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Nickelate superconductors are outstanding materials with intriguing analogies with the cuprates. These analogies suggest that their superconducting mechanism may be unconventional, although this fundamental question is currently under…

超导电性 · 物理学 2024-05-24 Q. N. Meier , J. B. de Vaulx , F. Bernardini , A. S. Botana , X. Blase , V. Olevano , A. Cano

Infinite-layer nickelate superconductors have recently been discovered to share both similarities and differences with cuprate superconductors. Notably, the incorporation of hydrogen (H) through topotactic reduction has been found to play a…

超导电性 · 物理学 2023-07-25 Chenye Qin , Mi Jiang , Liang Si

A key open question in the study of layered superconducting nickelate films is the role that hydrogen incorporation into the lattice plays in the appearance of the superconducting state. Due to the challenges of stabilizing highly…

Superconductivity has entered the nickel age marked by enormous experimental and theoretical efforts. Notwithstanding, synthesizing nickelate superconductors remains extremely challenging, not least due to incomplete oxygen reduction and…

超导电性 · 物理学 2022-08-29 Liang Si , Paul Worm , Karsten Held

Despite enormous experimental and theoretical efforts, obtaining generally accepted conclusions regarding the intrinsic magnetic and electronic properties of superconducting nickelates remains exceptionally challenging. Experiments show a…

材料科学 · 物理学 2023-04-19 Liang Si , Paul Worm , Dachuan Chen , Karsten Held

Employing combination of first-principles calculations, low-energy model construction, and variational Monte Carlo solution of the ab-initio derived Hubbard model, we study the effect of hydrogenation in the electronic structure and…

超导电性 · 物理学 2025-06-17 Manoj Gupta , Arun Kumar Maurya , Amal Medhi , Tanusri Saha Dasgupta

We present a theoretical prediction of a phonon-mediated two-gap superconductivity in infinite-layer nickelates Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ by performing $\textit{ab initio}$ $GW$ and $GW$ perturbation theory calculations. Electron $GW$…

超导电性 · 物理学 2024-09-20 Zhenglu Li , Steven G. Louie

Trilayer nickelates are a rich class of materials exhibiting diverse correlated phenomena, including superconductivity, density wave transitions, non-Fermi liquid behavior along with an unusual metal-to-metal transition around T* ~ 150 K.…

强关联电子 · 物理学 2025-12-04 Sonia Deswal , Deepu Kumar , Dibyata Rout , Surjeet Singh , Pradeep Kumar

Topotactic reduction utilizing metal hydrides as reagents emerges as an effective approach to achieve exceptionally low oxidization states of metal ions and unconventional coordination networks. This method opens avenues to the development…

Superconducting nickelates appear to be difficult to synthesize. Since the chemical reduction of ABO3 (A: rare earth; B transition metal) with CaH2 may result in both, ABO2 and ABO2H, we calculate the topotactic H binding energy by density…

强关联电子 · 物理学 2020-04-28 Liang Si , Wen Xiao , Josef Kaufmann , Jan M. Tomczak , Yi Lu , Zhicheng Zhong , Karsten Held

Hydrogen (H) plays a key role in the near-to-room temperature superconductivity of hydrides at megabar pressures. This suggests that H doping could have similar effects on the electronic and phononic spectra of materials at ambient pressure…

The observation of superconductivity in infinite-layer nickelates has attracted significant attention due to its potential as a new platform for exploring high $ \mathrm{\textit{T}}_{c} $ superconductivity. However, thus far,…

The dynamics of Higgs mode in superconductors, manifested as coherent oscillations of the superconducting order parameter amplitude, provides vital insights into the nature of the superconducting gap structure and symmetry. Here we utilize…

Superconductivity is one of the most intriguing properties of matter described by an attractive interaction that bounds electrons into Cooper pairs. To date, the highest critical temperature at ambient conditions is achieved in copper…

Since the discovery of superconductivity in infinite-layer nickelates RNiO$_2$ (R=La, Pr, Nd), great research efforts have been paid to unveil its underlying superconducting mechanism. However, the physical origin of the intriguing…

强关联电子 · 物理学 2022-07-20 T. Y. Xie , Z. Liu , Chao Cao , Z. F. Wang , J. L. Yang , W. Zhu

The discovery of superconducting nickelates provides a unique opportunity to explore the pairing mechanism of high-temperature superconductivity. Here, we use ultrafast terahertz spectroscopy to probe the temperature-dependent superfluid…

超导电性 · 物理学 2025-12-25 Qingming Huang , Xiaofang Fu , Junlong Wu , Laifeng Li , Liang Qiao , Ye Yang

Hydrogenation is known to tune superconductivity in a wide range of materials. While its microscopic role has been clarified in phonon-mediated superconductors such as hydrogenated MgB2, LaH10, and H3S, much less is known for hydrogenated…

超导电性 · 物理学 2026-04-29 Lan-Lin Du , Yang Yang , Shiqi Hu , Sheng Meng

We theoretically investigate the unconventional superconductivity in the newly discovered infinite-layer nickelates Nd$_{1-x}$Sr$_{x}$NiO$_{2}$ based on a two-band model. By analyzing the transport experiments, we propose that the doped…

超导电性 · 物理学 2020-12-08 Jun Chang , Jize Zhao , Yang Ding

The new family of superconducting nickelates centered around La$_{3}$Ni$_{2}$O$_{7}$ possesses attractive features, such as the high transition temperature and the presence of an antiferromagnetic ground state at ambient pressure,…

The discovery of pressurized superconductivity at 80 K in La3Ni2O7 officially brings nickelates into the family of high-temperature superconductors, which gives rise to not only new insights but also mysteries in the strongly correlated…

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