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Using the ab initio embedded DMFT (eDMFT) approach, we study the effect of long-range magnetic ordering on the spectral properties in the binary transition metal oxides, and find that the most significant changes appear in the momentum…

强关联电子 · 物理学 2019-12-11 Subhasish Mandal , Kristjan Haule , Karin M. Rabe , David Vanderbilt

Epitaxial strain in transition-metal oxides can induce dramatic changes in electronic and magnetic properties. A recent study on the epitaxially strained SrCoO$_3$ thin films revealed persistent ferromagnetism even across a metal-insulator…

Spin-state ordering - a periodic pattern of ions with different spin-state configurations along a crystal lattice - is a rare phenomenon, and its possible interrelation with other electronic degrees of freedom remains little explored. Here…

强关联电子 · 物理学 2024-03-27 E. Granado , C. W. Galdino , B. D. Moreno , G. King , D. C. Freitas

We study the electronic structure of cubic phase uranium dioxide at different volumes using a combination of density functional theory and dynamical mean-field theory. The \emph{ab initio} calculations predict an orbital-selective Mott…

强关联电子 · 物理学 2017-11-22 Li Huang , Yilin Wang , Philipp Werner

The subtle interplay between spin-orbit coupling, exchange interactions, and cation ordering can lead to exotic magnetic states in transition-metal ions. We report a comprehensive study of the Re-based (5$d^1$) ordered double perovskite…

We investigate the thickness-dependent electronic structure of ultrathin SrIrO$_3$ and discover a transition from a semimetallic to a correlated insulating state below 4 unit cells. Low-temperature magnetoconductance measurements show that…

We investigate the anomalous metal arising by hole doping the Mott insulating state of the periodic Anderson model. Using Dynamical Mean-Field Theory we show that, as opposed to the electron-doped case, in the hole-doped regime the…

强关联电子 · 物理学 2015-06-03 A. Amaricci , L. de Medici , G. Sordi , M. J. Rozenberg , M. Capone

Entanglement of spin and orbital degrees of freedom, via relativistic spin-orbit coupling, in 4$d$ transition metal oxides can give rise to a variety of novel quantum phases. A previous study of mixed 3$d$-4$d$ quasi-1D spin-chain oxide…

强关联电子 · 物理学 2025-02-10 A. Jain , D. T. Adroja , S. Rayaprol , A. D. Hillier , W. Kockelmann , S. M. Yusuf , E. V. Sampathkumaran

Ultrasound velocity measurements were performed on a single crystal of spin-frustrated ferrite spinel ZnFe$_2$O$_4$ from 300 K down to 2 K. In this cubic crystal, all the symmetrically-independent elastic moduli exhibit softening with a…

强关联电子 · 物理学 2015-11-26 Tadataka Watanabe , Shota Takita , Keisuke Tomiyasu , Kazuya Kamazawa

The optical orientation of Mn$^{2+}$ spins in the first excited state $^4$T$_1$ was experimentally observed in bulk (Zn, Mn)Se ($x_\mathrm{Mn}=0.01$) in the an external magnetic field of up to $6\,$T in Faraday geometry. This occurred…

介观与纳米尺度物理 · 物理学 2024-10-15 N. V. Kozyrev , K. A. Baryshnikov , B. R. Namozov , I. I. Kozlov , M. E. Boiko , N. S. Averkiev , Yu. G. Kusrayev

Cuprate superconductors remain central to condensed matter physics due to their technological relevance and unconventional, incompletely understood electronic behavior. While the canonical phase diagram and low-energy models have been…

$\alpha$-RuCl$_3$ is a promising candidate material to realize the so far elusive quantum spin liquid ground state. However, at low temperatures, the coexistence of different exchange interactions couple the effective pseudospins into an…

$Fe_3O_4$ is a mixed-valence strongly correlated transition metal oxide which displays the intriguing metal to insulator Verwey transition. Here we investigate the electronic and magnetic structure of $Fe_3O_4$ by a unique combination of…

The spin reorientation (SR) phenomenon of the square-lattice antiferromagnets RMnAsO (R = Ce, Nd) was investigated by analyzing the spin exchange interactions between the rare-earth and transition-metal ions (R3+ and Mn2+, respectively) on…

Muon-spin rotation (muSR) experiments are often used to study the magnetic field distribution in type-II superconductors in the vortex state. Based on the determination of the magnetic penetration depth it is frequently speculated---also…

超导电性 · 物理学 2011-10-31 B. M. Wojek , S. Weyeneth , S. Bosma , E. Pomjakushina , R. Puzniak

The crystal and magnetic structures of the spinel compounds ZnCr$_2$S$_4$ and ZnCr$_2$Se$_4$ were investigated by high resolution powder synchrotron and neutron diffraction. ZnCr$_2$Se$_4$ exhibits a first order phase transition at $T_N=21$…

We study theoretically the electronic states in a $5d$ transition metal oxide Na$_2$IrO$_3$, in which both the spin-orbit interaction and the electron correlation play crucial roles. Tight-binding model analysis together with the…

强关联电子 · 物理学 2009-06-25 Atsuo Shitade , Hosho Katsura , Jan Kunes , Xiao-Liang Qi , Shou-Cheng Zhang , Naoto Nagaosa

(MgFe)O is a solid solution with ferrous iron undergoing the high to low spin state (HS-LS) crossover under high pressure. The exact state of the material in the region of the crossover is still a mystery, as domains with different spin…

材料科学 · 物理学 2020-05-20 Konstantin Glazyrin , Saiana Khandarkhaeva , Leonid Dubrovinsky , Michael Sprung

We report muon spin relaxation ($\mu$SR) and magnetic susceptibility measurements on Cu(Cl,Br)La(Nb,Ta)$_{2}$O$_{7}$, which demonstrate: (a) the absence of static magnetism in (CuCl)LaNb$_{2}$O$_{7}$ down to 15 mK confirming a spin-gapped…

We investigate the evolution of the heavy fermion ground state under application of a strong external magnetic field. We present a richer version of the usual hybridization mean field theory that allows for hybridization in both the singlet…

强关联电子 · 物理学 2008-04-01 S. Viola Kusminskiy , K. S. D. Beach , A. H. Castro Neto , David K. Campbell
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