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Enhancement and active control of light-matter interactions at the atomic scale is important for developing next-generation nanophotonic and quantum optical devices. Here, we demonstrate electric control of both excitonic strong coupling…

Disentangling the contributions of radiative and non-radiative localized plasmonic modes from the photonic density of states of metallic nanocavities between atomically-sharp tips and flat substrates remains an experimental challenge…

The electroluminescence of molecules confined inside a nanocavity in the scanning tunneling microscopy possesses many intriguing but unexplained features. We present here a general theoretical approach based on the density matrix formalism…

介观与纳米尺度物理 · 物理学 2015-05-20 Guangjun Tian , Jicai Liu , Yi Luo

Atomic sized plasmonic tunnel junctions are of fundamental interest, with great promise as the smallest on-chip light sources in various optoelectronic applications. Several mechanisms of light emission in electrically driven plasmonic…

介观与纳米尺度物理 · 物理学 2022-11-09 Yunxuan Zhu , Longji Cui , Mahdiyeh Abbasi , Douglas Natelson

Plasmonic nanoparticles provide an ideal environment for the enhancement of fluorescent emission. On the one hand, they locally amplify the electromagnetic fields, increasing the emitter excitation rate, and on the other hand, they provide…

光学 · 物理学 2022-01-17 Henrikh M. Baghramyan , Cristian Ciracì

The accurate determination of electronic temperatures in metallic nanostructures is essential for many technological applications, like plasmon-enhanced catalysis or lithographic nanofabrication procedures. In this Letter we demonstrate…

The manipulation of coupled quantum excitations is of fundamental importance in realizing novel photonic and optoelectronic devices. We use electroluminescence to probe plasmon-exciton coupling in hybrid structures consisting of a nanoscale…

Plasmonic nanoantennas, metallodielectric structures with engineered size and shape, have attracted much attention lately as they make the control of the directionality and temporal characteristics of light emitted by fluorophores possible.…

Plasmonic cavities can be used to control the atom-photon coupling process at the nanoscale, since they provide ultrahigh density of optical states in an exceptionally small mode volume. Here we demonstrate strong coupling between molecular…

Plasmonic cavities can confine electromagnetic radiation to deep sub-wavelength regimes. This facilitates strong coupling phenomena to be observed at the limit of individual quantum emitters. Here we report an extensive set of measurements…

介观与纳米尺度物理 · 物理学 2021-02-03 Satyendra Nath Gupta , Ora Bitton , Tomas Neuman , Ruben Esteban , Lev Chuntonov , Javier Aizpurua , Gilad Haran

We present a methodology based on quantum mechanics for assigning quantum conductivity when an ac field is applied across a variable gap between two plasmonic nanoparticles with an insulator sandwiched between them. The quantum tunneling…

Inelastic electron tunneling in a scanning tunneling microscope (STM) is used to generate excitons in monolayer tungsten disulfide (WS$_2$). Excitonic electroluminescence is measured both at positive and negative sample bias. Using optical…

An efficient silicon based light source presents an unreached goal in the field of photonics, due to Silicons indirect electronic band structure preventing direct carrier recombination and subsequent photon emission. Here we utilize…

应用物理 · 物理学 2017-11-06 Hasan Göktaş Fikri Serdar Gökhan , Volker J. Sorger

We investigate the conditions yielding plasmon-exciton strong coupling at the single emitter level in the gap between two metal nanoparticles. A quasi-analytical transformation optics approach is developed that makes possible a thorough…

介观与纳米尺度物理 · 物理学 2016-09-07 Rui-Qi Li , D. Hernangómez-Pérez , F. J. García-Vidal , A. I. Fernández-Domínguez

Metamaterials exhibiting hyperbolic dispersion enable unprecedented control over light-matter interactions, from sub-diffraction imaging to enhanced spontaneous emission. However, conventional plasmonic hyperbolic metamaterials suffer from…

Control of excitons in transition metal dichalcogenides (TMDCs) and their heterostructures is fundamentally interesting for tailoring light-matter interactions and exploring their potential applications in high-efficiency optoelectronic and…

介观与纳米尺度物理 · 物理学 2023-06-13 Mahfujur Rahaman , Gwangwoo Kim , Kyung Yeol Ma , Seunguk Song , Hyeon Suk Shin , Deep Jariwala

We demonstrate that the emission of light by fluorescent molecules in the proximity of periodic arrays of nanoantennas or plasmonic crystals can be strongly modified when the arrays are covered by a dielectric film. The coupling between…

光学 · 物理学 2009-01-14 G. Vecchi , V. Giannini , J. Gómez Rivas

We develop a quantum master equation (QME) approach to investigate the electroluminesence (EL) of molecules confined between metallic electrodes and coupled to quantum plasmonic modes. Within our general state-based framework, we describe…

介观与纳米尺度物理 · 物理学 2018-03-06 Justin P. Bergfield , Joshua R. Hendrickson

We investigate plasmon-emitter interactions in a nanoparticle-on-a-mirror cavity. We consider two different sorts of emitters, those that sustain dipolar transitions, and those hosting only quadrupolar, dipole-inactive, excitons. By means…

介观与纳米尺度物理 · 物理学 2020-01-15 A. Cuartero-González , A. I. Fernández-Domínguez

Two-dimensional transition metal di-chalcogenide semiconductors provide unique possibilities to investigate strongly confined excitonic physics and a plasmonic platform integrable to such materials constitutes a hybrid system that can be of…

介观与纳米尺度物理 · 物理学 2022-05-26 Bidisha Roy , Maex Blauth , Siddharth Dhomkar , Michael Kaniber , Vinod M. Menon , Jonathan. J. Finley
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