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The physical and chemical conditions in photodissociation regions (PDRs) are largely determined by the influence of far ultraviolet radiation. Far-UV photons can efficiently dissociate molecular hydrogen, a process that must be balanced at…
Using a semi-classical model, we study the formation of highly excited neutral fragments during the fragmentation of $\mathrm{H_3^+}$, a two-electron triatomic molecule, driven by an intense near-IR laser field. To do so, we first formulate…
Hydrogen as a fuel can be stored safely with high volumetric density in metals. It can, however, also be detrimental to metals causing embrittlement. Understanding fundamental behavior of hydrogen at atomic scale is key to improve the…
We study the formation of the RbCs molecule by an intense laser pulse using nonlinear dynamics. Under the Born-Oppenheimer approximation, the system is modeled by a two degree of freedom rovibrational Hamiltonian, which includes the ground…
The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…
We have reviewed the chemistry and cooling behaviour of low-density (n<10^4 cm^-3) primordial gas and devised a cooling model wich involves 19 collisional and 9 radiative processes and is applicable for temperatures in the range (1 K < T <…
A possible formation mechanism of hydrogen molecules on a galactic scale is examined. We are interested especially in the role of hydrogen molecules for formation and evolution of primordial galaxies. Then, formation process of hydrogen…
Triple Higgs boson production (3H) may provide essential information to reconstruct the Higgs potential. We consider 3H-production in the International Linear Collider (ILC) both in the Minimal Supersymmetric Standard Model (MSSM) and in…
Since its discovery in the aurorae of Jupiter ~30 years ago, the H$_{3}^{+}$ ion has served as an invaluable probe of giant planet upper atmospheres. However, the vast majority of monitoring of planetary H$_{3}^{+}$ radiation has followed…
We formulate a three-dimensional semi-classical model to treat three-electron escape dynamics in a strongly-driven linear triatomic molecule, HeH$_{2}^{+}$. Our model includes the Coulomb singularities. Hence, to avoid unphysical…
Most protoplanetary disks experience a phase in which they are subjected to strong ultraviolet radiation from nearby massive stars. This UV radiation can substantially alter their chemistry by producing numerous radicals and molecular ions.…
Diffuse interstellar clouds show large abundances of H_3^+ which can be maintained only by a high ionization rate of H_2. Cosmic rays are the dominant ionization mechanism in this environment, so the large ionization rate implies a high…
Chemistry in diffuse molecular clouds relies primarily on rapid ion-molecule reactions. Formation of the initial ions, H$^+$ and H$_2^+$, is dominated by cosmic-ray ionization of H and H$_2$, making the cosmic-ray ionization rate (denoted…
We present a channel-resolved interpretation of laser-driven Coulomb explosion of the HCl dimer from an ensemble of trajectories. Three dominant outcomes are identified: a minor three-body channel and two four-body channels (sequential and…
The relaxation dynamics of superexcited superfluid He nanodroplets is thoroughly investigated by means of extreme-ultraviolet (XUV) femtosecond electron and ion spectroscopy complemented by time-dependent density functional theory (TDDFT).…
The H3+ molecule has been detected in many lines of sight within the central molecular zone (CMZ) with exceptionally large column densities and unusual excitation properties compared to diffuse local clouds. The detection of the (3,3)…
Previous work has shown the Orion Bar to be an interface between ionized and molecular gas, viewed roughly edge on, which is excited by the light from the Trapezium cluster. Much of the emission from any star-forming region will originate…
Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…
We present the detection analysis of a diffuse molecular cloud at z$_{abs}$=2.4636 towards the quasar SDSS J1513+0352(z$_{em}\,\simeq$ 2.68) observed with the X-shooter spectrograph(VLT). We measure very high column densities of atomic and…
The sheer interstellar abundance of helium makes any bound molecules or complexes containing it of potential interest for astrophysical observation. This work utilizes high-level and trusted quantum chemical techniques to predict the…