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相关论文: Strong coupling electron-photon dynamics: a real-t…

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A model designed to mimic the implications of the collective optical response of molecular ensembles in optical cavities on molecular vibronic dynamics is investigated. Strong molecule-radiation field coupling is often reached when a large…

化学物理 · 物理学 2022-10-05 Bingyu Cui , Abraham Nitzan

The quantum dynamics of a strongly driven, strongly coupled single-atom-cavity system is studied by evaluating time-dependent second- and third-order correlations of the emitted photons. The coherent energy exchange, first, between the atom…

A comprehensive theoretical understanding of electron-photon correlation is essential for describing the reshaping of molecular orbitals in quantum electrodynamics (QED) environments. The strong coupling QED Hartree-Fock (SC-QED-HF) theory…

化学物理 · 物理学 2024-09-04 Yassir El Moutaoukal , Rosario R. Riso , Matteo Castagnola , Henrik Koch

The concept of modifying molecular dynamics in strongly coupled exciton-polariton systems is an emerging topic in photonics due to its potential to produce customized chemical systems with tailored photophysical properties. However, before…

材料科学 · 物理学 2020-10-09 Bin Liu , Vinod M. Menon , Matthew Y. Sfeir

We propose a method to achieve photon pair propagation in an array of three-level superconducting circuits. Assuming experimentally accessible three-level artificial atoms with strong anharmonicity coupled via microwave transmission lines…

量子物理 · 物理学 2020-10-21 Sayan Lahiri , Suman Mondal , Kanhaiya Pandey , Tapan Mishra

This is a tutorial-style introduction to the field of molecular polaritons. We describe the basic physical principles and consequences of strong light-matter coupling common to molecular ensembles embedded in UV-visible or infrared…

化学物理 · 物理学 2020-03-18 Felipe Herrera , Jeffrey Owrutsky

Many optically active systems possess spatially asymmetric electron orbitals. These generate permanent dipole moments, which can be stronger than the corresponding transition dipole moments, significantly affecting the system dynamics and…

量子物理 · 物理学 2023-04-21 Adam Burgess , Marian Florescu , Dominic Michael Rouse

Strong-coupling between light and matter produces hybridized states (polaritons) whose delocalization and electromagnetic character allow for novel modifications in spectroscopy and chemical reactivity of molecular systems. Recent…

Recent advancements in time-resolved electron and photon detection enable novel correlative measurements of electrons and their associated cathodoluminescence (CL) photons within a transmission electron microscope. These studies are pivotal…

Electromagnetic (EM) probes such as photons and dileptons provide direct insight into the space-time evolution of the hot and dense matter formed in heavy-ion collisions. Being unaffected by strong interactions, they serve as penetrating…

核实验 · 物理学 2025-10-01 Sebastian Scheid

The hybridization of light and matter excitations in the form of polaritons has enabled major advances in understanding and controlling optical nonlinearities. Entering the quantum regime of strong interactions between individual photons…

Photons and dileptons are being used to probe the properties of nuclear and quark-gluon matter at high energy densities. This is an area where theory and experiment are driving each other to obtain solid results. However, it is important to…

核理论 · 物理学 2008-11-26 J. Kapusta

Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…

原子与分子团簇 · 物理学 2011-05-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

We theoretically model the electronic dynamics of a coupled quantum dot pair in a static electric field. We then investigate the possibility of polarization-entangled photon emission from the radiative cascade of the molecular biexciton…

介观与纳米尺度物理 · 物理学 2016-03-23 Cameron Jennings , Michael Scheibner

Molecular polaritons are the optical excitations which emerge when molecular transitions interact strongly with confined electromagnetic fields. Increasing interest in the hybrid molecular-photonic materials that host these excitations…

介观与纳米尺度物理 · 物理学 2018-02-26 Raphael F. Ribeiro , Luis A. Martínez-Martínez , Matthew Du , Jorge Campos-Gonzalez-Angulo , Joel Yuen-Zhou

We study the real-time evolution of an electron influenced by intense electromagnetic fields using the time-dependent basis light-front quantization (tBLFQ) framework. We focus on demonstrating the non-perturbative feature of the tBLFQ…

核理论 · 物理学 2017-06-07 Guangyao Chen , Xingbo Zhao , Yang Li , Kirill Tuchin , James P. Vary

The interaction of strong laser fields with matter intrinsically provides powerful tools to image transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules and…

Coupling photons to Rydberg excitations in a cold atomic gas yields unprecedentedly large optical nonlinearities at the level of individual light quanta, where the formation of nearby dark-state polaritons is blocked by the strong…

量子物理 · 物理学 2017-07-19 Callum R. Murray , Thomas Pohl

The interaction of a single photon with an individual two-level system is the textbook example of quantum electrodynamics. Achieving strong coupling in this system so far required confinement of the light field inside resonators or…

Experimental evidence of strong coupling between excitons confined in a quantum well and the photonic modes of a two-dimensional dielectric lattice is reported. Both resonant scattering and photoluminescence spectra at low temperature show…