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The realization and control of polaritons is of paramount importance in the prospect of novel photonic devices. Here, we investigate the emergence of plasmon-exciton polaritons in hybrid structures consisting of a two-dimensional (2D)…

介观与纳米尺度物理 · 物理学 2018-01-10 P. A. D. Gonçalves , L. P. Bertelsen , Sanshui Xiao , N. Asger Mortensen

Polaritons are compositional light-matter quasiparticles that have recently enabled remarkable breakthroughs in quantum and nonlinear optics, as well as in material science. Despite the enormous progress, however, a direct nanometer-scale…

Plexciton is the formation of new hybridized energy states originated from the coupling between plasmon and exciton. To reveal the optical properties of both exciton and plexciton, we develop a classic oscillator model to describe the…

光学 · 物理学 2022-07-12 Yuqing Cheng , Mengtao Sun

Hybrid systems of excitons strongly coupled to localized surface plasmons supported by metallic nanoparticles define a new approach to control light-matter interactions. Here, we report exciton-plasmon coupling in two-dimensional (2D)…

The advancement of quantum photonic technologies relies on the ability to precisely control the degrees of freedom of optically active states. Here, we realize real-time, room-temperature tunable strong plasmon-exciton coupling in 2D…

Plasmon-exciton polaritons provide exciting possibilities to control light-matter interactions at the nanoscale by enabling closer investigation of quantum optical effects and facilitating novel technologies based, for instance, on…

介观与纳米尺度物理 · 物理学 2020-02-25 Grigorios P. Zouros , Georgios D. Kolezas , N. Asger Mortensen , Christos Tserkezis

Transition-metal dichalcogenides with their exciton-dominated optical behavior emerge as promising materials for realizing strong light-matter interactions in the visible range and at ambient conditions. When these materials are combined…

Enhancement and active control of light-matter interactions at the atomic scale is important for developing next-generation nanophotonic and quantum optical devices. Here, we demonstrate electric control of both excitonic strong coupling…

We present an experimental demonstration of strong coupling between a surface plasmon propagating on a planar silver substrate, and the lowest excited state of CdSe nanocrystals. Variable-angle spectroscopic ellipsometry measurements…

材料科学 · 物理学 2009-12-16 D. E. Gómez , K. C. Vernon , T. J. Davis , T. L. Nguyen , P. Mulvaney

Strong coupling of two-dimensional semiconductor excitons with plasmonic resonators enables control of light-matter interaction at the subwavelength scale. Here we develop strong coupling in plasmonic nano-gap resonators that allow…

Strong interactions between surface plasmons in ultra-compact nanocavities and excitons in two dimensional materials have attracted wide interests for its prospective realization of polariton devices at room temperature. Here, we propose a…

The strong coherent coupling of quantum emitters to vacuum fluctuations of the light field offers opportunities for manipulating the optical and transport properties of nanomaterials, with potential applications ranging from ultrasensitive…

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

Semiconductor nanoparticles and nanostructures in the strong coupling regime exhibit an intriguing energy scale in the optical frequencies, which is specified by the Rabi splitting between the upper and lower exciton-polariton states.…

光学 · 物理学 2019-11-19 Burak Gerislioglu , Arash Ahmadivand

We investigate the conditions yielding plasmon-exciton strong coupling at the single emitter level in the gap between two metal nanoparticles. A quasi-analytical transformation optics approach is developed that makes possible a thorough…

介观与纳米尺度物理 · 物理学 2016-09-07 Rui-Qi Li , D. Hernangómez-Pérez , F. J. García-Vidal , A. I. Fernández-Domínguez

All-solid-state strong light-matter coupling systems with large vacuum Rabi splitting are great important for quantum information application, such as quantum manipulation, quantum information storage and processing. The monolayer…

介观与纳米尺度物理 · 物理学 2017-04-27 Jinxiu Wen , Hao Wang , Huanjun Chen , Shaozhi Deng , Ningsheng Xu

Formation of dressed light-matter states in optical structures, manifested as Rabi splitting of the eigen energies of a coupled system, is one of the key effects in quantum optics. In pursuing this regime with semiconductors, light is…

Strong-coupling of monolayer metal dichalcogenide semiconductors with light offers encouraging prospects for realistic exciton devices at room temperature. However, the nature of this coupling depends extremely sensitively on the optical…

Strong light-matter interactions between resonantly coupled metal plasmons and spin decoupled bright excitons from two dimensional (2D) transition metal dichalcogenides (TMDs) can produce discrete spin-resolved exciton-plasmon polariton…

介观与纳米尺度物理 · 物理学 2019-09-13 Rup Kumar Chowdhury , Prasanta Kumar Datta , Shivakiran Bhaktha BN , Samit Kumar Ray

Active control of light-matter interactions in semiconductors is critical for realizing next generation optoelectronic devices, with tunable control of the systems optical properties via external fields. The ability to manipulate optical…

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