相关论文: High-Pressure CO$_2$ Dissociation with Nanosecond …
We report first ns-resolved absorption measurements of the ro-vibrational excitation of CO$_2$. The high temporal resolution of 8 ns is made possible by a fast detector (rise-time 5 ns), sensitive in the mid-infrared region. The resolution…
In this work, evolution of parameters of nanosecond repetitively pulsed (NRP) discharges in pin-to-pin configuration in air was studied during transient stage of initial twenty discharge pulses. Gas and plasma parameters in the discharge…
The plasma dry reforming reaction of methane with carbon dioxide is investigated in a nanosecond repetitively pulsed discharge, a type of plasma that offers one of the highest non-equilibrium and performance characteristics. The…
In this contribution, nanosecond pulsed discharges in N$_{2}$ and N$_{2}$/0.9% H$_{2}$O at atmospheric pressure (at 300 K) are studied with time-resolved imaging, optical emission spectroscopy and Rayleigh scattering. A 170 ns high voltage…
A threefold increase in the CO2 conversion and energy efficiency due to the cooling of the post-discharge region by the counter gas flow has been achieved in the plasma of an atmospheric pressure discharge supported by microwave radiation…
Microwave plasmas are a promising technology for energy-efficient CO$_{2}$ valorization via conversion of CO$_{2}$ into CO and O$_2$ using renewable energies. A 2.45 GHz microwave plasma torch with swirling CO$_{2}$ gas flow is studied in a…
We present a novel microplasma flow reactor using a dielectric barrier discharge (DBD) driven by repetitively nanosecond high-voltage pulses. Our DBD-based geometry can generate a non-thermal plasma discharge at atmospheric pressure and…
CO2 conversion into value-added products has gained significant interest over the few last years, as the greenhouse gas concentrations constantly increase due to anthropogenic activities. Here we report on experiments for CO2 conversion by…
Nanosecond pulsed barrier discharges in atmospheric pressure argon are simulated using spatially one- and two-dimensional fluid-Poisson models using the reaction kinetics model presented by Stankov et al. [1], which considers all ten argon…
In this experimental study, a flowing dielectric barrier discharge operating at atmospheric pressure is used for the splitting of CO2 into O2 and CO. The influence of the applied frequency and plasma power on the microdischarge properties…
The 2.45 GHz plasma torch CO$_2\to$ CO + $\frac12$O$_2$ conversion experiment [F A D"Isa et al. Plasma Sources Sci. Technol., vol. 29 (2020) 105009] has been compared with thermo-chemical calculations. The 1.5D model of the…
Plasma processes are an innovative approach for the decomposition of CO2 in O radicals and CO as a valuable carbon source. In this experimental work, a tubular dielectric barrier discharge operating at atmospheric pressure has been used to…
In this work, we present an experimental study of nanosecond high-voltage discharges in a pin-to-pin electrode configuration at atmospheric conditions operating in single-pulse mode (no memory effects). Various discharge parameters,…
The kinetics of plasma assisted low temperature oxidation of C3H8O2Ar mixtures have been studied in a wide specific deposition energy with the help of nanosecond repetitively pulsed discharge. Two types of nanosecond pulsed plasma sources,…
Nanosecond and microsecond plasma-in liquid systems are explored to oxidize or regenerate a copper oxide surface in situ to serve as a catalyst for electrochemical CO$_2$ conversion. The plasma excitation generates H$_2$O$_2$ in the liquid,…
Non-equilibrium vibrational dissociation of CO$_2$ at low translational-rotational temperatures $T$ is investigated computationally for conditions of microwave induced plasmas. Semi-analytic treatment of vibrational relaxation in CO$_2$ in…
Nanosecond discharges are characterized by a shift in energy branching toward the excitation of electronic levels and dissociation, making them particularly attractive for plasma chemistry. Understanding the spatiotemporal structure of…
An influence of a high-voltage (3-17 kV) 20 ns pulse on a weakly-ionized low-pressure (0.1-10 Pa) capacitively-coupled radiofrequency (RF) argon plasma is studied experimentally. The plasma evolution after pulse exhibits two characteristic…
CO$_2$ dissociation stimulated by vibrational excitation in non-equilibrium discharges has drawn lots of attention. Ns-discharges are known for their highly non-equilibrium conditions. It is therefore of interest to investigate the CO$_2$…
In this work, we present the results of simulations carried out for N2-H2 capacitively coupled radio-frequency discharges, running at low pressure (0.3-0.9 mbar), low power (5-20 W), and for amounts of H2 up to 5 pct. Simulations are…