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In a dynamic nuclear polarization experiment on a 40 mM solution of 4-amino-TEMPO in a 40:60 water/glycerol mixture, we have observed that the bulk dipolar reservoir is cooled to a spin temperature of 15.5 micro-K, following microwave…

其他凝聚态物理 · 物理学 2009-04-01 Anatoly E. Dementyev , David G. Cory , Chandrasekhar Ramanathan

We analyze the polarization of nuclear spins in a quantum dot induced by a single-electron spin that is electrically driven to perform coherent Rabi oscillations. We derive the associated nuclear-spin polarization rate and analyze its…

介观与纳米尺度物理 · 物理学 2023-10-25 Peter Stano , Takashi Nakajima , Akito Noiri , Seigo Tarucha , Daniel Loss

Experiments suggest that nuclear spins play a significant role in the quantum Hall effect (QHE) near integer and fractional QHE spin transitions, but many of these phenomena still remain to be understood. Here we study theoretically the…

介观与纳米尺度物理 · 物理学 2026-02-03 Haotian Zhou , Yuli Lyanda-Geller

We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times…

原子与分子团簇 · 物理学 2017-02-08 S. Sheludiakov , J. Ahokas , J. Järvinen , O. Vainio , L. Lehtonen , S. Vasiliev , D. M. Lee , V. V. Khmelenko

We propose a correction to the coefficient of nuclear-spin diffusion by a factor $1/\sqrt{1-\overline{p}^{2}}$, where $\overline{p}$ is the average nuclear-spin polarization. The correction, derived by extending the Lowe-Gade theory to…

其他凝聚态物理 · 物理学 2021-06-25 Yu Wang , Kazuyuki Takeda

Polarization transfers from an electron spin to a nuclear spin are essential for various physical tasks, such as dynamic nuclear polarization in nuclear magnetic resonance and quantum state transformations on hybrid electron-nuclear spin…

量子物理 · 物理学 2015-11-11 Haidong Yuan , Robert Zeier , Nikolas Pomplun , Steffen J. Glaser , Navin Khaneja

Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

介观与纳米尺度物理 · 物理学 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

The hyperpolarization of nuclear spins can enable powerful imaging and sensing techniques provided the hyperpolarization is sufficiently long-lived. Recent experiments on nanodiamond $^{13}$C nuclear spins demonstrate that relaxation times…

介观与纳米尺度物理 · 物理学 2024-02-20 Gargee Sharma , Torsten Gaebel , Ewa Rej , David J. Reilly , Sophia E. Economou , Edwin Barnes

We analytically solve the {\it Non-Markovian} single electron spin dynamics due to hyperfine interaction with surrounding nuclei in a quantum dot. We use the equation-of-motion method assisted with a large field expansion, and find that…

介观与纳米尺度物理 · 物理学 2009-11-11 Changxue Deng , Xuedong Hu

Nuclear-spin diffusion in double quantum wells (QWs) is examined by using dynamic nuclear polarization (DNP) at a Landau level filling factor $\nu=2/3$ spin phase transition (SPT). The longitudinal resistance increases during the DNP of one…

介观与纳米尺度物理 · 物理学 2015-04-01 T. Hatano , W. Kume , S. Watanabe , K. Akiba , K. Nagase , Y. Hirayama

Low thermal polarization of nuclear spins is a primary sensitivity limitation for nuclear magnetic resonance. Here we demonstrate optically pumped (microwave-free) nuclear spin polarization of $^{13}\mathrm{C}$ and $^{15}\mathrm{N}$ in…

介观与纳米尺度物理 · 物理学 2017-08-09 Ben L. Green , Ben G. Breeze , Gregory J. Rees , John V. Hanna , Jyh-Pin Chou , Viktor Ivády , Adam Gali , Mark E. Newton

We studied spatial distribution of dynamic nuclear polarization (DNP) in a Hall-bar device in a breakdown regime of the quantum Hall effect (QHE). We detected nuclear magnetic resonance (NMR) signals from the polarized nuclear spins by…

介观与纳米尺度物理 · 物理学 2011-01-25 Minoru Kawamura , Kimitoshi Kono , Yoshiaki Hashimoto , Shingo Katsumoto , Tomoki Machida

The interplay of optical driving and hyperfine interaction between an electron confined in a quantum dot and its surrounding nuclear spin environment produces a range of interesting physics such as mode-locking. In this work, we go beyond…

介观与纳米尺度物理 · 物理学 2024-03-12 Arian Vezvaee , Gargee Sharma , Sophia E. Economou , Edwin Barnes

We report on a polarized-neutron Laue diffraction experiment on a single crystal of neodynium doped lanthanum magnesium nitrate hydrate containing polarized proton spins. By using dynamic nuclear polarization to polarize the proton spins,…

Efficient hyperpolarisation of nuclear spins via optically active defect centers, such as the nitrogen vacancy (NV) center in diamond, has great potential for enhancing NMR based quantum information processing and nanoscale magnetic…

Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday…

介观与纳米尺度物理 · 物理学 2019-04-04 E. Evers , T. Kazimierczuk , F. Mertens , D. R. Yakovlev , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer , A. Greilich

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

化学物理 · 物理学 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is…

介观与纳米尺度物理 · 物理学 2019-02-04 Thomas Nutz , Edwin Barnes , Sophia E. Economou

Dynamic nuclear polarization (DNP) is an attractive method for initializing nuclear spins that are strongly coupled to optically active electron spins because it functions at room temperature and does not require strong magnetic fields. In…