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We study the rotational diffusion of aging Laponite suspensions for a wide range of concentrations using depolarized dynamic light scattering. The measured orientational correlation functions undergo an ergodic to non-ergodic transition…

软凝聚态物质 · 物理学 2012-10-17 S. Jabbari-Farouji , G. H. Wegdam , Daniel Bonn

The ability to design artificial micro/nanomachines able to perform sophisticated tasks crucially depends on the understanding of their interaction with biosystems and their compatibility with the biological environment. Here, Janus…

软凝聚态物质 · 物理学 2024-03-18 Florent Fessler , Martin Wittman , Juliane Simmchen , Antonio Stocco

Colloidal gels formed by strongly attractive particles at low particle volume fractions are composed of space-spanning networks of uniformly sized clusters. We study the thermal fluctuations of the clusters using differential dynamic…

软凝聚态物质 · 物理学 2021-03-31 Jae Hyung Cho , Irmgard Bischofberger

Material failure is ubiquitous, with implications from geology to everyday life and material science. It often involves sudden, unpredictable events, with little or no macroscopically detectable precursors. A deeper understanding of the…

软凝聚态物质 · 物理学 2018-04-06 Stefano Aime , Laurence Ramos , Luca Cipelletti

Aging in an attraction-driven colloidal glass is studied by computer simulations. The system is equilibrated without attraction and instantaneously ``quenched'', at constant colloid volume fraction, to one of two states beyond the glass…

软凝聚态物质 · 物理学 2015-06-25 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

Within the mode-coupling theory for ideal glass-transitions, the mean-squared displacement and the correlation function for density fluctuations are evaluated for a colloidal liquid of particles interacting with a square-well potential for…

软凝聚态物质 · 物理学 2007-05-23 M. Sperl

We use dynamic light scattering and numerical simulations to study the approach to equilibrium and the equilibrium dynamics of systems of colloidal hard spheres over a broad range of density, from dilute systems up to very concentrated…

The physical gelation of colloids produces elastic structures that are commonly used to stabilize complex fluids in multiple industries. However, the ability to control the level of elastic modulus of these materials is limited by the…

软凝聚态物质 · 物理学 2021-12-21 Peng-Kai Kao , Michael J. Solomon , Mahesh Ganesan

Recent experiments have shown that colloidal suspensions can spontaneously self-assemble into dense clusters of various internal structures, sizes and dynamical properties when doped with active Janus particles. Characteristically, these…

软凝聚态物质 · 物理学 2020-01-29 Frederik Hauke , Hartmut Löwen , Benno Liebchen

Colloidal gels possess a memory of previous shear events, both steady and oscillatory. This memory, embedded in the microstructure, affects the mechanical response of the gel, and therefore enables precise tuning of the material properties…

软凝聚态物质 · 物理学 2022-03-10 Brice Saint-Michel , George Petekidis , Valeria Garbin

We investigated the viscoelastic properties of colloid-polymer mixtures at intermediate colloid volume fraction and varying polymer concentrations, thereby tuning the attractive interactions. Within the examined range of polymer…

软凝聚态物质 · 物理学 2008-12-05 M. Laurati , G. Petekidis , N. Koumakis , F. Cardinaux , A. B. Schofield , J. M. Brader , M. Fuchs , S. U. Egelhaaf

Active matter spans a wide range of time and length scales, from groups of cells and synthetic self-propelled particles to schools of fish, flocks of birds, or even human crowds. The theoretical framework describing these systems has shown…

The normal modes and relaxation rates of weak colloidal gels are investigated in computations employing different models of the hydrodynamic interactions between colloids. The eigenspectrum is computed for freely draining,…

流体动力学 · 物理学 2018-01-17 Zsigmond Varga , James W. Swan

We use x-ray photon correlation spectroscopy to investigate the dynamics of a high volume fraction emulsion creaming under gravity. The dodecane-in-water emulsion has interfaces stabilized solely by colloidal particles (silica). The samples…

软凝聚态物质 · 物理学 2009-11-13 E. M. Herzig , A. Robert , D. D. van 't Zand , L. Cipelletti , P. N. Pusey , P. S. Clegg

Natural and synthetic multi-component gels display emergent properties, which implies that they are more than just the sum of their components. This warrants the investigation of the role played by inter-species interactions in shaping gel…

软凝聚态物质 · 物理学 2024-11-15 Mauro L Mugnai , Rose Tchuenkam Batoum , Emanuela Del Gado

Using computer simulations, we identify the mechanisms causing aggregation and structural arrest of colloidal suspensions interacting with a short-ranged attraction at moderate and high densities. Two different non-ergodicity transitions…

凝聚态物理 · 物理学 2009-11-07 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

To gain insight into the kinetics of colloidal gel evolution at low particle volume fractions $\phi$, we utilize differential dynamic microscopy to investigate particle aggregation, geometric percolation, and the subsequent transition to…

软凝聚态物质 · 物理学 2020-03-02 Jae Hyung Cho , Roberto Cerbino , Irmgard Bischofberger

Light-activated self-propelled colloids are synthesized and their active motion is studied using optical microscopy. We propose a versatile route using different photoactive materials, and demonstrate a multiwavelength activation and…

软凝聚态物质 · 物理学 2014-10-28 J. Palacci , S. Sacanna , S. -H. Kim , G. -R. Yi , D. J. Pine , P. M. Chaikin

We systematically study the relationship between equilibrium and non-equilibrium phase diagrams of a system of short-ranged attractive colloids. Using Monte Carlo and Brownian dynamics simulations we find a window of enhanced…

软凝聚态物质 · 物理学 2009-11-13 Andrea Fortini , Eduardo Sanz , Marjolein Dijkstra

We report the modifications of the microscopic dynamics of a colloidal glass submitted to shear. We use multispeckle diffusing wave spectroscopy to monitor the evolution of the spontaneous slow relaxation processes after the sample have…

软凝聚态物质 · 物理学 2009-11-07 Virgile Viasnoff , Francois Lequeux