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Using a combination of high-temperature series expansion, exact diagonalization and quantum Monte Carlo, we perform a complementary analysis of the thermodynamic properties of quasi-one-dimensional mixed-spin systems with alternating…

强关联电子 · 物理学 2007-05-23 Noboru Fukushima , Andreas Honecker , Stefan Wessel , Wolfram Brenig

We present a model compound for the $S$=1/2 ferromagnetic Heisenberg chain composed of the verdazyl-based complex $[$Zn(hfac)$_2]$$[$4-Cl-$o$-Py-V-(4-F)$_2]$. $Ab$ $initio$ MO calculations indicate a predominant ferromagnetic interaction…

强关联电子 · 物理学 2019-03-19 N. Uemoto , Y. Kono , S. Kittaka , T. Sakakibara , T. Yajima , Y. Iwasaki , S. Miyamoto , Y. Hosokoshi , H. Yamaguchi

We study thermodynamic properties of the one-dimensional Heisenberg ferrimagnet with antiferromagnetically exchange-coupled two kinds of spins 1 and 1/2. The specific heat and the magnetic susceptibility are calculated employing a modified…

统计力学 · 物理学 2009-10-30 Shoji Yamamoto , Takahiro Fukui

We investigate the thermodynamic properties of Heisenberg ferrimagnetic mixed-spin chains both numerically and analytically with particular emphasis on the combination of ferromagnetic and antiferromagnetic features. Employing a new…

统计力学 · 物理学 2009-10-31 Shoji Yamamoto , Takahiro Fukui , Klaus Maisinger , Ulrich Schollwöck

We have succeeded in synthesizing single crystals of the verdazyl radical beta-2,6-Cl2-V [= beta-3-(2,6-dichlorophenyl)-1,5-diphenylverdazyl]. The ab initio MO calculation indicated the formation of an S = 1/2 Heisenberg antiferromagnetic…

强关联电子 · 物理学 2013-11-20 H. Yamaguchi , T. Okubo , K. Iwase , T. Ono , Y. Kono , S. Kittaka , T. Sakakibara , A. Matsuo , K. Kindo , Y. Hosokoshi

Motivated by a novel bimetallic chain compound in which alternating magnetic centers are ferromagnetically coupled, we investigate thermodynamic properties of one-dimensional spin-$(S,s)$ Heisenberg ferromagnets both numerically and…

统计力学 · 物理学 2009-11-11 Shoji Yamamoto , Hiromitsu Hori

We have implemented three approaches to describe the thermodynamic properties of ferrimagnetic ($S=5/2, s=2$) spin chains. The application of cumulant expansion has been generalized to the ferrimagnetic chain in the presence of an external…

强关联电子 · 物理学 2009-11-11 J. Abouie , S. A. Ghasemi , A. Langari

The thermodynamic properties of a spin S=1/2 tetrameric Heisenberg antiferromagnetic chain with alternating interactions AF1-AF2-AF1-F (AF and F denote the antiferromagnetic and ferromagnetic couplings, respectively) are studied by means of…

强关联电子 · 物理学 2009-07-11 Shou-Shu Gong , Song Gao , Gang Su

The magnetic and thermodynamic properties of a new ferrimagnetic decorated spin-(1/2,1) Heisenberg chain with spin-1 pendant spins are investigated for three cases: (A) J1,J2>0; (B) J1>0, J2<0; and (C) J1<0, J2>0, where J1 and J2 are the…

强关联电子 · 物理学 2010-06-23 Shou-Shu Gong , Wei Li , Yang Zhao , Gang Su

A spin-ice compound dysprosium titanate, Dy2Ti2O7, is studied by specific heat measurements in magnetic fields applied along the [110] direction of the cubic unit cell. Above a magnetic field of 0.4 T a relatively sharp peak at T = 1.1 K in…

材料科学 · 物理学 2009-11-10 Zenji Hiroi , Kazuyuki Matsuhira , Masao Ogata

Thermodynamic properties of a tetrameric bond-alternating Heisenberg spin chain with ferromagnetic-ferromagnetic-antiferromagnetic-antiferromagnetic exchange interactions are studied using the transfer-matrix renormalization group and…

强关联电子 · 物理学 2009-11-10 H. T. Lu , Y. H. Su , L. Q. Sun , J. Chang , C. S. Liu , H. G. Luo , T. Xiang

Using the quantum Monte Carlo Loop algorithm, we calculate the temperature dependence of the uniform susceptibility, the specific heat, the correlation length, the generalized staggered susceptibility and magnetization of a spin-1/2 chain…

凝聚态物理 · 物理学 2007-05-23 Beat Frischmuth , Manfred Sigrist , Beat Ammon , Matthias Troyer

We successfully synthesized a verdazyl-based complex, ($p$-Py-V-$p$-CN)$_2$[Cu(hfac)$_2$]. Molecular orbital calculations reveal that three types of antiferromagnetic (AF) interactions are involved in the formation of a spin-1/2 distorted…

We consider thermodynamic properties, e.g. specific heat, magnetic susceptibility, of alternating Heisenberg spin chains. Due to a hidden Ising symmetry these chains can be decomposed into a set of finite chain fragments. The problem of…

强关联电子 · 物理学 2009-10-30 H. Niggemann , G. Uimin , J. Zittartz

The ferrimagnetic spin-1/2 chain composed of alternating Ising and Heisenberg spins in an arbitrarily oriented magnetic field is exactly solved using the spin-rotation transformation and the transfer-matrix method. It is shown that the…

统计力学 · 物理学 2012-12-27 J. Strecka , M. Hagiwara , Y. Han , T. Kida , Z. Honda , M. Ikeda

We report high-resolution x-ray diffraction, muon-spin-rotation spectroscopic and specific heat measurements in the double spin-chains compound $\rm LiCu_2O_2$. The x-ray diffraction results show that the crystal structure of $\rm…

强关联电子 · 物理学 2009-10-31 B. Roessli , U. Staub , A. Amato , D. Herlach , P. Pattison , K. Sablina , G. A. Petrakovskii

The low-energy structure and the thermodynamic properties of ferrimagnetic Heisenberg chains of alternating spins $S$ and $s$ are investigated by the use of numerical tools as well as the spin-wave theory. The elementary excitations are…

统计力学 · 物理学 2009-10-31 Shoji Yamamoto , Takahiro Fukui , Toru Sakai

The thermodynamic properties (magnetization, magnetic susceptibility, transverse and longitudinal correlation lengths, specific heat) of one- and two-dimensional ferromagnets with arbitrary spin S in a magnetic field are investigated by a…

强关联电子 · 物理学 2009-11-13 I. Juhász Junger , D. Ihle , L. Bogacz , W. Janke

Motivated by recent magnetic measurements on A3Cu3(PO4)4 (A=Ca,Sr) and Cu(3-Clpy)2(N3)2 (3-Clpy=3-Chloropyridine), both of which behave like one-dimensional ferrimagnets, we extensively investigate the ferrimagnetic specific heat with…

强关联电子 · 物理学 2009-11-07 Takashi Nakanishi , Shoji Yamamoto

We present our theoretical and numerical results on thermodynamic properties and the microscopic mechanism of two successive transitions in vanadium spinel oxides $A$V$_2$O$_4$ ($A$=Zn, Mg, or Cd) obtained by Monte Carlo calculations of an…

强关联电子 · 物理学 2007-05-23 Yukitoshi Motome , Hirokazu Tsunetsugu
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