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We investigate the dynamics of water confined in soft ionic nano-assemblies, an issue critical for a general understanding of the multi-scale structure-function interplay in advanced materials. We focus in particular on hydrated…

材料科学 · 物理学 2017-08-23 Quentin Berrod , Samuel Hanot , Armel Guillermo , Stefano Mossa , Sandrine Lyonnard

We study the electrophoretic flow of suspensions of charged colloids with a mesoscopic method that allows to model generic experimental conditions. We show that for highly charged colloids their electrophoretic mobility increases…

软凝聚态物质 · 物理学 2015-05-28 Giovanni Giupponi , Ignacio Pagonabarraga

Surface charges play a fundamental role in physics and chemistry, particularly in shaping the catalytic properties of nanomaterials. Tracking nanoscale surface charge dynamics remains challenging due to the involved length and time scales.…

A migration of charged particles relative to a solvent, caused by a gradient of salt concentration and termed a diffusiophoresis, is of much interest being exploited in many fields. Existing theories deal with diffusiophoresis of passive…

软凝聚态物质 · 物理学 2024-10-15 Evgeny S. Asmolov , Olga I. Vinogradova

Recent experimental work has suggested that electroosmotic flows (EOF) through conical nanopores exhibit rectification in the opposite sense to the well-studied effect of ionic current rectification. A positive bias voltage generates large…

流体动力学 · 物理学 2015-06-02 Nadanai Laohakunakorn , Ulrich F. Keyser

A field theoretic variational approach is introduced to study ion penetration into water-filled cylindrical nanopores in equilibrium with a bulk reservoir. It is shown that (i) an ion located in a neutral pore undergoes two opposing…

软凝聚态物质 · 物理学 2015-05-19 Sahin Buyukdagli , Manoel Manghi , John Palmeri

Surface-bound electric charge on polymer materials can strongly influence droplet behaviour and solid-liquid charge transfer, but the mechanisms and the means to control these effects remain unclear. In this work, we systematically…

With the ability to selectively control ionic flux, biological protein ion channels perform a fundamental role in many physiological processes. For practical applications that require the functionality of a biological ion channel, graphene…

Guiding and confining light at interfaces is crucial for applications involving light-matter interactions such as surface spectroscopy, nonlinear optics, and quantum information technology. While dielectric surface waves offer promising…

We demonstrate that the driving forces for ion adsorption to the air-water interface for point charge models results from both cavitation and a term that is of the form of a negative electrochemical surface potential. We carefully…

软凝聚态物质 · 物理学 2013-07-08 Marcel D. Baer , Abraham C. Stern , Yan Levin , Douglas J. Tobias , Christopher J. Mundy

Energy harvesting from evaporation has become a hot topic in the last couple of years. Researchers have speculated on several possible mechanisms. Electrokinetic energy conversion is the least hypothetical one. The basics of pressure-driven…

软凝聚态物质 · 物理学 2022-07-21 Andriy Yaroshchuk

Alloyed metal nanoparticles are a promising platform for plasmonically enabled hot-carrier generation, which can be used to drive photochemical reactions. Although the non-plasmonic component in these systems has been investigated for its…

介观与纳米尺度物理 · 物理学 2024-08-15 Jakub Fojt , Tuomas P. Rossi , Priyank V. Kumar , Paul Erhart

We model and simulate a nanopore sensor that selectively binds analyte ions. This binding leads to the modulation of the local concentrations of the ions of the background electrolyte (KCl), and, thus, to the modulation of the ionic current…

应用物理 · 物理学 2019-11-07 Eszter Mádai , Mónika Valiskó , Dezső Boda

The electro-osmotic flow (EOF) in a neutral system consisting of an aqueous NaCl solution confined in a nanochannel with two parallel Molybdenum disulfide ($\textrm{MoS}_{\textrm{2}}$) walls and in the presence of an external electric field…

软凝聚态物质 · 物理学 2023-12-04 S. M. Kazem Manzoorolajdad , Hossein Hamzehpour , Jalal Sarabadani

We investigate a model nanopore sensor that is able to detect analyte ions that are present in the electrolyte solution in very small concentrations. The nanopore selectively binds the analyte ions with which the local concentrations of the…

应用物理 · 物理学 2018-12-31 Eszter Mádai , Mónika Valiskó , Dezső Boda

Electric-field-driven electrolyte transport through nanoporous membranes is important for applications including osmotic power generation, sensing and iontronics. We derive an analytical equation in the Debye--H\"uckel regime and a…

软凝聚态物质 · 物理学 2026-05-01 Holly C. M. Baldock , David M. Huang

The interaction of ultrashort, high intensity laser pulses with thin foil targets leads to ion acceleration on the target rear surface. To make this ion source useful for applications, it is important to optimize the transfer of energy from…

等离子体物理 · 物理学 2017-04-05 M. Blanco , M. T. Flores-Arias , C. Ruiz , M. Vranic

In this study, we innovatively modeled photon-enhanced thermionic emission (PETE) devices, incorporating positive ion injection and bidirectional discharge's effects on the space charge barrier simultaneously. Compared to previous models,…

加速器物理 · 物理学 2025-02-27 Xinqiao Lin , Zhiqiang Fan , Shunjie Zhang , Xiaohang Chen , Zhimin Yang , Jincan Chen , Shanhe Su

The fundamental aspect of physics of ferroelectric materials is the screening of uncompensated bound charges by the dissociative adsorption of ionic charges from the environment. The adsorption of ions can be especially strong when the…

材料科学 · 物理学 2025-02-04 Sergei V. Kalinin , Eugene A. Eliseev , Anna N. Morozovska

The interface properties of interest in multilayers include interfacial charge densities, dipole densities, band offsets, and screening-lengths, among others. Most such properties are inaccesible to direct measurements, but are key to…

材料科学 · 物理学 2009-11-13 Javier Junquera , Morrel H. Cohen , Karin M. Rabe