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We report an experimental study of the longitudinal relaxation time ($T_1$) of the electron spin associated with single nitrogen-vacancy (NV) defects hosted in nanodiamonds (ND). We first show that $T_1$ decreases over three orders of…

介观与纳米尺度物理 · 物理学 2015-06-15 J. -P. Tetienne , T. Hingant , L. Rondin , A. Cavailles , L. Mayer , G. Dantelle , T. Gacoin , J. Wrachtrup , J. -F. Roch , V. Jacques

Nitrogen-vacancy (NV) centers in diamond are reliable single-photon emitters, with applications in quantum technologies and metrology. Two charge states are known for NV centers: NV$^0$ and NV$^-$, with the latter being mostly studied due…

光学 · 物理学 2019-12-23 Magdalena Solà-Garcia , Sophie Meuret , Toon Coenen , Albert Polman

We present an experimental study of the longitudinal electron-spin relaxation of ensembles of negatively charged nitrogen-vacancy (NV ) centers in diamond. The measurements were performed with samples having different NV- concentrations and…

原子物理 · 物理学 2015-05-12 M. Mrozek , D. Rudnicki , P. Kehayias , A. Jarmola , D. Budker , W. Gawlik

Shallow nitrogen-vacancy (NV) centers in diamond offer unique opportunities for studying photochemical reactions at the single-molecule level, such as the photogeneration of radical pairs in proximal molecules. A prerequesite for such…

The nitrogen-vacancy (NV) centre in diamond is emerging as a promising platform for solid-state quantum information processing and nanoscale metrology. Of interest in these applications is the manipulation of the NV charge, which can be…

We report the experimental study of the temperature-dependence of the longitudinal spin relaxation time $T_1$ of single Nitrogen-Vacancy (NV) centers hosted in nanodiamonds. To determine the relaxation mechanisms at stake, measurements of…

介观与纳米尺度物理 · 物理学 2020-11-04 Timothée de Guillebon , Baptiste Vindolet , Jean-François Roch , Vincent Jacques , Loïc Rondin

As promising quantum sensors, nitrogen-vacancy (NV) centers in diamond have been widely used in frontier studies in condensed matter physics, material sciences, and life sciences. In practical applications, weak laser excitation is…

Nitrogen vacancy (NV) centers in diamond are at the heart of many emerging quantum technologies, all of which require control over the NV charge state. Hence, methods for quantification of the relative photoluminescence (PL) intensities of…

We present systematic measurements of longitudinal relaxation rates ($1/T_1$) of spin polarization in the ground state of the nitrogen-vacancy (NV$^-$) color center in synthetic diamond as a function of NV$^-$ concentration and magnetic…

量子物理 · 物理学 2015-12-17 A. Jarmola , A. Berzins , J. Smits , K. Smits , J. Prikulis , F. Gahbauer , R. Ferber , D. Erts , M. Auzinsh , D. Budker

The fluorescent nitrogen-vacancy (NV) defect in diamond has remarkable photophysical properties, including high photostability, which allows stable fluorescence emission for hours; as a result, there has been much interest in using…

Nitrogen-vacancy (NV) centers in millimeter-scale diamond samples were produced by irradiation and subsequent annealing under varied conditions. The optical and spin relaxation properties of these samples were characterized using confocal…

The nitrogen-vacancy (NV) color center in diamond has demonstrated great promise in a wide range of quantum sensing. Recently, there have been a series of proposals and experiments using NV centers to detect spin noise of quantum materials…

介观与纳米尺度物理 · 物理学 2023-04-14 Jacob Henshaw , Pauli Kehayias , Luca Basso , Michael Jaris , Rong Cong , Michael Titze , Tzu-Ming Lu , Michael P. Lilly , Andrew M. Mounce

We present a study of the spin properties of dense layers of near-surface nitrogen-vacancy (NV) centres in diamond created by nitrogen ion implantation. The optically detected magnetic resonance contrast and linewidth, spin coherence time,…

Significant attention has been recently focused on the realization of high precision nano-thermometry using the spin-resonance temperature shift of the negatively charged nitrogen-vacancy (NV-) center in diamond. However, the precise…

Nitrogen-vacancy (NV) and silicon-vacancy (SiV) color defects in diamond are promising systems for applications in quantum technology. The NV and SiV centers have multiple charge states, and their charge states have different electronic,…

材料科学 · 物理学 2023-09-08 Artur Pambukhchyan , Sizhe Weng , Indu Aravind , Stephen B. Cronin , Susumu Takahashi

Chemical sensors with high sensitivity that can be used in extreme conditions and can be miniaturized are of high interest in science and industry. The Nitrogen-vacancy (NV) center in diamond is an ideal candidate as a nanosensor due to the…

量子物理 · 物理学 2021-02-16 Hossein T. Dinani , Enrique Muñoz , Jeronimo R. Maze

Quantum sensing with spin defects in diamond, such as the nitrogen-vacancy (NV) center, enables the detection of various chemical species on the nanoscale. Molecules or ions with unpaired electronic spins are typically probed by their…

Single charge detection with nanoscale spatial resolution in ambient conditions is a current frontier in metrology that has diverse interdisciplinary applications. Here, such single charge detection is demonstrated using two…

The charge state stability of nitrogen-vacancy (NV) centers critically affects their application as quantum sensors and qubits. Understanding charge state conversion and equilibration is critical not only for NV centers in diamond but also…

材料科学 · 物理学 2025-12-02 Audrius Alkauskas , Chris G. Van de Walle , Lukas Razinkovas , Ronald Ulbricht

Thanks to their versatility, nitrogen-vacancy (NV) centers in nanodiamonds have been widely adopted as nanoscale sensors. However, their sensitivities are limited by their short coherence times relative to NVs in bulk diamond. A more…

介观与纳米尺度物理 · 物理学 2020-03-09 Aedan Gardill , Matthew C. Cambria , Shimon Kolkowitz