相关论文: Pulse Sequences to Observe NMR Coupled Relaxation …
A wide variety of nuclear magnetic resonance experiments rely on the prediction and analysis of relaxation processes. Recently, innovative approaches have been introduced where the sample travels through a broad range of magnetic fields in…
The NMR spectra of spin-1/2 pairs contains four peaks, with two inner peaks much stronger than the outer peaks in the near-equivalence regime. We have observed that the strong inner peaks have significantly different linewidths, when…
We show how to divide a coupled multi-spin system into a small subset of ``active'' spins that evolve under chemical shift or scalar coupling operators, and a larger subset of ``spectator'' spins which are returned to their initial states,…
We report an observation of extremely long-lived spin states in systems of dipolar-coupled nuclear spins in solids. The 'suspended echo' experiment uses a simple stimulated echo pulse sequence and creates non-equilibrium states which live…
In this work we experimentally study the efficiency of various dynamical decoupling sequences for suppressing decoherence of single as well as multiple quantum coherences on large spin-clusters. The system involves crystallites of a…
Multipulse sequences based on Carr-Purcell decoupling are frequently used for narrow-band signal detection in single spin magnetometry. We have analyzed the behavior of multipulse sensing sequences under real-world conditions, including…
Numerical modelling of coherent spin relaxation in nanomagnets, formed by magnetic molecules of high spins, is accomplished. Such a coherent spin dynamics can be realized in the presence of a resonant electric circuit coupled to the magnet.…
We propose two dimensional x-ray coherent correlation spectroscopy (2DXCS) for the study of interactions between core-electron and valence transitions. This technique might find experimental applications in the future when very high…
Dynamical decoupling multipulse sequences can be applied to solid state spins for sensing weak oscillating fields from nearby single nuclear spins. By periodically reversing the probing system's evolution, other noises are counteracted and…
The possibility that strongly correlated many-electron systems may exhibit spin-charge separation has generated great excitement, particularly in the light of recent experiments on low dimensional conductors and high temperature…
Phase structure of rapidly quenched solid helium samples is studied by the NMR technique. The pulse NMR method is used for measurements of spin-lattice $T_1$ and spin-spin $T_2$ relaxation times and spin diffusion coefficient $D$ for all…
Spin complexes comprising the nitrogen-vacancy (NV) center and neighboring spins are being considered as a building block for a new generation of spintronic and quantum information processing devices. Because assembling identical spin…
We investigate numerically the Multiple Quantum (MQ) NMR dynamics in systems of nuclear spins 1/2 coupled by the dipole-dipole interactions in the case of the pseudopure initial state. Simulations of the MQ NMR with the real molecular…
We demonstrate that CPMG and XYXY decoupling sequences with non-ideal $\pi$ pulses can reduce dipolar interactions between spins of the same species in solids. Our simulations of pulsed electron spin resonance (ESR) experiments show that…
The past decade has demonstrated increasing interests in using optimal control based methods within coherent quantum controllable systems. The versatility of such methods has been demonstrated with particular elegance within nuclear…
We study the decay of multiple quantum (MQ) NMR coherences in systems with the large number of equivalent spins. As being created on the preparation period of MQ NMR experiment, they decay due to the dipole-dipole interactions (DDI) on the…
Dense spin ensembles in solids present a natural platform for studying quantum many-body dynamics. Multiple-pulse coherent control can be used to manipulate the magnetic dipolar interaction between the spins to engineer their dynamics.…
We employ NMR techniques to investigate the nature of Mn spins in the I-II-V diluted magnetic semiconductor Li(Zn1-xMnx)P (x = 0.1, Curie temperature Tc = 25 K). We successfully identify the 7Li NMR signals arising from the Li sites…
The evolution of local spin polarization in finite systems involves interference phenomena that give rise to {\bf quantum dynamical echoes }and non-ergodic behavior. We predict the conditions to observe these echoes by exploiting the NMR…
We propose a new approach to the measurement of a single spin state, based on nuclear magnetic resonance (NMR) techniques and inspired by the coherent control over many-body systems envisaged by Quantum Information Processing (QIP). A…