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相关论文: Fluorite-related iridate Pr$_3$IrO$_7$: Crystal gr…

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The synergy of strong spin-orbit coupling and electron-electron interactions gives rise to unconventional topological states, such as topological Mott insulator, Weyl semimetal, and quantum spin liquid. In this study, we have grown single…

强关联电子 · 物理学 2024-07-18 Harish Kumar , M. Köpf , P. Telang , N. Bura , A. Jesche , P. Gegenwart , C. A. Kuntscher

We report the growth of large high quality crystals of the frustrated magnet, Pr2Zr2O7 by the floating zone technique. Several crystals have been produced starting with varying levels of excess of Pr6O11 to compensate for the loss of Pr2O3…

材料科学 · 物理学 2016-11-09 M. Ciomaga Hatnean , C. Decorse , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan

We study the structural evolution of Sr$_3$Ir$_2$O$_7$ as a function of pressure using x-ray diffraction. At a pressure of 54 GPa at room temperature, we observe a first-order structural phase transition, associated with a change from…

Strong spin-orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin-orbit and strong electron-electron interactions is just beginning to be understood. Central…

Infrared reflection and transmission as a function of temperature have been measured on single crystals of Cu$_{3}$Bi(SeO$_{3}$)$_{2}$O$_{2}$Cl. The complex dielectric function and optical properties along all three principal axes of the…

材料科学 · 物理学 2015-06-05 K. H. Miller , P. W. Stephens , C. Martin , E. Constable , R. A. Lewis , H. Berger , G. L. Carr , D. B. Tanner

Pyrochlore $\rm Pr^{3+}_{2+x}Zr^{4+}_{2-x}O_{7-x/2}$ samples in the form of both powders $(-0.02 \le x \le 0.02)$ and bulk single crystals have been studied to elucidate the dependence of their magnetic, compositional and structural…

材料科学 · 物理学 2014-07-08 S. M. Koohpayeh , J. -J. Wen , B. A. Trump , C. L. Broholm , T. M. McQueen

The optical properties of a V4O7 single crystal have been investigated from the high temperature metallic phase down to the low temperature antiferromagnetic insulating one. The temperature dependent behavior of the optical conductivity…

强关联电子 · 物理学 2015-06-22 I. Lo Vecchio , M. Autore , F. D'Apuzzo , F. Giorgianni , A. Perucchi , U. Schade , V. N. Andreev , V. A. Klimov , S. Lupi

We report on near normal far- and mid-infrared emission and reflectivity of NdMnO3 perovskite from room temperature to sample decomposition above 1800 K. At 300 K the number infrared active phonons is in close agreement with the 25…

The $f$-$d$ magnetic exchange interaction is considered to be a key ingredient for many exotic topological phases in pyrochlore iridates. Here, we have investigated the evolution of structural, magnetic and electronic properties in doped…

强关联电子 · 物理学 2020-02-07 Harish Kumar , K. C. Kharkwal , Kranti Kumar , K. Asokan , A. Banerjee , A. K. Pramanik

Electrons in the pyrochore iridates experience a large interaction energy in addition to a strong spin-orbit interaction. Both features make the iridates promising for realizing novel states such as the Topological Mott Insulator. The…

强关联电子 · 物理学 2017-09-21 Tian Liang , Timothy H. Hsieh , Jun J. Ishikawa , Satoru Nakatsuji , Liang Fu , N. P. Ong

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

The frustrated pyrochlore iridate Pr$_2$Ir$_2$O$_7$ was proposed as a metallic quantum spin liquid located at a zero-field quantum critical point. Here we present the ultralow-temperature thermal conductivity measurements on the…

强关联电子 · 物理学 2022-08-23 J. M. Ni , Y. Y. Huang , E. J. Cheng , Y. J. Yu , B. L. Pan , Q. Li , L. M. Xu , Z. M. Tian , S. Y. Li

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

强关联电子 · 物理学 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

We have investigated the structural, electronic, and magnetic properties of the pyrochlore iridates Eu2Ir2O7 and Pr2Ir2O7 using a combination of resonant elastic x-ray scattering, x-ray powder diffraction, and resonant inelastic x-ray…

The infrared reflectivity of a $\rm La_{0.67}Ca_{0.33}MnO_3$ single crystal is studied over a broad range of temperatures (78-340 K), magnetic fields (0-16 T), and wavenumbers (20-9000 cm$^{-1}$). The optical conductivity gradually changes…

Crystal structure, electronic state of Ir$^{4+}$, and magnetic properties of the antifluorite compound K$_2$IrBr$_6$ are studied using high-resolution synchrotron x-ray diffraction, resonant inelastic x-ray scattering (RIXS), thermodynamic…

强关联电子 · 物理学 2021-04-02 Nazir Khan , Danil Prishchenko , Mary H. Upton , Vladimir G. Mazurenko , Alexander A. Tsirlin

SrRuO3 is a highly interesting material due to its anomalous-metal properties related with ferromagnetism and its relevance as conductive perovskite layer or substrate in heterostructure devices. We have used optical floating zone technique…

强关联电子 · 物理学 2016-06-02 S. Kunkemöller , F. Sauer , A. A. Nugroho , M. Braden

The orthorhombic perovskite SrIrO3 is a semimetal, an intriguing exception in iridates where the strong spin-orbit interaction coupled with electron correlations tends to impose a novel insulating state. We report results of our…

强关联电子 · 物理学 2016-07-06 H. Zheng , J. Terzic , Feng Ye , X. G. Wan , D. Wang , Jinchen Wang , Xiaoping Wang , P. Schlottmann , S. J. Yuan , G. Cao

Ir-based materials have drawn much attention due to the observation of insulating phase believed to be driven by spin-orbit coupling while Ir 5$d$ states are expected to be weakly correlated due to their large orbital extensions. IrO$_2$, a…

We present a combined study of the thermal expansion and the thermal conductivity of the perovskite series RCoO_3 with R = La, Nd, Pr and Eu. The well-known spin-state transition in LaCoO_3 is strongly affected by the exchange of the R ions…

强关联电子 · 物理学 2010-01-04 K. Berggold , M. Kriener , P. Becker , M. Benomar , M. Reuther , C. Zobel , T. Lorenz
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