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Stable structures of layered SnS and SnSe and their associated electronic and vibrational spectra are predicted using first-principles DFT calculations. The calculations show that both materials undergo a phase transformation upon thinning…

材料科学 · 物理学 2019-06-04 Antoine Dewandre , Matthieu J. Verstraete , Nicole Grobert , Zeila Zanolli

Chiral interaction between light and two-dimensional transition metal dichalcogenides (2D-TMDs) has recently drawn enormous scientific attention. The optical selection rules of these atomically thin semiconductors allow the attribution of a…

光学 · 物理学 2021-06-08 Irina Komen , Sabrya E. van Heijst , Sonia Conesa-Boj , L. Kuipers

Phonons and magnons are engineered by periodic potential landscapes in phononic and magnonic crystals, and their combined studies may enable valley phonon transport tunable by the magnetic field. Through nonreciprocal surface acoustic wave…

介观与纳米尺度物理 · 物理学 2023-07-13 Liyang Liao , Jorge Puebla , Kei Yamamoto , Junyeon Kim , Sadamichi Meakawa , Yunyoung Hwang , You Ba , Yoshichika Otani

By enabling control of valley degrees of freedom in transition-metal dichalcogenides, valley-selective circular dichroism has become a key concept in valleytronics. In this manuscript, we show that valley excitons -- bound electron-hole…

材料科学 · 物理学 2022-11-21 Fabio Caruso , Maximilian Schebek , Yiming Pan , Cecilia Vona , Claudia Draxl

Manipulating quantum states through light-matter interactions has been actively pursued in two-dimensional (2D) materials research. Significant progress has been made towards the optical control of the valley degrees of freedom in…

材料科学 · 物理学 2023-10-17 Jiawei Ruan , Zhenglu Li , Chin Shen Ong , Steven G. Louie

Methods to generate spin-polarised electronic states in non-magnetic solids are strongly desired to enable all-electrical manipulation of electron spins for new quantum devices. This is generally accepted to require breaking global…

Preserving a high degree of valley polarization of excitons in photo-excited transition-metal dichalcogenide monolayers (TMD-MLs) is desirable for the valley-based photonic applications, but widely recognized as a hard task hindered by the…

介观与纳米尺度物理 · 物理学 2020-10-13 Ping-Yuan Lo , Guan-Hao Peng , Wei-Hua Li , Yi Yang , Shun-Jen Cheng

Valleytronics is a rising topic to explore the emergent degree of freedom for charge carriers in energy band edges and has attracted a great interest due to many intriguing quantum phenomena and potential application in information…

A class of septuple-atomic-layer two-dimensional (2D) materials, MA$_2$Z$_4$, is sought as an alternative to 2D hexagonal transition metal dichalcogenides in the field of valleytronics and spintronics. In these materials, the structural…

材料科学 · 物理学 2023-06-27 Sajjan Sheoran , Ankita Phutela , Ruman Moullik , Saswata Bhattacharya

Optical spectroscopy in high magnetic fields $B\leq65$ T is used to reveal the very different nature of carriers in monolayer and bulk transition metal dichalcogenides. In monolayer WSe$_{2}$, the exciton emission shifts linearly with the…

介观与纳米尺度物理 · 物理学 2015-06-16 A. A. Mitioglu , P. Plochocka , Á. Granados del Aguila , P. C. M. Christianen , G. Deligeorgis , S. Anghel , L. Kulyuk , D. K. Maude

We report experimental observation of 2s exciton radiative emission from monolayer tungsten diselenide, enabled by hexagonal boron nitride protected high-quality samples. The 2s luminescence is highly robust and persists up to 150K,…

介观与纳米尺度物理 · 物理学 2018-01-31 Shao-Yu Chen , Thomas Goldstein , Jiayue Tong , Takashi Taniguchi , Kenji Watanabe , Jun Yan

Monolayer group-VIB transition metal dichalcogenides have recently emerged as a new class of semiconductors in the two-dimensional limit. The attractive properties include: the visible range direct band gap ideal for exploring…

介观与纳米尺度物理 · 物理学 2015-07-30 Hongyi Yu , Xiaodong Cui , Xiaodong Xu , Wang Yao

The valley degree of freedom in layered transition-metal dichalcogenides (MX2) provides the opportunity to extend functionalities of novel spintronics and valleytronics devices. Due to spin splitting induced by spin-orbital coupling (SOC),…

介观与纳米尺度物理 · 物理学 2014-09-16 Hongtao Yuan , Xinqiang Wang , Biao Lian , Haijun Zhang , Xianfa Fang , Bo Shen , Gang Xu , Yong Xu , Shou-Cheng Zhang , Harold Y. Hwang , Yi Cui

Broken spatial inversion symmetry in semiconducting materials with time-reversal pair valleys can exhibit valley polarization. Based on first-principles calculations, here we propose a lateral heterostructure of kagome lattice of hBN and…

材料科学 · 物理学 2023-11-23 Souren Adhikary , Sasmita Mohakud , Sudipta Dutta

Coherent control and manipulation of quantum degrees of freedom such as spins forms the basis of emerging quantum technologies. In this context, the robust valley degree of freedom and the associated valley pseudospin found in…

介观与纳米尺度物理 · 物理学 2022-11-17 Mandeep Khatoniar , Nicholas Yama , Areg Ghazaryan , Sriram Guddala , Pouyan Ghaemi , Kausik Majumdar , Vinod Menon

The electron's charge and spin degrees of freedom are at the core of modern electronic devices. With the in-depth investigation of two-dimensional materials, another degree of freedom, valley, has also attracted tremendous research…

材料科学 · 物理学 2023-09-06 Ping Li , Bang Liu , Wei-Xi Zhang , Zhi-Xin Guo

Degenerate extrema in the energy dispersion of charge carriers in solids, also referred to as valleys, can be regarded as a binary quantum degree of freedom, which can potentially be used to implement valleytronic concepts in van der Waals…

Momentum-resolved spin textures and potential valley-contrasting physical properties in the momentum space are two intriguing characteristics of noncentrosymmetric materials, and they have broad applications in spintronics and…

材料科学 · 物理学 2026-05-12 Zeyu Yin , Li Liang , Zhichao Zhou , Xiao Li

Breaking space-time symmetries in two-dimensional crystals (2D) can dramatically influence their macroscopic electronic properties. Monolayer transition-metal dichalcogenides (TMDs) are prime examples where the intrinsically broken crystal…

介观与纳米尺度物理 · 物理学 2015-09-04 Edbert J. Sie , James W. McIver , Yi-Hsien Lee , Liang Fu , Jing Kong , Nuh Gedik

Optical control of spin in semiconductors has been pioneered using nanostructures of III-V and II-VI semiconductors, but the emergence of two-dimensional van der Waals materials offers an alternative low-dimensional platform for spintronic…