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Inelastic neutron scattering is used to study the magnetic excitations of the $S=1$ square-lattice antiferromagnet La$_2$NiO$_4$. We find that the spin waves cannot be described by a simple classical (harmonic) Heisenberg model with only…

We present a systematic study of spin and lattice dynamics in the quasi-one-dimensional spiral magnet CuBr2, using Raman scattering in conjunction with infrared and neutron spectroscopy. Along with the development of spin correlations upon…

Raman spectroscopy uses light scattering to extract information on low-energy excitations of solids. The Raman process is described by diagrams which are fourth order in the light-matter interaction, and in particular the resonant…

强关联电子 · 物理学 2024-01-30 Philipp Werner , Martin Eckstein , Naoto Tsuji

We present a general model study of surface-enhanced resonant Raman scattering and fluorescence, focusing on the interplay between electromagnetic (EM) effects and the molecular dynamics as treated by a density matrix calculation. The model…

其他凝聚态物理 · 物理学 2007-05-23 Peter Johansson , Hongxing Xu , Mikael Käll , ;

Anisotropic two-dimensional (2D) semiconductors recently have emerged as a promising platform for polarization-controlled Raman amplification. In this study, we probe energy-dependent resonant Raman scattering in few layer ReS2 under…

光学 · 物理学 2025-07-22 Pritam Das , Devarshi Chakrabarty , Neha Gill , Sajal Dhara

Investigation of dynamical excitations is difficult but crucial to the understanding of many exotic quantum phenomena discovered in quantum materials. This is particularly true for highly frustrated quantum antiferromagnets whose dynamical…

强关联电子 · 物理学 2022-11-24 Run-Ze Chi , Yang Liu , Yuan Wan , Hai-Jun Liao , T. Xiang

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

材料科学 · 物理学 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

We investigate the contribution of the low-energy electronic excitations towards the Raman spectrum of bilayer graphene for the incoming photon energy Omega >> 1eV. Starting with the four-band tight-binding model, we derive an effective…

介观与纳米尺度物理 · 物理学 2010-08-17 M. Mucha-Kruczynski , O. Kashuba , V. I. Fal'ko

We show that the low-energy peak in the polarized resonant Raman spectra of quantum wires, which is commonly associated with ``single particle excitations'', can be interpreted as signature of intra-band collective spin excitations. A broad…

强关联电子 · 物理学 2009-10-31 Maura Sassetti , Bernhard Kramer

Using resonant Raman scattering spectroscopy with 25 different laser lines, we describe the Raman scattering spectra of mono- and multi-layers 2H-molybdenum diselenide (MoSe$_2$) as well as the different resonances affecting the most…

介观与纳米尺度物理 · 物理学 2016-04-19 P. Soubelet , A. E. Bruchhausen , A. Fainstein , K. Nogajewski , C. Faugeras

We present a systematic experimental and theoretical study of the two-phonon (2D) Raman scattering in graphene under uniaxial tension. The external perturbation unveils that the 2D mode excited with 785nm has a complex line-shape mainly due…

Spin wave dispersion in the frustrated fcc type-III antiferromagnet MnS$_2$ has been determined by inelastic neutron scattering using a triple-axis spectrometer. Existence of multiple spin wave branches, with significant separation between…

强关联电子 · 物理学 2019-02-20 T. Chatterji , L. P. Regnault , S. Ghosh , A. Singh

The magnetic spectral response of black-phase mixed-valence Sm0.83Y0.17S has been measured by inelastic neutron scattering on a single crystal. Two magnetic peaks are observed in the energy range of the Sm2+ spin-orbit transition (25-40…

A theory of electronic Raman scattering in the presence of several energy bands crossing the Fermi surface is developed. The contributions to the light scattering cross section are calculated for each band and it is shown that the cross…

凝聚态物理 · 物理学 2009-10-28 T. P. Devereaux , A. Virosztek , A. Zawadowski

Early theoretical works on coherent anti-Stokes Raman scattering in optically active medium consider only heterodyne signal and subsequently, fourth- and fifth-rank tensor averages have been used. In this work, we presented a full signal…

量子物理 · 物理学 2019-01-03 Tuguldur Kh. Begzjav , Marlan O. Scully , Girish S. Agarwal

Although it is well accepted that the spin-$\frac{1}{2}$ triangular lattice Heisenberg antiferromagnet(TLHAF) has a long range ordered ground state, a thorough understanding of its spin dynamics is still missing. While the linear spin wave…

强关联电子 · 物理学 2020-08-12 Chun Zhang , Tao Li

Based on a two-band model, we study the electronic Raman scattering intensity in both normal and superconducting states of iron-pnictide superconductors. For the normal state, due to the match or mismatch of the symmetries between band…

超导电性 · 物理学 2015-03-19 C. S. Liu , W. C. Wu

The dipole-dipole interactions between excitons are of paramount importance in the nanoscale structures. When two excitons are placed together they can exchange the energy can manifest in the resonant Raman cross sections. We provide…

介观与纳米尺度物理 · 物理学 2024-04-09 Anna Wroblewska , Niclas S. Mueller , Mariusz Zdrojek , Stephanie Reich , Georgy Gordeev

Co-based materials have recently been explored due to potential to realise complex bond-dependent anisotropic magnetism. Prominent examples include Na$_2$Co$_2$TeO$_6$, BaCo$_2$(AsO$_4$)$_2$, Na$_2$BaCo(PO$_4$)$_2$, and CoX$_2$ (X = Cl, Br,…

We have performed polarized and temperature-dependent Raman scattering measurements on extremely large magnetoresitance compounds TaAs$_2$ and NbAs$_2$. In both crystals, all the Raman active modes, including six A$_g$ modes and three B$_g$…