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Electrons in the pyrochore iridates experience a large interaction energy in addition to a strong spin-orbit interaction. Both features make the iridates promising for realizing novel states such as the Topological Mott Insulator. The…

强关联电子 · 物理学 2017-09-21 Tian Liang , Timothy H. Hsieh , Jun J. Ishikawa , Satoru Nakatsuji , Liang Fu , N. P. Ong

Materials with strong spin-orbit interactions are presently a main target in the search for systems with novel magnetic properties. Magnetic anisotropies can be very large in such compounds, ranging from strongly frustrated Kitaev exchange…

The low-temperature spin dynamics of the orthorhombic TbFeO$_3$ perovskite has been studied. It has been found that the inelastic neutron scattering (INS) spectrum contains two modes corresponding to different sublattices in the compound.…

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

In the search for topological phases in correlated electron systems, iridium-based pyrochlores A2Ir2O7 -- materials with 5d transition-metal ions -- provide fertile grounds. Several novel topological states have been predicted but the…

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

强关联电子 · 物理学 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

Building a full understanding of the complex magnetism in the rare-earth pyrochlore iridates, A2Ir2O7, is an ongoing issue in condensed matter physics. The possibility of two interpenetrating and interacting frustrated magnetic pyrochlore…

强关联电子 · 物理学 2021-01-01 Ross H. Colman , Kristina Vlaskova , Adam Berlie , Milan Klicpera

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

We construct a model for interacting electrons with strong spin orbit coupling in the pyrochlore iridates. We establish the importance of the direct hopping process between the Ir atoms and use the relative strength of the direct and…

强关联电子 · 物理学 2012-02-02 William Witczak-Krempa , Yong Baek Kim

Metal-insulator transitions in pyrochlore iridates (A2Ir2O7) are believed to occur due to subtle interplay of spin-orbit coupling, geometric frustration, and electron interactions. In particular, the nature of magnetic ordering of iridium…

强关联电子 · 物理学 2014-07-29 Eric Kin-Ho Lee , Subhro Bhattacharjee , Yong Baek Kim

Topological magnons are bosonic analogues of topological fermions in electronic systems. They have been studied extensively by theory but rarely realized by experiment. Here, by performing inelastic neutron scattering measurements on single…

We used resonant inelastic x-ray scattering to reveal the nature of magnetic interactions in Sr2IrO4, a 5d transition-metal oxide with a spin-orbit entangled ground state and Jeff=1/2 magnetic momemts, referred to as 'isospins'. The magnon…

Twisted transition metal dichalcogenides (tTMDs) provide a highly tunable platform to explore the interplay between strong correlation and topology. Among them, the properties involving the charge degree of freedom have been extensively…

强关联电子 · 物理学 2025-08-25 Wei-Tao Zhou , Zhao-Yang Dong , Zhao-Long Gu , Jian-Xin Li

Transition-metal ions with $5d^2$ electronic configuration in a cubic crystal field are prone to have a vanishing dipolar magnetic moment but finite higher-order multipolar moments, and they are expected to exhibit exotic physical…

We use ab initio electronic structure calculations within the generalized gradient approximation (GGA+U) to density functional theory (DFT) to determine the microscopic exchange interactions in the series of orthorhombic rare-earth…

材料科学 · 物理学 2015-04-22 Natalya S. Fedorova , Claude Ederer , Nicola A. Spaldin , Andrea Scaramucci

We explore the relative strengths of spin orbit coupling and crystal field splitting in the Ir5+ compounds Ba2-xSrxYIrO6. In the case of strong spin orbit coupling and regular Ir5+ octahedra, one expects a nonmagnetic J = 0 state; in the…

强关联电子 · 物理学 2016-03-29 Brendan F. Phelan , Elizabeth M. Seibel , Daniel Badoe , Weiwei Xie , R. J. Cava

The possible existence of topological insulators in cubic pyrochlore iridates A$_{2}$Ir$_{2}$O$_{7}$ (A = Y or rare-earth elements) is investigated by taking into account the strong spin-orbit coupling and trigonal crystal field effect. It…

强关联电子 · 物理学 2015-03-14 Bohm-Jung Yang , Yong Baek Kim

The tunable band structure and nontrivial topology of multilayer rhombohedral graphene lead to a variety of correlated electronic states with isospin orders-meaning ordered states in the combined spin and valley degrees of freedom-dictated…

We used single-crystal x-ray and neutron diffraction to investigate the crystal and magnetic structures of trigonal lattice iridate Ca2Sr2IrO6. The crystal structure is determined to be $R\bar3$ with two distinct Ir sites. The system…

$\gamma$-triclinic and $\alpha$-monoclinic polymorphs of CoV$_{2}$O$_{6}$ are two of the few known transition metal ion based materials that display stepped $1/3$ magnetization plateaus at low temperatures. Neutron diffraction [M. Markkula…

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