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We report on time-resolved ultrafast terahertz third-harmonic generation spectroscopy of nonequilibrium dynamics of Weyl fermions in a nanometer thin film of the Weyl semimetal TaP. Terahertz third-harmonic generation is observed at room…

We have prepared high-quality epitaxial thin films of CaRuO$_3$ with residual resistivity ratios up to 55. Shubnikov-de Haas oscillations in the magnetoresistance and a $T^2$ temperature dependence in the electrical resistivity only below…

We report strong terahertz (~10^12 Hz) high harmonic generation in thin films of Cd3As2, a three-dimensional Dirac semimetal at room temperature. The third harmonics is detectable with tabletop light source and can be as strong as 100 V/cm…

SrRuO$_3$, a ferromagnet with an approximately 160\,K Curie temperature, exhibits a $T^2$ dependent dc resistivity below $\approx$ 30 K. Nevertheless, previous optical studies in the infrared and terahertz range show non-Drude dynamics at…

We investigate the optical conductivity of Sr$_{1-x}$Ca$_x$RuO$_3$ across the ferromagnetic to paramagnetic transition that occurs at $x=0.8$. The thin films were grown by metalorganic aerosol deposition with $0 \leq x \leq 1$ onto…

We report on the observation of terahertz radiation in a non-centrosymmetric insulating oxide, paratellurite ($\alpha$-TeO$_2$) by irradiation of a femtosecond laser pulse at room temperature. In the power spectrum of the terahertz…

材料科学 · 物理学 2015-06-22 M. Sotome , N. Kida , R. Takeda , H. Okamoto

Terahertz high harmonic generation (THz HHG) is a common property of nonlinear systems. Recently it has been used to investigate fundamental principles that govern transport and nonlinear dynamics in novel quantum materials like graphene,…

We report on TmMnO3 far infrared emissivity and reflectivity spectra from 1910 K to 4 K. At the highest temperature the number of infrared bands is lower than that predicted for centrosymmetric P63/mmc (D6h4) (Z=2) space group due high…

Calcium ruthenate ($CaRuO_3$) is widely believed to be located close to a quantum critical point due to the strong non-Fermi-liquid behavior expressed in the temperature dependence of electronic transport, specific heat, optical…

强关联电子 · 物理学 2018-10-23 I. M. Bradarić , V. M. Matić , I. Savić , Hugo Keller

We report on far- and mid-infrared reflectivity of NdMnO3 from 4 K to 300K. Two main features are distinguished in the infrared spectra: active phonons in agreement with the expected for orthorhombic D2h 16-Pbnm (Z=4) space group remaining…

Recent terahertz-pump second-harmonic-generation(SHG)-probe measurements of quantum paraelectrics observed a significant long-lived non-oscillatory SHG component following an ultrafast resonant excitation of the soft mode, which was…

材料科学 · 物理学 2025-07-16 F. Yang , X. J. Li , D. Talbayev , L. Q. Chen

The charge density wave system K_0.3MoO_3 has been studied using variable energy pump-probe spectroscopy, ellipsometry, and inelastic light scattering. The observed transient reflectivity response exhibits quite a complex behavior,…

强关联电子 · 物理学 2009-11-11 D. M. Sagar , A. A. Tsvetkov , D. Fausti , S. van Smaalen , P. H. M. van Loosdrecht

The Drude model describes the free-electron conduction in simple metals, governed by the freedom that the mobile electrons have within the material. In strongly correlated systems, however, a significant deviation of the optical…

Direct experimental estimations of the low-energy ($1.5\sim10$ meV) complex dielectric constants spectrum and its temperature variation have been investigated for La$_{0.7}$Ca$_{0.3}$MnO$_3$ thin films using terahertz time-domain…

材料科学 · 物理学 2009-10-31 N. Kida , M. Hangyo , M. Tonouchi

A density-matrix formalism within the length gauge is developed for the purpose of calculating the nonlinear response of intrinsic bilayer graphene at terahertz frequencies. Employing a tight-binding model, we find that interplay between…

介观与纳米尺度物理 · 物理学 2016-12-07 Riley McGouran , Ibraheem Al-Naib , Marc M. Dignam

We present time-domain THz spectroscopy of thin films of the heavy-fermion superconductor CeCoIn$_5$. Below the $\approx$ 40 K Kondo coherence temperature, a narrow Drude-like peak forms, as the result of the $f$ orbital - conduction…

Recent experiments with strong THz fields in both conventional and unconventional superconductors have clearly evidenced a marked third-harmonic generation below the superconducting temperature $T_c$. Its interpretation challenged…

超导电性 · 物理学 2021-01-27 G. Seibold , M. Udina , C. Castellani , L. Benfatto

Harmonic generation provides an efficient tool for the study of ultrafast nonlinear dynamics. We report on time-resolved optical-pump terahertz-harmonic-generation spectroscopic investigation of ultrafast nonlinearity in a prototypical…

We report the temperature dependent THz to mid-infrared response of hexagonal-ErMnO3 using absorption, reflectivity, and emissivity techniques from 2 K to 1700 K. At low temperatures, lowest frequency vibrational modes coexist with…

The frequency dependence of third harmonic generation (THG) in C_{60} is calculated, making use of a tight-binding model for pi-electrons. The magnitudes of the THG, about 10^{-12} esu, near zero frequency, agree with those in experiments…

凝聚态物理 · 物理学 2007-05-23 Kikuo Harigaya , Shuji Abe
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