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The nitrogen-vacancy (NV) center can serve as a magnetic sensor for electron paramagnetic resonance (EPR) measurements. Benefiting from its atomic size, the diamond chip can integrate a tremendous amount of NV centers to improve the…

Paramagnetic magnetic resonance, a powerful technique for characterizing and identifying chemical targets, is increasingly used for imaging; however, low spin polarization at room temperature and moderate magnetic fields poses challenges…

介观与纳米尺度物理 · 物理学 2019-09-04 C. M. Purser , V. P. Bhallamudi , C. S. Wolfe , H. Yusuf , B. A. McCullian , C. Jayaprakash , M. E. Flatté , P. C. Hammel

Electron paramagnetic resonance spectroscopy (EPR) is among the most important analytical tools in physics, chemistry, and biology. The emergence of nitrogen-vacancy (NV) centers in diamond, serving as an atomic-sized magnetometer, has…

An ultimate goal of electron paramagnetic resonance (EPR) spectroscopy is to analyze molecular dynamics in place where it occurs, such as in a living cell. The nanodiamond (ND) hosting nitrogen-vacancy (NV) centers will be a promising EPR…

The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

介观与纳米尺度物理 · 物理学 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

A key limitation of electron paramagnetic resonance (EPR), an established and powerful tool for studying atomic-scale biomolecular structure and dynamics is its poor sensitivity, samples containing in excess of 10^12 labeled biomolecules…

High concentration of negatively charged nitrogen-vacancy ($\text{NV}^{-}$) centers was created in diamond single crystals containing approximately 100 ppm nitrogen using electron and neutron irradiation and subsequent thermal annealing in…

A nitrogen-vacancy (NV) center in diamond is a promising sensor for nanoscale magnetic sensing. Here we report electron spin resonance (ESR) spectroscopy using a single NV center in diamond. First, using a 230 GHz ESR spectrometer, we…

介观与纳米尺度物理 · 物理学 2016-10-05 Chathuranga Abeywardana , Viktor Stepanov , Franklin H. Cho , Susumu Takahashi

Using an optical tweezers apparatus, we demonstrate three-dimensional control of nanodiamonds in solution with simultaneous readout of ground-state electron-spin resonance (ESR) transitions in an ensemble of diamond nitrogen-vacancy (NV)…

We propose an original analog method to perform instantaneous and quantitative spectral analysis of microwave signals. An ensemble of nitrogen-vacancy (NV) centers held in a diamond plate is pumped by a 532 nm laser. Its photoluminescence…

材料科学 · 物理学 2016-01-20 M. Chipaux , L. Toraille , C. Larat , L. Morvan , S. Pezzagna , J. Meijer , T. Debuisschert

Electron Spin Resonance (ESR) describes a suite of techniques for characterising electronic systems, with applications in physics, materials science, chemistry, and biology. However, the requirement for large electron spin ensembles in…

量子物理 · 物理学 2015-03-04 L. T. Hall , P. Kehayias , D. A. Simpson , A. Jarmola , A. Stacey , D. Budker , L. C. L. Hollenberg

We demonstrate a wide-band all-optical method of nanoscale magnetic resonance (MR) spectroscopy under ambient conditions. Our method relies on cross-relaxation between a probe spin, the electronic spin of a nitrogen-vacancy centre in…

We present a technique that uses an ensemble of nitrogen-vacancy (NV) centers in diamond to image magnetic fields with high spatio-temporal resolution and sensitivity. A focused laser beam is raster-scanned using an acousto-optic deflector…

Nitrogen-vacancy (NV) quantum defects in diamond are sensitive detectors of magnetic fields. Due to their atomic size and optical readout capability, they have been used for magnetic resonance spectroscopy of nanoscale samples on diamond…

Spectral analysis of electron spin resonance (ESR) is a powerful technique for various investigations including characterization of spin systems, measurements of spin concentration, and probing spin dynamics. The nitrogen-vacancy (NV)…

介观与纳米尺度物理 · 物理学 2019-07-19 Benjamin Fortman , Susumu Takahashi

Nitrogen-vacancy (NV) centers in millimeter-scale diamond samples were produced by irradiation and subsequent annealing under varied conditions. The optical and spin relaxation properties of these samples were characterized using confocal…

We present a new magnetometry method integrating an ensemble of nitrogen-vacancy (NV) centers in a single-crystal diamond with an extended dynamic range for monitoring the fast changing magnetic-field. The NV-center spin resonance frequency…

We perform pulsed optically detected electron spin resonance to measure the DC magnetic field sensitivity and electronic spin coherence time T_2 of an ensemble of near-surface, high-density nitrogen-vacancy (NV) centers engineered to have a…

介观与纳米尺度物理 · 物理学 2017-05-11 Kento Sasaki , Ed E. Kleinsasser , Zhouyang Zhu , Wen-Di Li , Hideyuki Watanabe , Kai-Mei C. Fu , Kohei M. Itoh , Eisuke Abe

In this paper cross-relaxation between nitrogen-vacancy (NV) centers and substitutional nitrogen in a diamond crystal was studied. It was demonstrated that optically detected magnetic resonance signals (ODMR) can be used to measure these…

Nitrogen vacancy (NV) color centers in diamond are a leading modality for both superresolution optical imaging and nanoscale magnetic field sensing. In this work, we solve the remaining key challenge of performing optical magnetic imaging…

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