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Frustration-induced strong quantum fluctuations accompanied by spin-orbit coupling and crystal electric field can give rise to rich and diverse magnetic phenomena associated with unconventional low-energy excitations in rare-earth based…

强关联电子 · 物理学 2024-02-13 J. Khatua , S. Bhattacharya , A. M. Strydom , A. Zorko , J. S. Lord , A. Ozarowski , E. Kermarrec , P. Khuntia

The interplay between competing degrees of freedom can stabilize non-trivial magnetic states in correlated electron materials. Frustration-induced strong quantum fluctuations can evade long-range magnetic ordering leading to exotic quantum…

强关联电子 · 物理学 2023-10-12 B. Sana , M. Barik , M. Pregelj , U. Jena , M. Baenitz , J. Sichelschmidt , K. Sethupathi , P. Khuntia

The subtle interplay between competing degrees of freedom, crystal electric fields, and spin correlations can lead to exotic quantum states in 4f ion-based frustrated triangular lattice antiferromagnets. We present the crystal structure,…

Quantum magnets based on honeycomb lattices with low-coordination number offer a viable ground to realize exotic emergent quantum excitations and phenomena arising from the interplay between competing magnetic interactions, spin…

强关联电子 · 物理学 2024-11-14 J. Khatua , M. Gomilsek , Kwang-Yong Choi , P. Khuntia

We delineate quantum magnetism in the strongly spin-orbit coupled, distorted honeycomb-lattice antiferromagnet BiYbGeO$_{5}$. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an…

Frustration, spin correlations and interplay between competing degrees of freedom are some of the key ingredients that underlie exotic states with fractional excitations in quantum materials. Rare-earth based two dimensional magnetic…

强关联电子 · 物理学 2022-09-13 J. Khatua , M. Pregelj , A. Elghandour , Z. Jaglicic , R. Klingeler , A. Zorko , P. Khuntia

We report a comprehensive experimental investigation of the structural, thermodynamic, static, and dynamic properties of a triangular lattice antiferromagnet Rb$_3$Yb(VO$_4$)$_2$. Through the analysis of magnetic susceptibility,…

材料科学 · 物理学 2025-06-10 Sebin J. Sebastian , R. Kolay , Abhidev. B , Q. -P. Ding , Y. Furukawa , R. Nath

We present the magnetic properties of a strongly spin-orbit coupled quantum dimer magnet based on Co$^{2+}$. The metal-organic framework compound Co$_2$(BDC)$_2$(DPTTZ)$_2$$\cdot$DMF features Co$^{2+}$ dimers arranged nearly orthogonal to…

强关联电子 · 物理学 2023-11-29 Sebin J. Sebastian , S. Mohanty , A. Nath , M. P. Saravanan , S. Mandal , A. A. Tsirlin , R. Nath

Honeycomb iridate Na2IrO3, a Jeff=1/2 magnet, is a potential platform for realizing the quantum spin liquid. Many experiments have shown that its magnetic ground state has a zigzag antiferromagnetic (AFM) order. However, there is still a…

强关联电子 · 物理学 2018-09-05 Y. S. Hou , J. H. Yang , H. J. Xiang , X. G. Gong

The intertwining between competing degrees of freedom, anisotropy, and frustration-induced quantum fluctuations offers an ideal ground to realize exotic quantum phenomena in the rare-earth-based kagome lattice. The magnetic susceptibility…

We present the ground state properties of a new quantum antiferromagnet YbBO$_3$ in which the isotropic Yb$^{3+}$ triangular layers are separated by a non-magnetic layer of partially occupied B and O(2) sites. The magnetization and heat…

强关联电子 · 物理学 2022-10-19 K. Somesh , S. S. Islam , S. Mohanty , G. Simutis , Z. Guguchia , Ch. Wang , J. Sichelschmidt , M. Baenitz , R. Nath

The quantum dimer magnet, with antiferromagnetic intradimer and interdimer Heisenberg exchange between spin-1/2 moments, is known to host an up/down - down/up singlet ground state when the intradimer exchange is dominant. Rare-earth-based…

Two-dimensional high-spin bipartite honeycomb networks, where anisotropy, competing exchange interactions, and spin fluctuations interplay, provide an alternative platform to test theoretical models that distinguish between classical and…

强关联电子 · 物理学 2026-05-05 M. Barik , Q. Faure , F. Damay , J. P. Embs , S. Petit , P. Khuntia

The interplay of magnetic correlations, crystal electric field interactions, and spin-orbit coupling in low-dimensional frustrated magnets fosters novel ground states with unusual excitations. Here, we report the magnetic properties and…

材料科学 · 物理学 2024-09-02 S. Guchhait , A. Painganoor , S. S. Islam , J. Sichelschmidt , M. D. Le , N. B. Christensen , R. Nath

Most of the searches for Kitaev materials deal with $4d/5d$ magnets with spin-orbit-coupled ${J=1/2}$ local moments such as iridates and $\alpha$-RuCl$_3$. Here we propose the monoclinic YbCl$_3$ with a Yb$^{3+}$ honeycomb lattice for the…

The intriguing interplay between competing degrees of freedom in frustrated magnets can lead to non-trivial magnetic phenomena with exotic low-energy excitations that are highly relevant for addressing some of the fundamental questions in…

强关联电子 · 物理学 2026-03-20 A. Yadav , U. Jena , A. Pradhan , Satish K. , P. Khuntia

We report the magnetic properties in the Co- and Zn-doped spin-1/2 honeycomb-lattice compound In$_3$Cu$_2$VO$_9$. The magnetic susceptibility and specific heat experiments show no long-range ordering down to 2 K in In$_3$Cu$_2$VO$_9$. In…

强关联电子 · 物理学 2012-06-05 Y. J. Yan , Z. Y. Li , T. Zhang , X. G. Luo , G. J. Ye , Z. J. Xiang , P. Cheng , Liang-Jian Zou , X. H. Chen

We report on band structure calculations and a microscopic model of the low-dimensional magnet beta-Cu2V2O7. Magnetic properties of this compound can be described by a spin-1/2 anisotropic honeycomb lattice model with the averaged coupling…

强关联电子 · 物理学 2010-10-12 Alexander A. Tsirlin , Oleg Janson , Helge Rosner

Single crystal neutron diffraction, inelastic neutron scattering, bulk magnetization measurements, and first-principles calculations are used to investigate the magnetic properties of the honeycomb lattice $\rm Tb_2Ir_3Ga_9$. While the…

High-frequency ESR results on the S=1/2 Heisenberg hexagonal antiferromagnet InCu2/3V1/3O3 are reported. This compound appears to be a rare model substance for the honeycomb lattice antiferromagnet with very weak interlayer couplings. The…

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