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The magnetic properties of a new family of molecular-based quasi-two dimension $S=1/2$ Heisenberg antiferromagnets are reported. Three compounds, ($Cu(pz)_2(ClO_4)_2$, $Cu(pz)_2(BF_4)_2$, and $[Cu(pz)_2(NO_3)](PF_6)$) contain similar planes…

$^{31}$P nuclear magnetic resonance (NMR) measurements have been carried out to investigate the magnetic properties and spin dynamics of Fe$^{3+}$ ($S$ = 5/2) spins in the two-dimensional triangular lattice (TL) compound…

强关联电子 · 物理学 2022-11-23 Devi V. Ambika , Qing-Ping Ding , Sebin J. Sebastian , Ramesh Nath , Yuji Furukawa

The spin dynamics of the semiclassical Heisenberg model with uniaxial anisotropy, on the layered triangular lattice with antiferromagnetic coupling for both intralayer nearest neighbor interaction and interlayer interaction is studied both…

强关联电子 · 物理学 2007-05-23 Ranjan Chaudhury

Inelastic neutron scattering (INS) from polycrystalline antiferromagnetic LaMnAsO, LaMnSbO, and BaMnAsF are analyzed using a $J_1-J_2-J_c$ Heisenberg model in the framework of the linear spin-wave theory. All three systems show clear…

$^{75}$As NMR measurements were performed on a polycrystalline sample of spin-1/2 alternating-spin-chain Heisenberg antiferromagnet AgVOAsO$_4$. Temperature-dependent NMR shift $K(T)$, which is a direct measure of the intrinsic spin…

材料科学 · 物理学 2017-12-27 N. Ahmed , P. Khuntia , H. Rosner , M. Baenitz , A. A. Tsirlin , R. Nath

Recently, several putative quantum spin liquid (QSL) states were discovered in ${\tilde S} = 1/2$ rare-earth based triangular-lattice antiferromagnets (TLAF) with the delafossite structure. A way to clarify the origin of the QSL state in…

The quest for Kitaev quantum spin liquids has led to great interest in honeycomb quantum magnets with strong spin-orbit coupling. It has been recently proposed that even Mott insulators with $3d$ transition metal ions, having nominally weak…

强关联电子 · 物理学 2021-11-25 Shreya Das , Sreekar Voleti , Tanusri Saha-Dasgupta , Arun Paramekanti

We study, on the basis of the general entangled-plaquette variational ansatz, the ground-state properties of the spin-1/2 antiferromagnetic Heisenberg model on the triangular lattice. Our numerical estimates are in good agreement with…

强关联电子 · 物理学 2015-05-19 Fabio Mezzacapo , J. Ignacio Cirac

Hybrid density functional calculations are performed for a variety of systems containing d9 ions (Cu2+, Ag2+), and exhibiting quasi-one-dimensional magnetic properties. In particular we study fluorides containing these ions in a rarely…

强关联电子 · 物理学 2017-11-01 Dominik Kurzydlowski , Wojciech Grochala

For temperatures T well above the ordering temperature T*=3.0+-0.2K the magnetic properties of the metal-organic material Mn[C10H6(OH)(COO)]2x2H20 built from Mn^2+ ions and 3-hydroxy-2-naphthoic anions can be described by a S=5/2 quantum…

Magnetic anisotropy in atomically thin correlated heterostructures is essential for exploring quantum magnetic phases for next-generation spintronics. Whereas previous studies have mostly focused on van der Waals systems, here, we…

Classical uniaxially anisotropic Heisenberg and XY antiferromagnets in a field along the easy axis on a square lattice are analysed, applying ground state considerations and Monte Carlo techniques. The models are known to display…

统计力学 · 物理学 2009-11-13 M. Holtschneider , W. Selke

Changes in the spin configuration of atomically-thin, magnetic van-der-Waals multilayers can cause drastic modifications in their opto-electronic properties. Conversely, the opto-electronic response of these systems provides information…

介观与纳米尺度物理 · 物理学 2020-05-28 Zhe Wang , Marco Gibertini , Dumitru Dumcenco , Takashi Taniguchi , Kenji Watanabe , Enrico Giannini , Alberto F. Morpurgo

The behavior in magnetic field of a paramagnetic center is characterized by its $g$ tensor. An anisotropic form of the latter implies different kind of response along different crystallographic directions. Here we shed light on the…

强关联电子 · 物理学 2019-12-04 Ziba Zangeneh , Stanislav Avdoshenko , Jeroen van den Brink , Liviu Hozoi

Chiral quantum magnets with spin-states separated by a large energy gap are technologically attractive but difficult to realize. Geometrically frustrated topological states with nanoscale chirality may offer a chemical pathway to such…

A quantum spin liquid (QSL) is an exotic state in which electron spins are highly entangled, yet keep fluctuating even at zero temperature. Experimental realization of model QSLs has been challenging due to imperfections, such as antisite…

Spangolite (Cu$_6$Al(SO$_4$)(OH)$_{12}$Cl$\cdot$3H$_2$O) is a hydroxy-hydrated copper sulfate mineral with a one-seventh depleted triangular lattice of Cu$^{2+}$ ions in each layer. Experimental measurements revealed a non-magnetic ground…

强关联电子 · 物理学 2025-08-18 Philipp Schmoll , Harald O. Jeschke , Yasir Iqbal

We study classical and quantum Heisenberg antiferromagnets with exchange anisotropy of XXZ-type and crystal field single-ion terms of quadratic and cubic form in a field. The magnets display a variety of phases, including the spin-flop (or,…

统计力学 · 物理学 2011-01-12 W. Selke , G. Bannasch , M. Holtschneider , I. P. McCulloch , D. Peters , S. Wessel

Nearly two decades ago, Alexei Kitaev proposed a model for spin-$1/2$ particles with bond-directional interactions on a two-dimensional honeycomb lattice which had the potential to host a quantum spin-liquid ground state. This work…

材料科学 · 物理学 2022-01-19 Faranak Bahrami , Mykola Abramchuk , Oleg I. Lebedev , Fazel Tafti

Inspired by the recently synthesized hexagonal layered phase of FeF$_2$, we studied the magnetic properties of the 1T-FeF$_2$ monolayer and its Janus Fe$X$F ($X$ = O, S) derivatives by first-principles calculations. Our results confirm that…

材料科学 · 物理学 2025-10-14 Xixiang Zhang , Busheng Wang , Yanfeng Ge , Yong Liu , Wenhui Wan