generated in a mesoscopic n-doped GaAs channel under intense laser excitation is studied. Laser excitation induces an interband…

介观与纳米尺度物理 · 物理学 2026-05-19 Yu. A. Pusep , M. A. T. Patricio , G. M. Jacobsen , M. D. Teodoro , G. M. Gusev , A. K. Bakarov

Mixing iodide and bromide in halide perovskite semiconductors is an effective strategy to tune their bandgap, therefore mixed-halide perovskites hold great promise for color-tunable LEDs and tandem solar cells. However, the bandgap of…

We investigate photoluminescence from a high-density electron-hole plasma in semiconductor quantum wells created via intense femtosecond excitation in a strong perpendicular magnetic field, a fully-quantized and tunable system. At a…

其他凝聚态物理 · 物理学 2009-11-11 Y. D. Jho , X. Wang , J. Kono , D. H. Reitze , X. Wei , A. A. Belyanin , V. V. Kocharovsky , Vl. V. Kocharovsky , G. S. Solomon

We construct a theory for Bose-Einstein condensation of light in nano-fabricated semiconductor microcavities. We model the semiconductor by one conduction and one valence band which consist of electrons and holes that interact via a Coulomb…

量子气体 · 物理学 2016-07-27 A. -W. de Leeuw , E. C. I. van der Wurff , R. A. Duine , D. van Oosten , H. T. C. Stoof

Photons do not carry sufficient momentum to induce indirect optical transitions in semiconducting materials such as silicon, necessitating the assistance of lattice phonons to conserve momentum. Compared to direct bandgap semiconductors,…

Recent advances in colloidal synthesis methods have led to increased research focus on halide perovskites. Due to highly ionic crystal structure of perovskite materials, stability issue pops up especially against polar solvents such as…

材料科学 · 物理学 2018-03-08 Baris Akbali , Gokhan Topcu , Tugrul Guner , Mehmet Ozcan , Mustafa Muammer Demir , Hasan Sahin

Entangled photon sources (EPS), the major building block for a variety of quantum communication protocols, are commonly developed by utilizing the spontaneous parametric down-conversion (SPDC) in $\chi^{2}$ nonlinear bulk optical materials.…

量子物理 · 物理学 2022-07-14 Sandeep Singh , Vimlesh Kumar , Anirban Ghosh , G. K. Samanata

We report on enhanced fluorescence of lead sulfide quantum dots interacting with leaky modes of slab-type silicon photonic crystals. The photonic crystal slabs were fabricated supporting leaky modes in the near infrared wavelength range.…

光学 · 物理学 2017-08-23 C. Barth , S. Roder , D. Brodoceanu , T. Kraus , M. Hammerschmidt , S. Burger , C. Becker