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The interplay between magnetism and light can create abundant optical phenomena. Here, we demonstrate the emergence of an unconventional magnetization-induced second-harmonic generation (MSHG) stemming from vector spin chirality, denoted as…

材料科学 · 物理学 2025-04-08 Dezhao Wu , Yong Xu , Meng Ye , Wenhui Duan

Spectroscopy of the centrosymmetric magnetic semiconductors EuTe and EuSe reveals spin-induced optical second harmonic generation (SHG) in the band gap vicinity at 2.1-2.4eV. The magnetic field and temperature dependence demonstrates that…

Recent experiments in the topological Weyl semimetal TaAs have observed record-breaking second-harmonic generation, a non-linear optical response at $2\omega$ generated by an incoming light source at $\omega$. However, whether…

Second harmonic generation (SHG), as one of the most significant \c{hi}(2) nonlinear optical processes, plays crucial roles in a broad variety of optical and photonic applications. Designing various delicate schemes to achieve highly…

光学 · 物理学 2021-09-01 Lei Wang , XiuQuan Zhang , Feng Chen

Since the first observation of second harmonic generation (SHG), there have been extensive studies on this nonlinear phenomenon not only to clarify its physical origin but also to realize unconventional functionalities. Nonetheless, a…

Altermagnets are a recently identified class of collinear antiferromagnets that host large spin-split electronic bands, offering a promising platform for efficient spin-current generation. Among proposed candidates, the metallic oxide RuO2…

We have studied second harmonic generation (SHG) in a polar ferrimagnet GaFeO_3, employing a FeO_6 cluster model in which the Fe atom is slightly shifted from the center of the octahedron. The electric-dipole transition could take place…

强关联电子 · 物理学 2015-05-19 Jun-ichi Igarashi , Tatsuya Nagao

An anomalous optical second-harmonic generation (SHG) signal was previously reported in Sr$_2$IrO$_4$ and attributed to a hidden odd-parity bulk magnetic state. Here we investigate the origin of this SHG signal using a combination of bulk…

强关联电子 · 物理学 2020-11-25 K. L. Seyler , A. de la Torre , Z. Porter , E. Zoghlin , R. Polski , M. Nguyen , S. Nadj-Perge , S. D. Wilson , D. Hsieh

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

软凝聚态物质 · 物理学 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

MnN is a centrosymmetric collinear antiferromagnet belonging to the transition metal nitride family with a high Neel temperature, a low anisotropy field, and a large magnetic moment per Mn atom. Despite several recent experimental and…

材料科学 · 物理学 2022-06-28 Joongwon Lee , Zexuan Zhang , Huili Xing , Debdeep Jena , Farhan Rana

Metallic nanostructures exhibit strong nonlinear-optical response at surface plasmon resonances, where the light-matter coupling efficiency is enhanced. An active modulation of this response can be realized by means of an external magnetic…

介观与纳米尺度物理 · 物理学 2020-05-29 Ilya Razdolski , Gaspar Armelles , Alfonso Cebollada , Andrey Kirilyuk

Second harmonic generation (SHG) extensively employs periodically poled nonlinear crystals through forward quasi-phase-matching to achieve efficient frequency conversion. As poling periods approach sub-micrometers, backward…

光学 · 物理学 2024-07-15 Fengyan Yang , Juanjuan Lu , Mohan Shen , Guangcanlan Yang , Hong X. Tang

Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…

Nonreciprocal devices that allow the light propagation in only one direction are indispensable in photonic circuits and emerging quantum technologies. Contemporary optical isolators and circulators, however, require large size or strong…

材料科学 · 物理学 2021-10-12 Shingo Toyoda , Manfred Fiebig , Taka-hisa Arima , Yoshinori Tokura , Naoki Ogawa

Second-harmonic generation (SHG) is a direct measure of the strength of second-order nonlinear optical effects, which also include frequency mixing and parametric oscillations. Natural and artificial materials with broken…

Understanding the mechanisms and spatial correlations of crystallographic symmetry breaking in ferroelectric materials is essential to tuning their functional properties. While optical second harmonic generation (SHG) has long been utilized…

材料科学 · 物理学 2022-08-10 Wei Li , Yunpeng Ma , Tianyi Feng , Sergei V. Kalinin , Jing-Feng Li , Qian Li

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…

Spin semimetals are amongst the most recently discovered new class of spintronic materials, which exhibit a band gap in one spin channel and semimetallic feature in the other, thus facilitating tunable spin transport. Here, we report…

Half-metallic ferromagnets show 100% spin-polarization at the Fermi level and are ideal candidates for spintronic applications. Despite the extensive research in the field, very few materials have been discovered so far. Here we present…

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