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相关论文: Odd-parity multipole order in the spin-orbit coupl…

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The 5d pyrochlore oxide superconductor Cd2Re2O7 (CRO) has attracted significant interest as a spin-orbit-coupled metal (SOCM) that spontaneously undergoes a phase transition to an odd-parity multipole phase by breaking the spatial inversion…

强关联电子 · 物理学 2023-09-18 Daigorou Hirai , Atsuhito Fukui , Hajime Sagayama , Takumi Hasegawa , Zenji Hiroi

The 5d-transition metal pyrochlore oxide Cd2Re2O7, which was recently suggested to be a prototype of the spin-orbit-coupled metal [Phys. Rev. Lett. 115, 026401 (2015)], exhibits an inversion-symmetry breaking (ISB) transition at 200 K and a…

The superconducting pyrochlore oxide Cd2Re2O7 is revisited with a particular emphasis on the sample-quality issue. The compound has drawn attention as the only superconductor (Tc = 1.0 K) that has been found in the family of…

Strong electron interactions can drive metallic systems toward a variety of well-known symmetry-broken phases, but the instabilities of correlated metals with strong spin-orbit coupling have only recently begun to be explored. We uncovered…

强关联电子 · 物理学 2017-04-26 J. W. Harter , Z. Y. Zhao , J. -Q. Yan , D. G. Mandrus , D. Hsieh

We report the X-ray study for the pyrochlore oxide Cd2Re2O7. Two symmetry-lowering structural transitions were observed at Ts1=200K and Ts2=120K. The former is of the second order from the ideal cubic pyrochlore structure with space group…

强关联电子 · 物理学 2009-11-07 Jun-Ichi Yamaura , Zenji Hiroi

Theoretical model is presented to describe the anomalous ordered phase of Pr ions in PrBa_2Cu_3O_(6+x) below T_Pr = 12-17 K. The model considers the Pr multipole degrees of freedom and coupling between the Cu and Pr subsystems. We identify…

强关联电子 · 物理学 2015-05-19 A. Kiss , F. Simon

The superconducting pyrochlore oxide Cd2Re2O7 (Tc = 1 K), which is now considered as a candidate of the spin-orbit-coupled metal, shows an inversion-symmetry-breaking structural transition at Ts1 = 200 K. Ts1 decreases with increasing…

强关联电子 · 物理学 2018-04-30 Yasuhito Matsubayashi , Takumi Hasegawa , Norio Ogita , Jun-ichi Yamaura , Zenji Hiroi

A rare combination of strong spin-orbit coupling and electron-electron correlations makes the iridate Mott insulator Sr$_2$IrO$_4$ a promising host for novel electronic phases of matter. The resemblance of its crystallographic, magnetic and…

强关联电子 · 物理学 2016-01-11 L. Zhao , D. H. Torchinsky , H. Chu , V. Ivanov , R. Lifshitz , R. Flint , T. Qi , G. Cao , D. Hsieh

We report a structural phase transition found at Ts = 200 K in a pyrochlore oxide Cd2Re2O7 which shows superconductivity at Tc = 1.0 K. X-ray diffractionexperiments indicate that the phase transition is of the second order, from a…

超导电性 · 物理学 2009-11-07 M. Hanawa , J. Yamaura , Y. Muraoka , F. Sakai , Z. Hiroi

In electronic solids with strong spin-orbit interactions (SOIs), the spin and orbital degrees of freedom of an electron are quantum mechanically entangled, which may result in an exotic multipolar order instead of a conventional dipolar…

强关联电子 · 物理学 2020-07-01 Daigorou Hirai , Hajime Sagayama , Shang Gao , Hiroyuki Ohsumi , Gang Chen , Taka-hisa Arima , Zenji Hiroi

We study the lead rhenium oxide PbRe2O6 as a candidate spin-orbit-coupled metal (SOCM), which has attracted much attention as a testing ground for studying unconventional Fermi liquid instability associated with a large spin-orbit…

Single crystal X-ray diffraction measurements have been carried out on Cd_2Re_2O_7 near and below the phase transition it exhibits at Tc' ~195 K. Cd_2Re_2O_7 was recently discovered as the first, and to date only, superconductor with the…

强关联电子 · 物理学 2009-11-07 J. P. Castellan , B. D. Gaulin , J. van Duijn , M. J. Lewis , M. D. Lumsden , R. Jin , J. He , S. E. Nagler , D. Mandrus

Full pattern Le-Bail refinement using x-ray powder diffraction profiles of Sr1-xCaxTiO3 for x=0.02, 0.04 in the temperature range 12 to 300 K reveals anomalies in the unit cell parameters at 170, 225 K due to an antiferrodistortive (cubic…

材料科学 · 物理学 2015-05-13 Sanjay Kumar Mishra , Dhananjai Pandey

We report our theoretical results on the order parameters for the pyrochlore metal Cd$_2$Re$_2$O$_7$, which undergoes enigmatic phase transitions with inversion symmetry breaking. By carefully examining active electronic degrees of freedom…

强关联电子 · 物理学 2019-04-17 Satoru Hayami , Yuki Yanagi , Hiroaki Kusunose , Yukitoshi Motome

The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single…

强关联电子 · 物理学 2024-07-18 Harish Kumar , M. Köpf , P. Telang , N. Bura , A. Jesche , P. Gegenwart , C. A. Kuntscher

The subtle interplay between spin-orbit coupling, exchange interactions, and cation ordering can lead to exotic magnetic states in transition-metal ions. We report a comprehensive study of the Re-based (5$d^1$) ordered double perovskite…

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

Recently, a general formalism was presented for gyrotropic, ferroelectric, and multipolar order in spin-orbit coupled metals induced by spin-spin interactions. Here, I point out that the resulting order parameters are equivalent to…

强关联电子 · 物理学 2015-08-12 M. R. Norman

Evidence for another phase transition at 120 K in the metallic pyrochlore oxide Cd2Re2O7, following the structural transition at 200 K and followed by the superconducting transition at 1.0 K, is given through resistivity, magnetoresistance,…

强关联电子 · 物理学 2009-11-07 Zenji Hiroi , Jun-Ichi Yamaura , Yuji Muraoka , Masafumi Hanawa

The structural, electronic, and optical properties of pyrochlore-type Pb$_{2}$Ir$_{2}$O$_{6}$O'$_{0.55}$, which is a metal without spatial inversion symmetry at room temperature, were investigated. Structural analysis revealed that the…

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