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Based on density functional theory calculations and group theoretical analysis, we have studied NaLaMnWO$_{6}$ compound which has been recently synthesized [Phys. Rev. B 79, 224428 (2009)] and belongs to the $AA'BB'{\rm O}_{6}$ family of…

材料科学 · 物理学 2017-09-13 T. Fukushima , A. Stroppa , S. Picozzi , J. M. Perez-Mato

The magnetic correlations in double perovskites La2Mn2-xNixO6 (x = 0.5, 0.75, 1.0, 1.25 and 1.5) have been systematically investigated across macroscopic, mesoscopic, and microscopic length scales using temperature-dependent bulk DC…

材料科学 · 物理学 2025-10-14 A. K. Bera , K. S. Chikara , B. Saha , S. M. Yusuf , Mohd. Nasir , S. Sen

The search for room-temperature magnetocaloric materials for refrigeration has led to investigations of double perovskites. In particular, a puzzle has appeared in the La$_2$MnNiO$_6$, La$_2$MnCoO$_6$ and La$_2$MnFeO$_6$ family of…

Recent experimental and theoretical work has shown that the double perovskite NaLaMnWO$_6$ exhibits antiferromagnetic ordering owing to the Mn $d$ states, and computational studies further predict it to exhibit a spontaneous electric…

材料科学 · 物理学 2015-11-18 Joshua Young , Alessandro Stroppa , Silvia Picozzi , James M. Rondinelli

Magnetic refrigeration at room-temperature is a technology that could potentially be more environmentally-friendly, efficient and affordable than traditional refrigeration. The search for suitable materials for magnetocaloric refrigeration…

强关联电子 · 物理学 2019-03-13 C. Gauvin-Ndiaye , A. -M. S. Tremblay , R. Nourafkan

Among multifunctional double perovskite oxides, La2NiMnO6 has recently drawn significant attention due to its importance both in terms of understanding of fundamental physics and potential for device applications. The relative alteration in…

Despite the great technological and scientific importance, a well-controlled coupled behavior in magnetoelectric multiferroic materials at room temperature remains challenging. We demonstrate that the self-ordered A2BBO6 (e.g., A = La, B =…

材料科学 · 物理学 2015-05-14 M. P. Singh , K. D. Truong , S. Jandl , P. Fournier

Double-perovskite A2BB'O6 oxides with magnetic B and B' ions and E*-type antiferromagnetic order (E*-AFM, i.e. the ++-- structure) are believed to exhibit promising multiferroic properties, and Y2CoMnO6 (YCMO) is one candidate in this…

材料科学 · 物理学 2015-10-28 C. Y. Ma , S. Dong , P. X. Zhou , Z. Z. Du , M. F. Liu , H. M. Liu , Z. B. Yan , J. M. Liu

The non-stoichiometric double perovskite oxide La2Ni1.19Os0.81O6 was synthesized by solid state reaction and its crystal and magnetic structures were investigated by powder x-ray and neutron diffraction. La2Ni1.19Os0.81O6 crystallizes in…

We present a comprehensive study on the magnetic structure, dynamics, and phase evolution in the single-phase double perovskite $La_2CoMnO_6$. The mixed valence state due to oxygen deficiency is verified by X-ray photoelectron spectroscopy,…

The electron spin polarization on half-metallic double-perovskites is usually conditioned to the ordered rock-salt arrangement of the transition-metal ions along the lattice. In this work, we investigate a polycrystalline sample of the…

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

In previous studies, we have reported that double perovskite La2NiMnO6 presents a non-negligible potential for room temperature magnetocaloric tasks. With the aim of improving even further the cooling performances and the working…

Coupling between different interactions allows to control physical aspects in multifunctional materials by perturbing any of the degrees of freedom. Here, we aim to probe the correlation among structural, electronic and magnetic observables…

Double perovskites provide a unique opportunity to induce and control multiferroic behaviors in oxide systems. The appealing possibility to design materials with a strong coupling between the magnetization and the polarization fields may be…

材料科学 · 物理学 2009-04-06 M. P. Singh , K. D. Truong , P. Fournier , P. Rauwel , E. Rauwel , L. P. Carignan , D. Menard

The magnetism of double perovskites is a complex phenomenon, determined from intra- or interatomic magnetic moment interactions, and strongly influenced by geometry. We take advantage of the complementary length and time scales of the muon…

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

We report multiferroic behavior in double perovskite Y2CoMnO6 with ferroelectric transition temperature Tc = 80K. The origin of ferroelectricity is associated with magnetic ordering of Co2+ and Mn4+ moments in a up-up-down-down arrangement.…

材料科学 · 物理学 2015-06-15 G. Sharma , J. Saha , S. Patnaik

We present a new member of the multiferroic oxides, Lu$_2$MnCoO$_6$, which we have investigated using X-ray diffraction, neutron diffraction, specific heat, magnetization, electric polarization, and dielectric constant measurements. This…

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