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The duality between localized and itinerant nature of magnetism in $5\textit{f}$ electron systems has been a longstanding puzzle. Here, we report inelastic neutron scattering measurements, which reveal both local and itinerant aspects of…

The paper deals with the U based compound UPt$_2$Si$_2$ (UPS). The material was first treated as a localized 5f-electron system. Later, an opposite opinion of a predominantly itinerant nature of the system was put forward. The most recent…

强关联电子 · 物理学 2024-03-29 L. M. Sandratskii , V. M. Silkin , L. Havela

Uranium compounds can manifest a wide range of fascinating many-body phenomena, and are often thought to be poised at a crossover between localized and itinerant regimes for 5f electrons. The antiferromagnetic dipnictide USb2 has been of…

Magnetism of $UGe_2$ is due to the magnetic ordered moments of $5f$ uranium electrons. The strong spin-orbit coupling splits them into two groups. The magnetization is investigated in terms of two vector fields ${\bf M}_{1i}$ and ${\bf…

强关联电子 · 物理学 2015-03-17 Naoum Karchev

We consider singlet magnetism for the uranium ions in UPt$_3$ and URu$_2$Si$_2$ assuming that time-reversal symmetry is broken for the {\em coherent state of intermediate valence}. The relative weight of the two involved configurations…

凝聚态物理 · 物理学 2009-10-28 Victor Barzykin , Lev P. Gor'kov

The debate whether uranium 5f electrons are closer to being localized or itinerant in the ferromagnetic compound UGa2 is not yet fully settled. The experimentally determined magnetic moments are large, approximately 3 Bohr magnetons,…

强关联电子 · 物理学 2021-07-14 Banhi Chatterjee , Jindrich Kolorenc

Systematic experimental (vibrating sample magnetometry) and theoretical (electronic structure calculations using charge and spin self-consistent Korringa-Kohn-Rostoker Green function method) studies were performed on a series of…

强关联电子 · 物理学 2014-11-12 J. Cieslak , S. M. Dubiel , M. Reissner , J. Tobola

A consistent picture on the mean-field level of the magnetic properties and electronic structure of the superconducting itinerant ferromagnet UGe$_2$ is shown to require inclusion of correlation effects beyond the local density…

超导电性 · 物理学 2009-10-31 A. B. Shick , W. E. Pickett

The recent discovery of spin-triplet superconductivity emerging from a non-magnetic parent state in UTe$_2$ has stimulated great interest in the underlying mechanism of Cooper pairing. Experimental characterization of short-range electronic…

Materials containing non-Kramers magnetic ions can show unusual quantum excitations because of the exact mapping of the two-singlet crystal-field ground state to a quantum model of Ising spins in a transverse magnetic field. Here, we model…

Eu$_5$In$_2$Sb$_6$ is a member of a family of orthorhombic nonsymmorphic rare-earth intermetallics that combines large localized magnetic moments and itinerant exchange with a low carrier density and perpendicular glide planes. This may…

Recent calculations, concerning the magnetism of uranium in the U/Fe multilayer system have described the spatial dependence of the 5f polarization that might be expected. We have used the x-ray resonant magnetic reflectivity technique to…

We present a comparative investigation of singlet ground state induced magnetism for singlet, doublet and triplet excited CEF states of non-Kramers f-electrons relevant primarily for Pr- and U- based compounds. This type of magnetic order…

强关联电子 · 物理学 2024-03-11 Peter Thalmeier , Alireza Akbari

Single-crystalline UAu$_2$Si$_2$ has been grown by a floating-zone melting method, and its magnetic, thermal and transport properties have been investigated through measurements of magnetization, specific heat and electrical resistivity to…

Inelastic neutron scattering was used to study the low energy magnetic excitations of the ferromagnetic superconductor UGe$_{2}$. The ferromagnetic fluctuations are of Ising nature with a non-conserved magnetization and have an intermediate…

强关联电子 · 物理学 2009-11-10 S. Raymond , A. Huxley

Fe3-xGeTe2 is an itinerant ferromagnet composed of two-dimensional layers weakly connected by van der Waals bonding that shows a variety of intriguing phenomena. Inelastic neutron scattering measurements on bulk single crystals of…

强关联电子 · 物理学 2019-03-27 S. Calder , A. I. Kolesnikov , A. F. May

The one-dimensional cobaltate Ca3Co2O6 is an intriguing material having an unconventional magnetic structure, displaying quantum tunneling phenomena in its magnetization. Using a newly developed experimental method, s-core-level…

Magnetism in transition metal compounds is usually considered starting from a description of isolated ions, as exact as possible, and treating their (exchange) interaction at a later stage. We show that this standard approach may break down…

强关联电子 · 物理学 2016-10-24 S. V. Streltsov , D. I. Khomskii

We report a dc magnetization study of the critical phenomenon around the ferromagnetic transition temperature T_C in high-quality single crystals of uranium ferromagnetic superconductors UGe2 and URhGe. The critical exponents, beta for the…

超导电性 · 物理学 2014-03-26 Naoyuki Tateiwa , Yoshinori Haga , Tatsuma D. Matsuda , Etsuji Yamamoto , Zachary Fisk

The recent discovery that superconductivity occurs in several clean itinerant ferromagnets close to low temperature magnetic instabilities naturally invites an interpretation based on a proximity to quantum criticality. Here we report…

强关联电子 · 物理学 2009-11-07 C. Pfleiderer , A. D. Huxley
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