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Glasses derive their functional properties from complex relaxation dynamics that remain enigmatic under extreme conditions. While the temperature dependence of these relaxation processes is well-established, their behavior under…

We present a study of the relaxation dynamics of the photoexcited conductivity of the impurity states in the low-density electronic glass, phosphorous-doped silicon Si:P. Using optical pump-terahertz probe spectroscopy we find strongly…

无序系统与神经网络 · 物理学 2010-09-16 V. K. Thorsmølle , N. P. Armitage

We theoretically investigate the temperature dependence of the reversible structural relaxation time and diffusion constant of metallic glasses under pressure. The compression not only changes the glassy dynamics, but also generates a…

材料科学 · 物理学 2021-05-28 Nguyen K. Ngan , Anh D. Phan , Alessio Zaccone

Densified SiO2 glasses, obtained from different pressure and temperature routes have been annealed over a wide range of temperature far below the glass transition temperature (500$^\circ$C-900$^\circ$C). Hot and cold compressions were…

While lot of measurements describe the relaxation dynamics of the liquid state, experimental data of the glass dynamics at high temperatures are much scarcer. We use ultrafast scanning calorimetry to expand the timescales of the glass to…

The effect of tensile stress applied during cooling of binary glasses on the potential energy states and mechanical properties is investigated using molecular dynamics simulations. We study the three-dimensional binary mixture that was…

软凝聚态物质 · 物理学 2021-01-01 Nikolai V. Priezjev

The time evolution of the pore size distributions and mechanical properties of amorphous solids at constant pressure is studied using molecular dynamics simulations. The porous glasses were initially prepared at constant volume conditions…

软凝聚态物质 · 物理学 2018-10-22 Nikolai V. Priezjev , Maxim A. Makeev

We present results of temperature dependent measurements of dynamics of micellar nanoparticle - polymer composites of fixed volume fraction and variable polymer chain grafting density. For nanoparticles with lower grafting density we…

软凝聚态物质 · 物理学 2008-09-12 A. K. Kandar , S. Srivastava , J. K. Basu , M. K. Mukhopadhyay , S. Seifert , S. Narayanan

The relaxation dynamics of glass-forming systems shows a multitude of features that are absent in normal liquids, such as non-exponential relaxation and a strong temperature-dependence of the relaxation time. Connecting these dynamic…

无序系统与神经网络 · 物理学 2019-04-03 Zhen Wei Wu , Walter Kob , Wei-Hua Wang , Limei Xu

We investigated the dynamics of a series of room temperature ionic liquids based on the same 1-butyl-3-methyl imidazolium cation and different anions by means of broadband dielectric spectroscopy covering 15 decades in frequency…

无序系统与神经网络 · 物理学 2009-11-11 Alberto Rivera , Ernst A. Roessler

Glasses encode the memory of any thermo-mechanical treatment applied to them. This ability is associated to the existence of a myriad of metastable amorphous states which can be probed through different experimental pathways. It is usually…

Thermal conductivity of a model glass-forming system in the liquid and glass states is studied using extensive numerical simulations. We show that near the glass transition temperture, where the structural relaxation time becomes very long,…

无序系统与神经网络 · 物理学 2020-02-26 Pranab Jyoti Bhuyan , Rituparno Mandal , Pinaki Chaudhuri , Abhishek Dhar , Chandan Dasgupta

The onset of structural arrest and glass formation in a concentrated suspension of silica nanoparticles in a water-lutidine binary mixture near its consolute point is studied by exploiting the near-critical fluid degrees of freedom to…

软凝聚态物质 · 物理学 2009-11-13 Xinhui Lu , S. G. J. Mochrie , S. Narayanan , A. R. Sandy , M. Sprung

We report a thorough characterization of the dielectric relaxation behavior and the ionic conductivity in the plastic-crystalline mixture of 60% succinonitrile and 40% glutaronitrile. The plastic phase can be easily supercooled and the…

无序系统与神经网络 · 物理学 2011-02-16 Th. Bauer , M. Köhler , P. Lunkenheimer , A. Loidl , C. A. Angell

The process of structural relaxation in disordered solids subjected to repeated tension-compression loading is studied using molecular dynamics simulations. The binary glass is prepared by rapid cooling well below the glass transition…

软凝聚态物质 · 物理学 2020-05-04 Pritam Kumar Jana , Nikolai V. Priezjev

A central question concerning glass-formation has been what governs the kinetic arrest of the quenched liquid - cooling reduces the thermal energy which molecules need to surmount local potential barriers, while the accompanying volume…

软凝聚态物质 · 物理学 2007-05-23 CM Roland R Casalini

Glass-forming liquids have only a modest tendency to crystallize and hence their dynamics can be studied even below the melting temperature. The relaxation dynamics of most of these liquids shows at a temperature $T_c$, somewhat above the…

软凝聚态物质 · 物理学 2025-01-17 Francesco Rusciano , Raffaele Pastore , Francesco Greco , Walter Kob

Acoustic levitation is a container-free method for examining novel crystallization effects, though liquid-to-solid phase change has seen little investigation for levitated nanofluids. Recent developments have allowed for examining the…

应用物理 · 物理学 2024-09-13 Adam McElligott , André Guerra , Alejandro D. Rey , Phillip Servio

We investigate the effect of a single heat treatment cycle on the potential energy states and mechanical properties of metallic glasses using molecular dynamics simulations. We consider the three-dimensional binary mixture, which was…

软凝聚态物质 · 物理学 2019-06-14 Nikolai V. Priezjev

Upon cooling, glass-forming liquids experience a two-step relaxation associated to the cage rattling and the escape from the cage, and the following decoupling between the \b{eta}- and the {\alpha}-relaxations. The found decoupling…

无序系统与神经网络 · 物理学 2017-06-07 P. Luo , P. Wen , H. Y. Bai , B. Ruta , W. H. Wang
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