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In a honeycomb-lattice spin-orbit assisted Mott insulator {\alpha}-RuCl3, an ultrafast magnetization is induced by circularly polarized excitation below the Mott gap. Photo-carriers play an important role, which are generated by turning…

We theoretically investigate photoinduced phenomena induced by time-periodic driving fields in two-dimensional electron gases under perpendicular magnetic fields with Rashba spin-orbit coupling. Using perturbation theory, we provide…

介观与纳米尺度物理 · 物理学 2020-10-23 Daniel Hernangómez-Pérez , Juan Daniel Torres , Alexander López

We present time-resolved magneto-optical spectroscopy on the magnetic Mott-Hubbard-insulating Kitaev spin liquid candidate $\alpha$-RuCl$_3$ to investigate the nonequilibrium dynamics of its antiferromagnetically ordered zigzag groundstate…

{\alpha}-RuCl3 is a Kitaev material suggested to be a proximate quantum spin liquid in a certain temperature and magnetic field range. Nonequilibrium measurements of transient dynamics have been proposed to detect fractionalized particles…

强关联电子 · 物理学 2024-08-23 Haochen Zhang , Subin Kim , Young-June Kim , Hae-Young Kee , Luyi Yang

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

强关联电子 · 物理学 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

Recently considerable excitement has arisen due to the experimental observation of a field-induced spin liquid phase in the compound $\alpha$-RuCl$_3$. However, the nature of this putative spin liquid phase and the relevant microscopic…

强关联电子 · 物理学 2019-10-23 Yi-Fan Jiang , Thomas P. Devereaux , Hong-Chen Jiang

Photoinduced hidden phases are often observed in materials with intertwined orders. Understanding the formation of these non-thermal phases is challenging and requires a resolution of the cooperative interplay between different orders on…

强关联电子 · 物理学 2018-11-06 Jiajun Li , Hugo U. R. Strand , Philipp Werner , Martin Eckstein

Mott insulators with strong spin-orbit coupling have been proposed to host unconventional magnetic states, including the Kitaev quantum spin liquid. The 4$d$ system $\alpha$-RuCl$_3$ has recently come into view as a candidate Kitaev system,…

We study the spin-wave excitations in $\alpha$-RuCl$_3$ by the spin-wave theory. Starting from the five-orbital Hubbard model and the perturbation theory, we derive an effective isospin-$1/2$ model in the large Hubbard ($U$) limit. Based on…

强关联电子 · 物理学 2017-09-07 Wei Wang , Zhao-Yang Dong , Shun-Li Yu , Jian-Xin Li

The honeycomb compound $\alpha$-RuCl$_3$ is widely discussed as a proximate Kitaev spin-liquid material. This scenario builds on spin-orbit entangled $j = 1/2$ moments arising for a $t_{2g}^5$ electron configuration with strong spin-orbit…

Multiorbital Hubbard models with Hund coupling and crystal-field splitting exhibit an instability toward spin-triplet excitonic order in the parameter regime characterized by strong local spin fluctuations. Upon chemical doping, two…

强关联电子 · 物理学 2026-02-10 Lei Geng , Sujay Ray , Philipp Werner

We study periodically driven pure Kitaev model and ferromagnetic phase of the Kitaev-Heisenberg model on the honeycomb lattice by off-resonant linearly and circularly-polarized lights at zero magnetic field. Using a combination of linear…

强关联电子 · 物理学 2019-05-30 S. A. Owerre , Paula Mellado , G. Baskaran

Excitation by light pulses enables the manipulation of phases of quantum condensed matter. Here, we photoexcite high-energy holon-doublon pairs as a way to alter the magnetic free energy landscape of the Kitaev-Heisenberg magnet…

Novel ground states might be realized in honeycomb lattices with strong spin-orbit coupling. Here we study the electronic structure of ${\alpha}$-RuCl$_3$, in which the Ru ions are in a d5 configuration and form a honeycomb lattice, by…

Within the Floquet theory of periodically driven quantum systems, the nonlinear single-spin dynamics under pulse of a circularly polarized electromagnetic field is analyzed. It is demonstrated that the field, first, lifts the spin…

量子物理 · 物理学 2022-04-11 O. V. Kibis

A quantum spin-liquid might be realized in $\alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $\alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic…

Frustrated magnets with strong spin-orbit coupling promise to host topological states of matter, with fractionalized excitations and emergent gauge fields. Kitaev's proposal for a honeycomb-lattice Majorana spin liquid has triggered an…

强关联电子 · 物理学 2021-05-19 P. Lampen-Kelley , L. Janssen , E. C. Andrade , S. Rachel , J. -Q. Yan , C. Balz , D. G. Mandrus , S. E. Nagler , M. Vojta

We study the photoinduced ultrafast dynamics in relativistic Mott insulators, i.e., Mott insulators with strong spin-orbit coupling. For this purpose, we consider a minimal one-band Hubbard model on lattices with square and triangular…

强关联电子 · 物理学 2020-10-20 Jiajun Li , Nagamalleswararao Dasari , Martin Eckstein

Recent realization of well-controlled quantum simulators of the triangular-lattice Fermi-Hubbard model, including the triangular optical lattices loaded with ultracold Fermions and the heterostructures of the transition-metal…

量子气体 · 物理学 2022-09-15 Shuai A. Chen , Qianqian Chen , Zheng Zhu

The spin-orbit assisted Mott insulator $\alpha$-RuCl$_3$ is a prime candidate for material realization of the Kitaev quantum spin liquid. While little attention has been paid to charge degrees of freedom, charge effects, such as electric…

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