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Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to coherently induce targeted structural deformations in solids. This form of dynamical crystal-structure design has been applied to control…

应用物理 · 物理学 2021-05-19 Meredith Henstridge , Michael Först , Edward Rowe , Michael Fechner , Andrea Cavalleri

The bulk photovoltaic effect (BPVE) refers to current generation due to illumination by light in a homogeneous bulk material lacking inversion symmetry. In addition to the intensively studied shift current, the ballistic current, which…

材料科学 · 物理学 2021-05-05 Zhenbang Dai , Aaron M. Schankler , Lingyuan Gao , Liang Z. Tan , Andrew M. Rappe

Ultrafast photocurrent experiments are performed on semiconducting, single-walled carbon nanotubes under a resonant optical excitation of their subbands. The photogenerated excitons are dissociated at large electric fields and the resulting…

介观与纳米尺度物理 · 物理学 2017-04-19 Christoph Karnetzky , Lukas Sponfeldner , Max Engl , Alexander W. Holleitner

The interplay between crystal symmetry and its optical responses is at the heart of tremendous recent advances in light-matter interactions and applications. Nonlinear optical processes that produce electric currents, for example bulk…

材料科学 · 物理学 2021-10-27 Yongliang Shi , Jian Zhou

Photodetection is an indispensable function of optoelectronic devices in modern communication and sensing systems. Contrary to the near-infrared/visible regions, the fast and sensitive photodetectors operated at room temperature for the…

Ultrafast optical control of ferroelectricity using intense terahertz fields has attracted significant interest. Here we show that the nonlinear interactions between two optical phonons in SnTe, a two-dimensional in-plane ferroelectric…

Theory of the Linear photogalvanic effect is developed for direct optical transitions between surface states of three-dimensional topological insulators. The photocurrent governed by the orientation of the polarization plane of light and…

介观与纳米尺度物理 · 物理学 2023-04-10 N. V. Leppenen , L. E. Golub

We report the optical excitation-dependent output photocurrent characteristics of GaN-based polariton diode lasers operated under reverse-bias at room temperature. The photocurrent demonstrates a non-linear enhancement at an incident…

Solid systems with strong correlations and interactions under light illumination have the potential for exhibiting interesting bulk photovoltaic behavior in the non-perturbative regime, which has remained largely unexplored in the past…

强关联电子 · 物理学 2022-04-06 Sangeeta Rajpurohit , C. Das Pemmaraju , Tadashi Ogitsu , Liang Z Tan

Amplification of light through stimulated emission or nonlinear optical interactions has had a transformative impact on modern science and technology. The amplification of other bosonic excitations, like phonons in solids, is likely to open…

Electronic transport in a model molecular device coupled to local phonon modes is theoretically analyzed. The method allows for obtaining an accurate approximation of the system's quantum state irrespective of the electron and phonon energy…

介观与纳米尺度物理 · 物理学 2007-10-10 Antonino La Magna , Ioannis Deretzis

The bulk photovoltaic effect (BPVE) has attracted an increasing interest due to its potential to overcome the efficiency limit of traditional photovoltaics, and much effort has been devoted to understanding its underlying physics. However,…

材料科学 · 物理学 2022-01-05 Zhenbang Dai , Andrew M. Rappe

We explore a novel coupling mechanism of electrons with the transverse optical (TO) phonon branch in a regime when the TO mode becomes highly anharmonic and drives the ferroelectric phase transition. We show that this anharmonicity, which…

强关联电子 · 物理学 2020-03-04 P. Chudzinski

The correlation between the shift current mechanism for the bulk photovoltaic effect (BPVE) and the structural and electronic properties of ferroelectric perovskite oxides is not well understood. Here, we study and engineer the shift…

材料科学 · 物理学 2015-03-03 Fenggong Wang , Steve M. Young , Fan Zheng , Ilya Grinberg , Andrew M. Rappe

Steady current in metals induces a thermal gradient, a phenomenon known as the Peltier effect. The Peltier effect is one of the fundamental phenomena in the thermoelectric properties of materials and is also used in applications such as…

介观与纳米尺度物理 · 物理学 2024-08-15 Hiroaki Ishizuka , Masahiro Sato

We introduce a variational wave-function to study the polaron formation when the electronic transfer integral depends on the relative displacement between nearest-neighbor sites giving rise to a non-local electron-phonon coupling with…

强关联电子 · 物理学 2009-11-10 C. A. Perroni , E. Piegari , M. Capone , V. Cataudella

Photogalvanic effect (PGE) occurring in noncentrosymmetric materials enables the generation of the open-circuit voltage that is much larger than the bandgap, making it rather attractive in solar cells. However, the magnitude of the PGE…

应用物理 · 物理学 2020-08-11 Juan Zhao , Yibin Hu , Yiqun Xie , Lei Zhang , Yin Wang

We report a comprehensive study of polarized infrared/terahertz photocurrents in bulk tellurium crystals. We observe different photocurrent contributions and show that, depending on the experimental conditions, they are caused by the…

介观与纳米尺度物理 · 物理学 2023-12-07 M. D. Moldavskaya , L. E. Golub , S. N. Danilov , V. V. Bel'kov , D. Weiss , S. D. Ganichev

Nonlinear phononics provides a route to control crystal structures through light-induced phonon excitation. In this study, we apply nonlinear phononics to an iron-based superconductor, LaFeAsO, with the aim of tuning its crystal structure…

超导电性 · 物理学 2026-04-09 Shu Kamiyama , Tatsuya Kaneko , Kazuhiko Kuroki , Masayuki Ochi

Nonlinear phononics play important role in strong laser-solid interactions. We discuss nonlinear dynamical protocols which allow for efficient excitation and control of nonlinear phonons. We consider recent inspiring proposals: inducing…

其他凝聚态物理 · 物理学 2018-05-16 A. P. Itin , M. I. Katsnelson
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