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We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave and radio-frequency pulses to recursively transfer spin polarization from…

量子物理 · 物理学 2014-12-18 Daniela Pagliero , Abdelghani Laraoui , Jacob D. Henshaw , Carlos A. Meriles

After initial proof-of-principle demonstrations, optically pumped nitrogen-vacancy (NV) centres in diamond have been proposed as a non-invasive platform to achieve hyperpolarisation of nuclear spins in molecular samples over macroscopic…

介观与纳米尺度物理 · 物理学 2021-01-27 J. -P. Tetienne , L. T. Hall , A. J. Healey , G. A. L. White , M. -A. Sani , F. Separovic , L. C. L. Hollenberg

Solid-state electron spin qubits, like the nitrogen-vacancy center in diamond, rely on control sequences of population inversion to enhance sensitivity and improve device coherence. But even for this paradigmatic system, the fundamental…

The realisation of optically detected magnetic resonance via nitrogen vacancy centers in diamond faces challenges at high magnetic fields which include growing energy consumption of control pulses as well as decreasing sensitivities. Here…

量子物理 · 物理学 2018-11-01 J. Casanova , Z. -Y. Wang , I. Schwartz , M. B. Plenio

The ability to create time-dependent magnetic fields of controlled polarization is essential for many experiments with magnetic resonance. We describe a microstrip circuit that allows us to generate strong magnetic field at microwave…

原子物理 · 物理学 2015-05-28 Mariusz Mrozek , Janusz Mlynarczyk , Daniel S. Rudnicki , Wojciech Gawlik

Nitrogen-Vacancy (NV) centers in diamond are attractive tools for sensing and quantum information. Realization of this potential requires effective tools for controlling the spin degree of freedom by microwave (mw) magnetic fields. In this…

量子物理 · 物理学 2023-02-06 Anton Savitsky , Jingfu Zhang , Dieter Suter

The ability to optically initialize the electronic spin of the nitrogen-vacancy (NV) center in diamond has long been considered a valuable resource to enhance the polarization of neighboring nuclei, but efficient polarization transfer to…

介观与纳米尺度物理 · 物理学 2018-08-01 F. Shagieva , S. Zaiser , P. Neumann , D. B. R. Dasari , R. Stöhr , A. Denisenko , R. Reuter , C. A. Meriles , J. Wrachtrup

The nitrogen-vacancy (N-V) center in diamond is promising as an electron spin qubit due to its long-lived coherence and optical addressability. The ground state is a spin triplet with two levels ($m_s = \pm 1$) degenerate at zero magnetic…

其他凝聚态物理 · 物理学 2007-10-15 T. P. Mayer Alegre , C. Santori , G. Medeiros-Ribeiro , R. G. Beausoleil

The use of nitrogen-vacancy centers in diamond as a non-invasive platform for hyperpolarizing nuclear spins in molecular samples is a promising area of research with the potential to enhance the sensitivity of nuclear magnetic resonance…

量子物理 · 物理学 2024-08-08 H. Espinós , C. Munuera-Javaloy , I. Panadero , P. Acedo , R. Puebla , J. Casanova , E. Torrontegui

Optically polarizable nitrogen-vacancy (NV) center in diamond enables the hyperpolarization of $^{13}$C nuclear spins at low magnetic field and room temperature. However, achieving a high level of polarization comparable to conventional…

量子物理 · 物理学 2024-10-01 Vladimir V. Kavtanyuk , Changjae Lee , Keunhong Jeong , Jeong Hyun Shim

We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an…

量子物理 · 物理学 2021-04-21 P. Huillery , J. Leibold , T. Delord , L. Nicolas , J. Achard , A. Tallaire , G. Hétet

Recently, rotation sensors utilizing the nuclear spins of nitrogen-vacancy color centers in diamond have been demonstrated. However, these devices are power-intensive and challenging to integrate into small chip-based radiofrequency…

The nitrogen-vacancy (N-V) center in diamond is a widely-used platform for quantum information processing and metrology. The electron-spin state of N-V center could be initialized and readout optically, and manipulated by resonate microwave…

量子物理 · 物理学 2019-12-16 Yumeng Song , Yu Tian , Zhiyi Hu , Feifei Zhou , Tengteng Xing , Dawei Lu , Bing Chen , Ya Wang , Nanyang Xu , Jiangfeng Du

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

The nitrogen-vacancy (NV) centre in diamond has emerged as a candidate to non-invasively hyperpolarise nuclear spins in molecular systems to improve the sensitivity of nuclear magnetic resonance (NMR) experiments. Several promising proof of…

介观与纳米尺度物理 · 物理学 2021-05-26 A. J. Healey , L. T. Hall , G. A. L. White , T. Teraji , M. -A. Sani , F. Separovic , J. -P. Tetienne , L. C. L. Hollenberg

Individual nitrogen vacancy (NV) color centers in diamond are versatile, spin-based quantum sensors. Coherently controlling the spin of NV centers using microwaves in a typical frequency range between 2.5 and 3.5 GHz is necessary for…

材料科学 · 物理学 2021-08-23 Oliver Roman Opaluch , Nimba Oshnik , Richard Nelz , Elke Neu

We experimentally demonstrate high degree of polarization of 13C nuclear spins weakly interacting with nitrogen-vacancy (NV) centers in diamond. We combine coherent microwave excitation pulses with optical illumination to provide controlled…

量子物理 · 物理学 2019-10-25 Jiwon Yun , Kiho Kim , Dohun Kim

Defects in solid state materials provide an ideal, robust platform for quantum sensing. To deliver maximum sensitivity, a large ensemble of non-interacting defects hosting coherent quantum states are required. Control of such an ensemble is…

Nuclear spins in the solid state environment of diamond are highly coherent, but difficult to rapidly control due to the small nuclear gyromagnetic ratio. Here we demonstrate a more than 50-fold enhancement of the effective nuclear…

介观与纳米尺度物理 · 物理学 2016-08-05 S. Sangtawesin , J. R. Petta

High fidelity quantum control over qubits is of crucial importance for realistic quantum computing, and it turns to be more challenging when there are inevitable interactions among qubits. By employing a bandselective shaped pulse, we…

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