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FePSe3 is a collinear honeycomb antiferromagnet with an easy-axis anisotropy and large spins S=2. It belongs to a family of magnetic van der Waals materials, which recently attracted a considerable attention. In this work we present an…

Magnon gap excitations selectively coupled to phonon modes have been studied in FePSe$_3$ layered antiferromagnet with magneto-Raman scattering experiments performed at different temperatures. The bare magnon excitation in this material has…

Recently it was discovered that van der Waals-bonded magnetic materials retain long range magnetic ordering down to a single layer, opening many avenues in fundamental physics and potential applications of these fascinating materials. One…

The hybridization of magnons (spin waves) with phonons, if sufficiently strong and comprising long wavelength excitations, may offer a new playground when manipulating the magnetically ordered systems with light. Applying a magnetic field…

Magnetic excitations are investigated for a hexagonal polar magnet Fe2Mo3O8 by terahertz spectroscopy. We observed magnon modes including an electric-field active magnon, electromagnon, in the collinear antiferromagnetic phase with spins…

强关联电子 · 物理学 2017-01-09 T. Kurumaji , Y. Takahashi , J. Fujioka , R. Masuda , H. Shishikura , S. Ishiwata , Y. Tokura

The Raman scattering response of the biaxial antiferromagnet CoPS$_3$ has been investigated as a function of both magnetic field and temperature. The peaks observed in the low-frequency spectral range (90--200~cm$^{-1}$) have been…

Ultrafast and coherent generation of magnons is of great significance for high-speed antiferromagnetic spintronics. One possible route is by exciton-magnon pairwise optical excitation. To date, such exciton-magnon transitions have been…

Magnetic layered materials have emerged recently as promising systems to introduce magnetism in structures based on two-dimensional (2D) materials and to investigate exotic magnetic ground states in the 2D limit. In this work, we apply high…

We combine polarized infrared magneto-transmission and Faraday angle rotation measurements to map the collective excitations of the van der Waals antiferromagnet FePS$_3$. Below the N\'{e}el temperature ($T_\mathrm{N} \approx 118$ K), the…

强关联电子 · 物理学 2025-08-21 Kartik Panda , Itzik Kapon , Dumitru Dumcenco , Dirk van der Marel , Alexey Kuzmenko , Nimrod Bachar

Emergent cooperative motions of individual degrees of freedom, i.e. collective excitations, govern the low-energy response of system ground states under external stimulations and play essential roles for understanding many-body phenomena in…

We report the emergence of a two-dimensional (2D) polar metal phase in van der Waals compound FePSe$_3$ under moderate pressures. This layered material is a Mott insulator with antiferromagnetic order under ambient conditions. We show that…

Spin-waves e.g. magnons are the conventional elementary excitations of ordered magnets. However, other possibilities exist. For instance, magnon bound-states can arise due to attractive magnon-magnon interactions and drastically impact the…

The control of antiferromagnets with ultrashort optical pulses has emerged as a prominent field of research. Tailored laser excitation can launch coherent spin waves at terahertz frequencies, yet a comprehensive description of their…

Magneto-spectroscopy methods have been employed to study the zero-wavevector magnon excitations in MnPSe$_3$. Experiments carried out as a function of temperature and the applied magnetic field show that two low-energy magnon branches of…

Optical magneto-spectroscopy methods (Raman scattering, far-infrared transmission, and photoluminescence) have been applied to investigate the properties of the NiPS3 semiconducting antiferromagnet. The fundamental magnon gap excitation in…

介观与纳米尺度物理 · 物理学 2023-06-14 Dipankar Jana , P. Kapuscinski , I. Mohelsky , D. Vaclavkova , I. Breslavetz , M. Orlita , C. Faugeras , M. Potemski

Collective excitations of bound electron-hole pairs -- known as excitons -- are ubiquitous in condensed matter, emerging in systems as diverse as band semiconductors, molecular crystals, and proteins. Recently, their existence in strongly…

In the rich phases of van der Waals (vdW) materials featuring intertwined electronic order and collective phenomena, characterizing elementary dynamics that entail the low-energy Hamiltonian and electronic degrees of freedom is of paramount…

Van der Waals (vdW) magnets are an ideal platform for tailoring two-dimensional (2D) magnetism with immense potential for spintronics applications and are intensively investigated. However, little is known about the microscopic origin of…

We report on optical excitations in the magnetically ordered phases of multiferroic Fe$_{1.86}$Zn$_{0.14}$Mo$_3$O$_8$ in the frequency range from 10-130 cm$^{-1}$ (0.3-3.9 THz). In the collinear easy-axis antiferromagnetic phase below…

强关联电子 · 物理学 2020-11-11 B. Csizi , S. Reschke , A. Strinic , L. Prodan , V. Tsurkan , I. Kézsmárki , J. Deisenhofer

Magnetic excitations in van der Waals (vdW) materials, especially in the two-dimensional (2D) limit, are an exciting research topic from both the fundamental and applied perspectives. Using temperature-dependent, magneto-Raman spectroscopy,…

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